We develop a general Hamiltonian treatment of spontaneous four-wave mixing in a microring resonator side-coupled to a channel waveguide. The effect of scattering losses in the ring is included, as well as parasitic nonlinear effects including self- and cross-phase modulation. A procedure for computing the output of such a system for arbitrary parameters and pump states is presented. For the limit of weak pumping an expression for the joint spectral intensity of generated photon pairs, as well as the singles-to-coincidences ratio, is derived.
We develop a general Hamiltonian treatment of spontaneous four-wave mixing in a microring resonator side-coupled to a channel waveguide. The effect of scattering losses in the ring is included, as well as parasitic nonlinear effects including self- and cross-phase modulation. A procedure for computing the output of such a system for arbitrary parameters and pump states is presented. For the limit of weak pumping an expression for the joint spectral intensity of generated photon pairs, as well as the singles-to-coincidences ratio, is derived.
We present a detailed analysis of strongly driven spontaneous four-wave mixing in a lossy integrated microring resonator side coupled to a channel waveguide. A nonperturbative, analytic solution within the undepleted pump approximation is developed for a cw pump input of arbitrary intensity. In the strongly driven regime self- and cross-phase modulation, as well as multipair generation, lead to a rich variety of power-dependent effects; the results are markedly different than in the low-power limit. The photon-pair generation rate, single-photon spectrum, and joint spectral intensity (JSI) distribution are calculated. Splitting of the generated single-photon spectrum into a doublet structure associated with both pump detuning and cross-phase modulation is predicted, as well as substantial narrowing of the generated signal and idler bandwidths associated with the onset of optical parametric oscillation at intermediate powers. Both the correlated and the uncorrelated contributions to the JSI are calculated, and for sufficient powers the uncorrelated part of the JSI is found to form a quadruplet structure. The pump detuning is found to play a crucial role in all of these phenomena, and a critical detuning is identified which divides the system behavior into distinct regimes, as well as an optimal detuning strategy which preserves many of the low-power characteristics of the generated photons for arbitrary input power.
We present two complementary strategies for modeling nonlinear quantum optics in realistic resonant integrated optical devices, where scattering loss is present. In the first strategy, we model scattering loss as an effective absorption; in the second, we employ a Hamiltonian treatment, with the loss modelled as a coupling to a 'phantom' channel. As an example, we use these two approaches to model spontaneous four-wave mixing in (i) a ring-channel system and (ii) an add-drop system. We present the rates of photon pairs, broken pairs, and lost pairs for both systems, as well as the full biphoton wavefunction (BWF) including the effects of scattering. We find that for a high-finesse resonator coupled to an arbitrary number of channels, the full BWF can be extracted from the BWF associated with photon pairs in an experimentally accessible output channel.
We investigate entangled photon-pair generation in a lossy microring resonator using an input-output formalism based on the work of M. G. Raymer and C. J. McKinstrie [Phys. Rev. A 88, 043819 (2013)] and P. M. Alsing et al. [Phys. Rev. A 95, 053828 (2017)] that incorporates circulation factors that account for the multiple round-trips of the fields within the cavity. We consider the nonlinear processes of spontaneous parametric down-conversion and spontaneous four-wave mixing, and we compute the generated biphoton signal-idler state from a single-bus microring resonator, along with the generation, coincidence-to-accidental, and heralding efficiency rates. We compare these generalized results to those obtained by previous works employing the standard Langevin input-output formalism.
Microring resonators (MRR) are becoming a standard resource for highly efficient entangled photon pair generation. We examine the nonlinear processes in MRR using an input-output formalism that explicitly accounts for the contribution of the round trip circulation of the fields inside the MRR. This formalism reduces to the standard Langevin operator input-output formalism for cavities in the high cavity Q limit, near cavity resonances. Our approach is more general, applicable for arbitrary internal and bus-ring coupling losses, and away from resonances. We compare/contrast these two formalisms, and apply our approach to the output quantum state resulting from spontaneous parametric down conversion and spontaneous four wave mixing within the MRR. We compare our results to similar calculations employing the standard IO formalism, and note the role of the commutators of the noise operators on the undesired accidental singles rate.
