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arXiv:1809.07532 · Physical Review Letters

Diffusive to Nonergodic Dipolar Transport in a Dissipative Atomic Medium

S. Whitlock, H. Wildhagen, Hendrik Weimer, Matthias Weidemüller

Published Nov 22, 2019• 14 citations
arXivHTMLPDF

Abstract

We investigate the dipole-mediated transport of Rydberg impurities through an ultracold gas of atoms prepared in an auxiliary Rydberg state. In one experiment, we continuously probe the system by coupling the auxiliary Rydberg state to a rapidly decaying state that realizes a dissipative medium. In situ imaging of the impurities reveals diffusive spreading controlled by the intensity of the probe laser. By preparing the same density of hopping partners, but then switching off the dressing fields, the spreading is effectively frozen. This is consistent with numerical simulations, which indicate the coherently evolving system enters a nonergodic extended phase. This opens the way to study transport and localization phenomena in systems with long-range hopping and controllable dissipation.

DOI
10.1103/physrevlett.123.213606

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We investigate the dipole-mediated transport of Rydberg impurities through an ultracold gas of atoms prepared in an auxiliary Rydberg state. In one experiment, we continuously probe the system by coupling the auxiliary Rydberg state to a rapidly decaying state that realizes a dissipative medium. In situ imaging of the impurities reveals diffusive spreading controlled by the intensity of the probe laser. By preparing the same density of hopping partners, but then switching off the dressing fields, the spreading is effectively frozen. This is consistent with numerical simulations, which indicate the coherently evolving system enters a nonergodic extended phase. This opens the way to study transport and localization phenomena in systems with long-range hopping and controllable dissipation.
We investigate the transport of excitations through a chain of atoms with nonlocal dissipation introduced through coupling to additional short-lived states. The system is described by an effective spin-1/2 model where the ratio of the exchange interaction strength to the reservoir coupling strength determines the type of transport, including coherent exciton motion, incoherent hopping, and a regime in which an emergent length scale leads to a preferred hopping distance far beyond nearest neighbors. For multiple impurities, the dissipation gives rise to strong nearest-neighbor correlations and entanglement. These results highlight the importance of nontrivial dissipation, correlations, and many-body effects in recent experiments on the dipole-mediated transport of Rydberg excitations.
This thesis investigates different aspects of strongly interacting ultracold Rydberg gases coupled by light, including the excitation of correlated structures called Rydberg aggregates and dipolar energy transport. For this purpose an experimental apparatus has been constructed. We study coherent population trapping (CPT) and electromagnetically induced transparency (EIT) involving Rydberg states. To study the formation of Rydberg aggregates we use full counting statistics (FCS) which makes it possible to infer the size of Rydberg aggregates. Dephasing during the excitation is found to have a dramatic effect on the formation process, leading to sequential growth around an initial grain. Rydberg state EIT is used to realize a new direct optical imaging scheme for Rydberg atoms which combines highly sensitive detection with high spatial and temporal resolution. Applying this technique we observe dipole-mediated energy transport processes between Rydberg atoms. We study classical transport in the presence of strong measurement induced decoherence. The strong interactions are seen to mediate long-range hopping significantly beyond nearest neighbors. We present first indications for coherent transport in this system. These experiments shed light on the role of correlations in the excitation and evolution of strongly interacting quantum systems and e.g. could possibly be used to model energy transport in biological systems. \n
The long-range, anisotropic nature of the interaction among atoms in an ultracold dipolar gas leads to a rich array of possibilities for studying many-body physics. In this work, an ultracold gas of highly excited atoms is used to study energy transport due to the long-range dipole-dipole interaction. A technique is developed to measure both the internal energy states of the interacting Rydberg atoms and their positions in space. This technique is demonstrated by observing energy exchange between two spatially separated groups of Rydberg atoms excited to two different internal states. Simulations confirm the general features of the energy transport in this system and highlight subtleties associated with the homogeneity of the electric field used in this experiment.
