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arXiv:1503.07044 · Physical Review A

Multistable particle-field dynamics in cavity-generated optical lattices

Dominik J. Winterauer, Wolfgang Niedenzu, Helmut Ritsch

Published May 18, 2015• 9 citations
arXivHTMLPDF

Abstract

Polarizable particles trapped in a resonator-sustained optical-lattice potential generate strong position-dependent backaction on the intracavity field. In the quantum regime, particles in different energy bands are connected to different intracavity light intensities and optical-lattice depths. This generates a highly nonlinear coupled particle-field dynamics. For a given pump strength and detuning, a factorizing mean-field approach predicts several self-consistent stationary solutions of strongly distinct photon numbers and motional states. Quantum Monte Carlo wave-function simulations of the master equation confirm these predictions and reveal complex multimodal photon-number and particle-momentum distributions. Using larger nanoparticles in such a setup thus constitutes a well-controllable playground to study nonlinear quantum dynamics and the buildup of macroscopic quantum superpositions at the quantum-classical boundary.

DOI
10.1103/physreva.91.053829

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•Sep 13, 2013•0 citations
Polarizable particles trapped in a resonator-sustained optical-lattice potential generate strong position-dependent backaction on the intracavity field. In the quantum regime, particles in different energy bands are connected to different intracavity light intensities and optical-lattice depths. This generates a highly nonlinear coupled particle-field dynamics. For a given pump strength and detuning, a factorizing mean-field approach predicts several self-consistent stationary solutions of strongly distinct photon numbers and motional states. Quantum Monte Carlo wave-function simulations of the master equation confirm these predictions and reveal complex multimodal photon-number and particle-momentum distributions. Using larger nanoparticles in such a setup thus constitutes a well-controllable playground to study nonlinear quantum dynamics and the buildup of macroscopic quantum superpositions at the quantum-classical boundary.
The light force on particles trapped in the field of a high-QQQ cavity mode depends on the quantum state of field and particle. Different photon numbers generate different optical potentials and different motional states induce different field evolution. Even for negligible internal particle excitation, which yields linear polarizability, the quantum character of particle motion generates nonlinear field dynamics. We derive a corresponding effective field Hamiltonian containing all the powers of the photon number operator, which predicts nonlinear phase shifts and squeezing even at the few-photon level. Simulations of the full particle-field dynamics confirm this and show significant particle-field entanglement.
The quantum dynamics of particles optically trapped in a symmetrically pumped high-QQQ ring cavity exhibits much richer physics than for a standing-wave resonator. In addition to modifying the lattice depth, light scattering by the particles shifts and reshapes the trapping potential. We calculate the corresponding changes in tunneling amplitudes and damping by an effective bipotential (two-level) model for the particle motion. As a crude truncation of the Bose-Hubbard model, expansion to the lowest band decouples particle and field dynamics. Only including excitations to higher bands can capture this essential additional physics and correctly describe decoherence, damping, and long-range correlations of the particle dynamics. The validity limits of the analytic models are confirmed by quantum Monte Carlo wave-function simulations, which exhibit correlated particle-field quantum jumps as unambiguous quantum signature of the system dynamics.
This is a review of state-of-the-art theory and experiment of the motion of cold and ultracold atoms coupled to the radiation field within a high-finesse optical resonator in the dispersive regime of the atom-field interaction with small internal excitation. The optical dipole force on the atoms together with the backaction of atomic motion onto the light field gives rise to a complex nonlinear coupled dynamics. As the resonator constitutes an open driven and damped system, the dynamics is nonconservative and in general enables cooling and confining the motion of polarizable particles. In addition the emitted cavity field allows for real-time monitoring of the particle's position with minimal perturbation up to subwavelength accuracy. For many-body systems, the resonator field mediates controllable long-range atom-atom interactions, which set the stage for collective phenomena. Besides the correlated motion of distant particles, one finds critical behavior and nonequilibrium phase transitions between states of different atomic order in conjunction with superradiant light scattering. Quantum-degenerate gases inside optical resonators can be used to emulate optomechanics as well as novel quantum phases such as supersolids and spin glasses. Nonequilibrium quantum phase transitions as predicted by, e.g., the Dicke Hamiltonian can be controlled and explored in real time via monitoring the cavity field. In combination with optical lattices, the cavity field can be utilized for nondestructive probing Hubbard physics and tailoring long-range interactions for ultracold quantum systems.