This thesis presents an analysis of photon pairs generated via either spontaneous parametric downconversion or spontaneous four-wave mixing in channel waveguides as well as in microring resonators side-coupled to channel waveguides. The state of photons exiting a particular device is calculated within a general Hamiltonian formalism that simplifies the link between quantum nonlinear optics experiments and classical nonlinear optics experiments. This state contains information regarding photon pair production efficiency as well as modal and spectral correlations between the two photons, characterized by a two-dimensional spectral distribution function called the biphoton wave function.\n\nIn the limit of a low probability of pair production, photon pair production fficiencies are cast into forms resembling corresponding well-known classical nonlinear optical frequency conversion efficiencies, making it easy to see what plays the role of a classical “seed” field in an un-seeded (quantum) process. This also allows photon pair production efficiencies to be calculated based on the results of classical nonlinear optical experiments. It is further calculated that, unless enerated photons are collected over a very narrow frequency range, their generation efficiency does not scale the same way with device length in a channel waveguide, or resonance quality factor in a microring resonator, as might be expected from the corresponding classical frequency conversion efficiency. Although calculations do not include self- or cross-phase modulation, nor two-photon absorption\nor free-carrier absorption, it is calculated that their neglect is justified in the low pair production probability limit. Linear (scattering) loss is also neglected, though partially addressed in the final chapter of this thesis.\n\nBiphoton wave functions are calculated explicitly, such that their shape and orientation, including approximate analytic expressions for their widths, can easily be determined. This further allows estimation of the suitability of their associated photon pairs for various quantum information processing applications. As an alternative to dispersion engineering a channel waveguide photon pair source, it is calculated that microring resonators can very naturally produce nearly spectrally uncorrelated photon pairs, which behave very much like idealized single-mode photons and are thus useful for applications involving the interference of photons from multiple sources.
In this thesis I study in detail the quantum dynamics of several nonlinear optical processes in microresonator systems. A Heisenberg-picture input-output formalism is developed from first principles that includes the effects of scattering losses and independent quality factors and coupling ratios for different resonances. The task of calculating the device output is then reduced to solving a set of driven, damped, ordinary differential equations for the resonator mode operators alone. This theoretical framework is used to study photon pair generation via spontaneous four-wave mixing in the weakly pumped regime, on which the effects of scattering losses are appraised. A more strongly driven regime is studied for continuous wave pumps, demonstrating when self- and cross-phase modulation and multi-photon pair generation become important, and their effects on the spectral and power scaling properties of the system are examined; A detuning strategy is presented that compensates for some of these effects. The results of the weak-pump regime are applied to study microresonator-based her- alded single photon sources. The impact of scattering losses is studied, revealing that typical systems suffer from low heralding efficiency due to these losses. A technique to improve heralding efficiency is presented through over-coupling the resonator-channel system, and a resultant trade-off between heralding rate and heralding efficiency is un- covered. Limitations to the spectral purity of the heralded single photon output for conventional microresonator systems are also analysed, and a more sophisticated cou- pling scheme presented to overcome the upper bound for spectral purity of 93% that exists in typical systems, permitting the generation of single photons with spectral pu- rity arbitrarily close to 100% without spectral filtering or sophisticated phase-matching techniques. The theory of quantum frequency conversion in microresonators using four-wave mix- ing is then developed in detail, and the spectral conversion probability and conversion efficiency studied. Efficiencies exceeding 90% using less than 100 mW of pump power are predicted to be achievable with current technology. A dressed mode picture is developed to better understand the conversion dynamics. Rabi-like spectral splitting and temporal oscillations of the intraresonator mean photon number are predicted, exhibiting a novel regime of strongly coupled photonic modes.