This thesis describes studies on a Rydberg-dressed ultracold atom system as a versatile platform for non-equilibrium physics research, atom-light interactions analysis and atomic sensing applications. This work includes a description of the experimental system, an ultracold potassium atom setup where we can prepare a gas of atoms in an optical dipole trap and precisely control their ground state properties. To excite the atoms to strongly-interacting Rydberg states, we set up and characterize a high-power and widely tunable excitation laser system, for driving both single and two-photon Rydberg excitations. Together this establishes a unique system for studying the effects of driving, long-range interactions and dissipation (due to the relatively short lifetime of excited states) on many-body dynamics. Using this setup we study the phase structure of a driven-dissipative system out of equilibrium , where exploiting the atom loss rate as an observable,we discover different power-laws depending on the system parameters (i.e driving,dissipation and interaction). We study further in detail a regime which shows loss rates much larger than those for single particles, and discover that due to the Rydberg population decay the system evolves to a self-organized critical state.Our key observations can be well described by effectively classical models for the many-body dynamics, which we understand as a consequence of rapid dephasing of atomic coherences. To quantify the coherence of the atom-light interactions, we realize a Rydberg dressed interferometer. This technique combines the precision of atomic clock transitions with the exaggerated properties of Rydberg atoms such as their long-range interactions and extreme response to electric fields. Using the interferometer, we are able to characterize the Rydberg-dressed ensemble, including the effects of population decay and dephasing both of which affect the coherence time. This enables us to identify power fluctuations in the excitation laser as the dominant effects limiting the coherence in the system, which will be used in the experiment for future improvements of the coherence time. As an additional application, we demonstrate that the Rydberg dressed interferometer can be used to precisely measure static electric fields down to 17 mV/cm which is comparable to state-of-the-art electrometers. These results together highlight the versatility of the Rydberg platform and pave the way towards a better understanding of long-range interacting systems out-of-equilibrium. This work paves the way to new studies of non-equilibrium phenomena and applications of many-body quantum systems which make use of both quantum coherent and dissipative interactions.
We show that integrable and non-integrable dynamics can coexist in the same Rydberg-atom chain, depending on the initial state in which the system is prepared. In the setting we consider, Rydberg atoms mainly experience an effective dipolar interaction and, within the nearest-neighbor approximation, their dynamics can be mapped onto an effective integrable Fermi gas with ballistic transport. The inclusion of longer-range couplings, however, is essential for the theory to be predictive; those terms break the conservation laws associated with integrability, enabling, in particular, the emergence of genuine diffusive transport. We study the dynamics generated by a bipartition protocol and reveal a sharp qualitative change in behavior as the particle density is varied, suggesting the possibility of accessing weaker and stronger integrability breaking dynamics in the same Hamiltonian depending on the relevance of local interactions. We propose a theoretical mechanism that accounts for the differences. Our findings provide clear and concrete evidence that integrability breaking is not solely a property of the Hamiltonian and of the magnitude of the couplings that break integrability, but also of the state in which the system is prepared.
A three-level atomic medium can be made transparent to a resonant probe field in the presence of a strong control field acting on an adjacent atomic transition to a long-lived state, which can be represented by a highly excited Rydberg state. The long-range interactions between the Rydberg state atoms then translate into strong, non-local, dispersive or absorptive interactions between the probe photons, which can be used to achieve deterministic quantum logic gates and single photon sources. Here we show that long-range dipole–dipole exchange interaction with one or more spins—two-level systems represented by atoms in suitable Rydberg states—can play the role of control field for the optically dense medium of atoms. This induces transparency of the medium for a number of probe photons n p not exceeding the number of spins n s , while all the excess photons are resonantly absorbed upon propagation. In the most practical case of a single spin atom prepared in the Rydberg state, the medium is thus transparent only to a single input probe photon. For larger number of spins n s , all n p ≤ n s photon components of the probe field would experience transparency but with an n p -dependent group velocity.