Quantum gases of atoms and molecules in optical cavities offer a formidable laboratory for studying the out-of-equilibrium dynamics of open quantum systems with long-range interactions. Long-range interactions are here mediated by multiple scattering of cavity photons and can induce the formation of quantum structures in space and time. Control of these dynamics requires a detailed understanding of all relevant mechanisms at play. Due to the strong correlations induced by light, however, perturbative theoretical models, which reduce the number of degrees of freedom, do not correctly capture the regime where the interplay of photon-mediated long-range forces and quantum fluctuations of light and matter become significant, such as across the transition to self-organization. In this work, we present the derivation of an effective Lindblad master equation for the dynamics of the sole motional variables of polarizable particles, such as atoms or molecules, that dispersively couple to cavity fields. The master equation is valid even for relatively large intracavity photon numbers and is apt to study both the steady-state regime and the out-of-equilibrium dynamics where quantum fluctuations of the field seed the onset of macroscopic coherences. We validate the theoretical description by showing that it captures the dynamics across a wide temperature interval, from Doppler cooling down to the ultracold regime, and from weak to strong cavity-mediated interactions. Our theory provides a powerful framework for the description of cavity-induced dynamics of quantum matter. In doing so, it permits to connect models of statistical mechanics with cavity-QED experimental platforms, thus enabling quantum simulation of long-range-interacting matter.
Quantum gases of atoms and molecules in optical cavities offer a formidable laboratory for studying the out-of-equilibrium dynamics of open quantum systems with long-range interactions. Long-range interactions are here mediated by multiple scattering of cavity photons and can induce the formation of quantum structures in space and time. Control of these dynamics requires a detailed understanding of all relevant mechanisms at play. Due to the strong correlations induced by light, however, perturbative theoretical models, which reduce the number of degrees of freedom, do not correctly capture the regime where the interplay of photon-mediated long-range forces and quantum fluctuations of light and matter become significant, such as across the transition to self-organization. In this work, we present the derivation of an effective Lindblad master equation for the dynamics of the sole motional variables of polarizable particles, such as atoms or molecules, that dispersively couple to cavity fields. The master equation is valid even for relatively large intracavity photon numbers and is apt to study both the steady-state regime and the out-of-equilibrium dynamics where quantum fluctuations of the field seed the onset of macroscopic coherences. We validate the theoretical description by showing that it captures the dynamics across a wide temperature interval, from Doppler cooling down to the ultracold regime, and from weak to strong cavity-mediated interactions. Our theory provides a powerful framework for the description of cavity-induced dynamics of quantum matter. In doing so, it permits to connect models of statistical mechanics with cavity-QED experimental platforms, thus enabling quantum simulation of long-range-interacting matter.
Ultracold atomic gases loaded into optical cavities constitute one of the most versatile platforms for the study of out-of-equilibrium dynamics and quantum simulation of many- body systems. In this thesis, we explore these two possibilities, motivated by current state-of-the-art atom-cavity experiments, uncovering novel phenomena and opening up new theoretical and experimental avenues into the intriguing world of quantum many- body physics. First, we study a gas of ultracold atoms coupled to three optical resonators. We show that the inherent Z2 symmetries, associated with each atom-cavity coupling, can be combined into a global SO(3) rotational symmetry which can be spontaneously broken. We determine the phase diagram of the system, which shows the emergence and breaking of the continuous symmetries and displays first- and second-order phase transitions. We argue that by coupling the atoms equally to n different modes, it will in general be possible to generate a global SO(n) symmetry. Second, we investigate the dynamics of a spinor BEC inside an optical cavity. We focus on a two-component Dicke model with complex light-matter couplings, accounting for photon losses. We compute the steady-state phase diagram and find dynamical in- stabilities in the form of limit cycles, heralded by the presence of exceptional points and level attraction. We show that the instabilities are induced by dissipative processes that generate nonreciprocal couplings between the two collective spins. Lastly, we explore the dynamics of a BEC inside an optical cavity in the presence of an optical lattice. We derive an effective master equation by adiabatically eliminating the cavity field. In the bad-cavity regime, we find an infinite-temperature steady state, but with relaxation dynamics that can be highly nontrivial. For small hopping, the interplay between dissipation and strong interactions leads to an algebraic relaxation of the system, whereas for large hopping, the approach to the steady state is exponential. In the good- cavity regime, we show that the system allows for optical pumping between momentum modes, enabling cavity cooling.
We investigate the out-of-equilibrium dynamics of ultracold atoms trapped in an optical lattice and loaded into an optical resonator that is driven transversely. We derive an effective quantum master equation for weak atom-light coupling that can be brought into Lindblad form in both the bad- and good-cavity limits. In the so-called bad-cavity regime, we find that the steady state is always that of infinite temperature, but that the relaxation dynamics can be highly nontrivial. For small hopping, the interplay between dissipation and strong interactions generally leads to anomalous diffusion in the space of atomic configurations. However, for a fine-tuned ratio of cavity-mediated and on-site interactions, we discover a limit featuring normal diffusion. In contrast, for large hopping and vanishing on-site interactions, the system can be described by a linear rate equation leading to an exponential approach of the infinite-temperature steady state. Finally, in the good-cavity regime, we show that for vanishing on-site interactions, the system allows for optical pumping between momentum mode pairs enabling cavity cooling.
