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arXiv:1504.01892 · Physical Review Letters

Correlated Exciton Transport in Rydberg-Dressed-Atom Spin Chains

H. Schempp, G. Günter, Sebastian Wüster, Matthias Weidemüller, S. Whitlock

Published Aug 26, 2015• 95 citations
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Abstract

We investigate the transport of excitations through a chain of atoms with nonlocal dissipation introduced through coupling to additional short-lived states. The system is described by an effective spin-1/2 model where the ratio of the exchange interaction strength to the reservoir coupling strength determines the type of transport, including coherent exciton motion, incoherent hopping, and a regime in which an emergent length scale leads to a preferred hopping distance far beyond nearest neighbors. For multiple impurities, the dissipation gives rise to strong nearest-neighbor correlations and entanglement. These results highlight the importance of nontrivial dissipation, correlations, and many-body effects in recent experiments on the dipole-mediated transport of Rydberg excitations.

DOI
10.1103/physrevlett.115.093002

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We investigate the transport of excitations through a chain of atoms with nonlocal dissipation introduced through coupling to additional short-lived states. The system is described by an effective spin-1/2 model where the ratio of the exchange interaction strength to the reservoir coupling strength determines the type of transport, including coherent exciton motion, incoherent hopping, and a regime in which an emergent length scale leads to a preferred hopping distance far beyond nearest neighbors. For multiple impurities, the dissipation gives rise to strong nearest-neighbor correlations and entanglement. These results highlight the importance of nontrivial dissipation, correlations, and many-body effects in recent experiments on the dipole-mediated transport of Rydberg excitations.
We present a scheme for engineering quantum transport dynamics of spin excitations in a chain of laser-dressed Rydberg atoms, mediated by synthetic spin exchange arising from diagonal van der Waals interaction. The dynamic tunability and long-range interaction feature of our scheme allows for the exploration of transport physics unattainable in conventional spin systems. As two concrete examples, we first demonstrate a topological exciton pumping protocol that facilitates quantized entanglement transfer, and second we discuss a highly nonlocal correlated transport phenomenon which persists even in the presence of dephasing. Unlike previous schemes, our proposal requires neither resonant dipole-dipole interaction nor off-diagonal van der Waals interaction. It can be readily implemented in existing experimental systems.
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We consider the interplay between excitonic and atomic motion in a regular, flexible chain of Rydberg atoms, extending our recent results on entanglement transport in Rydberg chains (Wüster et al 2010 Phys. Rev. Lett. 105 053004). In such a Rydberg chain, similar to molecular aggregates, an electronic excitation is delocalized due to long-range dipole–dipole interactions among the atoms. The transport of an exciton that is initially trapped by a chain dislocation is strongly coupled to nuclear dynamics, forming a localized pulse of combined excitation and displacement. This pulse transfers entanglement between dislocated atoms adiabatically along the chain. Details about the interaction and the preparation of the initial state are discussed. We also present evidence that the quantum dynamics of this complex many-body problem can be accurately described by selected quantum–classical methods, which greatly simplify investigations of excitation transport in flexible chains.
We investigate the dipole-mediated transport of Rydberg impurities through an ultracold gas of atoms prepared in an auxiliary Rydberg state. In one experiment, we continuously probe the system by coupling the auxiliary Rydberg state to a rapidly decaying state that realizes a dissipative medium. In situ imaging of the impurities reveals diffusive spreading controlled by the intensity of the probe laser. By preparing the same density of hopping partners, but then switching off the dressing fields, the spreading is effectively frozen. This is consistent with numerical simulations, which indicate the coherently evolving system enters a nonergodic extended phase. This opens the way to study transport and localization phenomena in systems with long-range hopping and controllable dissipation.
Randomness and disorder have strong impact on transport processes in quantum systems and give rise to phenomena such as Anderson localization [1-3], many-body localization [4] or glassy dynamics [5]. Their characteristics thereby depend on the strength and type of disorder. An important class are hopping models, where particles or excitations move through a system which has randomized couplings. This includes, e.g., spin glasses [5], coupled optical waveguides [6], or NV center arrays [7]. They are also key to understand excitation transport in molecular and biological systems, such as light harvesting complexes [8]. In many of those systems, the microscopic coupling mechanism is provided by the dipole-dipole interaction. Rydberg systems [9] are therefore a natural candidate to study random hopping models. Here, we experimentally study a three-dimensional many-body Rydberg system with random dipole-dipole couplings. We measure the spectrum of the many-body system and find good agreement with an effective spin model. We also find spectroscopic signatures of a localization-delocalization transition. Our results pave the way to study transport processes and localization phenomena in random hopping models in detail. The inclusion of strong correlations is experimentally straightforward and will allow to study the interplay between random hopping and localization in strongly interacting systems.
A key insight from recent studies is that noise, such as dephasing, can improve the efficiency of quantum transport by suppressing coherent single-particle interference effects. However, it is not yet clear whether dephasing can enhance transport in an interacting many-body system. Here, we address this question by analyzing the transport properties of a boundary driven spinless fermion chain with nearest-neighbor interactions subject to bulk dephasing. The many-body nonequilibrium stationary state is determined using large-scale matrix product simulations of the corresponding quantum master equation. We find dephasing enhanced transport only in the strongly interacting regime, where it is shown to induce incoherent transitions bridging the gap between bound dark states and bands of mobile eigenstates. The generic nature of the transport enhancement is illustrated by a simple toy model, which contains the basic elements required for its emergence. Surprisingly, the effect is significant even in the linear response regime of the full system, and it is predicted to exist for any large and finite chain. The response of the system to dephasing also establishes a signature of an underlying nonequilibrium phase transition between regimes of transport degradation and enhancement. The existence of this transition is shown not to depend on the integrability of the model considered. As a result, dephasing enhanced transport is expected to persist in more realistic nonequilibrium strongly correlated systems.