Quantum gases of atoms and molecules in optical cavities offer a formidable laboratory for studying the out-of-equilibrium dynamics of open quantum systems with long-range interactions. Long-range interactions are here mediated by multiple scattering of cavity photons and can induce the formation of quantum structures in space and time. Control of these dynamics requires a detailed understanding of all relevant mechanisms at play. Due to the strong correlations induced by light, however, perturbative theoretical models, which reduce the number of degrees of freedom, do not correctly capture the regime where the interplay of photon-mediated long-range forces and quantum fluctuations of light and matter become significant, such as across the transition to self-organization. In this work, we present the derivation of an effective Lindblad master equation for the dynamics of the sole motional variables of polarizable particles, such as atoms or molecules, that dispersively couple to cavity fields. The master equation is valid even for relatively large intracavity photon numbers and is apt to study both the steady-state regime and the out-of-equilibrium dynamics where quantum fluctuations of the field seed the onset of macroscopic coherences. We validate the theoretical description by showing that it captures the dynamics across a wide temperature interval, from Doppler cooling down to the ultracold regime, and from weak to strong cavity-mediated interactions. Our theory provides a powerful framework for the description of cavity-induced dynamics of quantum matter. In doing so, it permits to connect models of statistical mechanics with cavity-QED experimental platforms, thus enabling quantum simulation of long-range-interacting matter.
A cold gas of polarizable particles moving in the optical potential of a standing wave high finesse optical resonator acts as a dynamic refractive index. For a sufficiently strong cavity pump the optical forces generated by the intra cavity field perturb the particles phase space distribution, which shifts the optical resonance frequency and induces a nonlinear optical response. By help of the corresponding Vlasov equation we predict that beyond the known phenomenon of optical bi-stability one finds regions in parameter space, where no stable stationary solution exists. The atom field dynamics then exhibits oscillatory solutions converging to stable limit cycles of the system. The linearized analytical predictions agree well with corresponding numerical solutions of the full time dependent equations and first experimental observation in both cases.
Ultracold atoms in an optical lattice Bloch oscillate when subject to a constant force. In the first work presented in this thesis we have theoretically studied the scenario where the optical lattice potential is provided by the electric field inside an optical cavity. The coherent atom-light interaction in a cavity gives rise to a backaction effect on the light field which can modify the intracavity field amplitude and phase. In our first treatment of this problem we model the cavity light field and atoms by classical fields and solve the coupled atom-light equations of motion. As a result, we find that the amplitude and phase of the transmitted light field is modulated at the Bloch frequency. Remarkably, the Bloch frequency itself is not modified by the backaction. Thus the transmitted light field can be used to observe the oscillations continuously, allowing high-precision measurement with small clouds of atoms. In the second problem presented in this thesis, we explore the band structure of the steady state solutions of the atom-cavity system. A crucial first step towards determining the band structure is the identification of an energy functional that describes the coupled atom-light system. Although, we do not include direct atom-atom interactions in our models, the coupling of the atoms to the single mode light field of the cavity introduces an effective mutual interaction which is correctly taken into account by the energy functional we introduce. Corresponding to each point in the band there exists a steady state light field associated with an average cavity photon number. The dispersive nonlinear atom-light interaction can lead to bistable solutions for this intracavity photon number. For parameters where the atom-cavity system exhibits bistability, the atomic band structure develops loop structures akin to the ones predicted for Bose-Einstein condensates in ordinary (non-cavity) optical lattices. However, in our case the nonlinearity derives from the cavity backaction rather than from direct interatomic interactions. We find both bi- and tri-stable regimes associated with the lowest band, and show that the multistability we observe can be analysed in terms of swallowtail catastrophes. Dynamic and energetic stability of the meanfield solutions is also studied, and we show that the bistable solutions have, as expected, one unstable and two stable branches. The presence of loops in the band structure can lead to a breakdown in adiabaticity during Bloch oscillations as the entire band is sampled during the dynamics. We therefore use the insight gleaned from this work in choosing parameters for the Bloch oscillation measurement proposal presented in the rest of the thesis. In the third work presented in the thesis, we go beyond the mean field description and consider effects of the quantised nature of the light and atomic fields. The cavity light field is always in contact with external electromagnetic fields through the partially transmissive mirrors. This coupling to the external modes enters as quantum noise in the dynamics of the intracavity field and can also be viewed as a manifestation of quantum measurement backaction corresponding to the continuous observation of the transmitted light field. We solve the Heisenberg-Langevin equations for linearized fluctuations about the atomic and optical meanfields and examine how this influences the signal-to-noise ratio of a measurement of external forces using this system. In particular, we investigate the effects of changing the number of atoms, the intracavity lattice depth, and the atom-light coupling strength, and show how resonances between the Bloch oscillation dynamics and the quasiparticle spectrum have a strong influence on the signal-to-noise ratio as well as heating effects. One of the hurdles we overcome along the way is the proper treatment of fluctuations about time-dependent meanfields in the context of cold atom cavity-QED.