This is a review of state-of-the-art theory and experiment of the motion of cold and ultracold atoms coupled to the radiation field within a high-finesse optical resonator in the dispersive regime of the atom-field interaction with small internal excitation. The optical dipole force on the atoms together with the backaction of atomic motion onto the light field gives rise to a complex nonlinear coupled dynamics. As the resonator constitutes an open driven and damped system, the dynamics is nonconservative and in general enables cooling and confining the motion of polarizable particles. In addition the emitted cavity field allows for real-time monitoring of the particle's position with minimal perturbation up to subwavelength accuracy. For many-body systems, the resonator field mediates controllable long-range atom-atom interactions, which set the stage for collective phenomena. Besides the correlated motion of distant particles, one finds critical behavior and nonequilibrium phase transitions between states of different atomic order in conjunction with superradiant light scattering. Quantum-degenerate gases inside optical resonators can be used to emulate optomechanics as well as novel quantum phases such as supersolids and spin glasses. Nonequilibrium quantum phase transitions as predicted by, e.g., the Dicke Hamiltonian can be controlled and explored in real time via monitoring the cavity field. In combination with optical lattices, the cavity field can be utilized for nondestructive probing Hubbard physics and tailoring long-range interactions for ultracold quantum systems.
Experimental platforms based on ultracold atomic gases have significantly advanced the quantum simulation of complex systems, yet the exploration of phenomena driven by long-range interactions remains a formidable challenge. Currently available methods utilizing dipolar quantum gases or multimode cavities allow us to implement long-range interactions with a 1 / r 3 character or with a spatial profile fixed by the mode structure of the vacuum electromagnetic field surrounding the atoms, respectively. Here, we propose an experimental scheme employing laser-painted cavity-mediated interactions, which enables the realization of atom-atom interactions that are fully tunable in range, shape, and sign. Our approach combines the versatility of cavity quantum electrodynamics with the precision of laser manipulation, thus providing a highly flexible platform for simulating and understanding long-range interactions in quantum many-body systems. Our analytical predictions are supported by numerical simulations describing the full dynamics of the atoms, the laser, and the cavity. These reveal the self-organization of domains in the density of the atomic cloud, confirming the finite-range nature of the induced interactions. We demonstrate that there is a wide and experimentally accessible parameter regime in which our protocol works robustly, with negligible heating of the quantum gas. The methodology not only paves the way for exploring new territories in quantum simulation but also enhances the understanding of fundamental physics, potentially leading to the discovery of novel quantum states and phases. Published by the American Physical Society 2024
Recent advances in theoretical physics have increasingly focused on the dynamics of quantum systems with many interacting degrees of freedom, while ultracold atom platforms now enable the realization of diverse theoretical models with precise control over system parameters and advanced monitoring techniques. A prominent example is cavity quantum electrodynamics (CQED), where large atomic or molecular ensembles are coupled to high-finesse optical cavities, enabling strong interaction with confined electromagnetic modes and leading to phenomena such as the superradiant phase transition, in which atoms and photons form a coherent state. Most theoretical studies of CQED have concentrated on regimes of spatially uniform atom–cavity coupling, where collective behavior allows a description in terms of the classical dynamics of a few macroscopic variables. However, experimental capabilities now permit exploration beyond this limit, though theoretical progress is hindered by the exponential computational complexity of simulating large quantum systems, particularly when environmental coupling is included. This thesis addresses such challenges by developing efficient approaches, within the Keldysh formalism of non-equilibrium quantum field theory, to study systems with strongly disordered interactions coupled to external reservoirs. Two representative models are considered: a disordered spin–boson model describing light–matter interactions with quenched disorder, relevant to recent CQED experiments in confocal cavities, and a fermion–phonon system governed by the Yukawa–Sachdev–Ye–Kitaev (Yukawa-SYK) model. Both systems are quantum critical, exhibiting a continuum of low-energy modes above their stationary states, yet disorder produces qualitatively distinct dynamical behaviors: in the spin–boson system it induces slow, glassy relaxation, whereas in the Yukawa-SYK model it leads to rapid thermalization. These contrasting outcomes reveal the non-trivial role of disorder in quantum many-body systems and motivate further investigation into its effects on non-equilibrium quantum dynamics.
We present the Born-Markov approximated Redfield quantum master equation (RQME) description for an open system of noninteracting particles (bosons or fermions) on an arbitrary lattice of N sites in any dimension and weakly connected to multiple reservoirs at different temperatures and chemical potentials. The RQME can be reduced to the Lindblad equation, of various forms, by making further approximations. By studying the N=2 case, we show that RQME gives results which agree with exact analytical results for steady-state properties and with exact numerics for time-dependent properties over a wide range of parameters. In comparison, the Lindblad equations have a limited domain of validity in nonequilibrium. We conclude that it is indeed justified to use microscopically derived full RQME to go beyond the limitations of Lindblad equations in out-of-equilibrium systems. We also derive closed-form analytical results for out-of-equilibrium time dynamics of two-point correlation functions. These results explicitly show the approach to steady state and thermalization. These results are experimentally relevant for cold atoms, cavity QED, and far-from-equilibrium quantum dot experiments.