This is a review of state-of-the-art theory and experiment of the motion of cold and ultracold atoms coupled to the radiation field within a high-finesse optical resonator in the dispersive regime of the atom-field interaction with small internal excitation. The optical dipole force on the atoms together with the backaction of atomic motion onto the light field gives rise to a complex nonlinear coupled dynamics. As the resonator constitutes an open driven and damped system, the dynamics is nonconservative and in general enables cooling and confining the motion of polarizable particles. In addition the emitted cavity field allows for real-time monitoring of the particle's position with minimal perturbation up to subwavelength accuracy. For many-body systems, the resonator field mediates controllable long-range atom-atom interactions, which set the stage for collective phenomena. Besides the correlated motion of distant particles, one finds critical behavior and nonequilibrium phase transitions between states of different atomic order in conjunction with superradiant light scattering. Quantum-degenerate gases inside optical resonators can be used to emulate optomechanics as well as novel quantum phases such as supersolids and spin glasses. Nonequilibrium quantum phase transitions as predicted by, e.g., the Dicke Hamiltonian can be controlled and explored in real time via monitoring the cavity field. In combination with optical lattices, the cavity field can be utilized for nondestructive probing Hubbard physics and tailoring long-range interactions for ultracold quantum systems.
This is a review of state-of-the-art theory and experiment of the motion of cold and ultracold atoms coupled to the radiation field within a high-finesse optical resonator in the dispersive regime of the atom-field interaction with small internal excitation. The optical dipole force on the atoms together with the backaction of atomic motion onto the light field gives rise to a complex nonlinear coupled dynamics. As the resonator constitutes an open driven and damped system, the dynamics is nonconservative and in general enables cooling and confining the motion of polarizable particles. In addition the emitted cavity field allows for real-time monitoring of the particle's position with minimal perturbation up to subwavelength accuracy. For many-body systems, the resonator field mediates controllable long-range atom-atom interactions, which set the stage for collective phenomena. Besides the correlated motion of distant particles, one finds critical behavior and nonequilibrium phase transitions between states of different atomic order in conjunction with superradiant light scattering. Quantum-degenerate gases inside optical resonators can be used to emulate optomechanics as well as novel quantum phases such as supersolids and spin glasses. Nonequilibrium quantum phase transitions as predicted by, e.g., the Dicke Hamiltonian can be controlled and explored in real time via monitoring the cavity field. In combination with optical lattices, the cavity field can be utilized for nondestructive probing Hubbard physics and tailoring long-range interactions for ultracold quantum systems.
A common goal of recent research is the elucidation and control over quantum mechanical behavior in ever-larger physical systems. In this thesis I present an alternative target for investigating the quantum motion of macroscopic bodies: the collective motion of an ultracold atomic gas trapped within a high-finesse Fabry-Perot optical cavity in the single-atom strong-coupling regime of cavity quantum electrodynamics (CQED). When ultracold atoms are trapped in the Lamb-Dicke regime, the cavity-mode structure selects a single collective degree of freedom that is at once actuated by the optical forces from cavity probe light and measured by the cavity’s optical properties. Dispersive optical bistability arising from collective motion of the atomic medium was observed. Measurement of the collective motion was subject to quantum measurement backaction by the quantum force fluctuations of the cavity optical field. The strength and spectrum of these backaction force fluctuations was measured by quantifying the cavity-light-induced heating rate of the intracavity atomic ensemble, finding quantitative agreement with the expected heating rate from quantum optical fluctuations. Dynamical phenomena in the optomechanical system were explored experimentally and theoretically. Quantum limited measurements are discussed and were
Ultracold atomic gases loaded into optical cavities constitute one of the most versatile platforms for the study of out-of-equilibrium dynamics and quantum simulation of many- body systems. In this thesis, we explore these two possibilities, motivated by current state-of-the-art atom-cavity experiments, uncovering novel phenomena and opening up new theoretical and experimental avenues into the intriguing world of quantum many- body physics. First, we study a gas of ultracold atoms coupled to three optical resonators. We show that the inherent Z2 symmetries, associated with each atom-cavity coupling, can be combined into a global SO(3) rotational symmetry which can be spontaneously broken. We determine the phase diagram of the system, which shows the emergence and breaking of the continuous symmetries and displays first- and second-order phase transitions. We argue that by coupling the atoms equally to n different modes, it will in general be possible to generate a global SO(n) symmetry. Second, we investigate the dynamics of a spinor BEC inside an optical cavity. We focus on a two-component Dicke model with complex light-matter couplings, accounting for photon losses. We compute the steady-state phase diagram and find dynamical in- stabilities in the form of limit cycles, heralded by the presence of exceptional points and level attraction. We show that the instabilities are induced by dissipative processes that generate nonreciprocal couplings between the two collective spins. Lastly, we explore the dynamics of a BEC inside an optical cavity in the presence of an optical lattice. We derive an effective master equation by adiabatically eliminating the cavity field. In the bad-cavity regime, we find an infinite-temperature steady state, but with relaxation dynamics that can be highly nontrivial. For small hopping, the interplay between dissipation and strong interactions leads to an algebraic relaxation of the system, whereas for large hopping, the approach to the steady state is exponential. In the good- cavity regime, we show that the system allows for optical pumping between momentum modes, enabling cavity cooling.
This thesis summarizes the research work we did in the past years, which focuses on the theoretical study of quantum effects of ordered atomic structures interacting with the quantum electric field of an optical resonator. Within this work we investigated the quantum properties of the light at the cavity output, emitted by this kind of system, and the quantum state of the atoms confined by the light fields of the cavity mode. Following one possible partition, we have organized the thesis in two parts. The first part of the thesis is devoted to the quantum properties of the light at the output of optical cavities, in which atoms are confined. After a brief introduction on the basics of atom-photon interactions, we show theoretically, that two atomic dipoles in a resonator can behave as a quantum non-linear medium, whose response can be controlled through the interactomic distance of the atoms inside the resonator. We identify the parameter regime, for which the system operates as a parametric amplifier, based on the atoms' collective dipole cascade emission. Moreover we also determine the corresponding field squeezing spectrum at the cavity output. These dynamics could be observed as a result of self-organization processes of laser-cooled atoms in resonators. The second part of the thesis studies the quantum ground state of an ultracold atomic gas trapped inside an optical resonator by the mechanical effects of atom-photon interactions. Due to the strong coupling regime, the ultracold atomic gas feels a quantum potential, where the fluctuations at the single photon level may be relevant in determining the trapping conditions. This potential depends on the atomic distribution, which at the same time determines the intracavity field amplitude. Here, after a brief introduction on ultracold atoms in optical lattices, we study the low temperature physics of an ultracold atomic gas in the quantum potential formed inside a pumped cavity, by mapping the dynamics to an effective Bose-Hubbard model. We predict the existence of non-compressible states of the atomic gas, and determine a phase diagram as a function of the cavity parameters. Novel effects are encountered, such as the existence of overlapping stability regions corresponding to competing insulator-like states when the laser pumps the cavity, to provide one example out of many. At the end of the thesis a concluding chapter presents some general outlooks to this thesis work.
Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. Several experiments have demonstrated that such environments can give rise to new competing quantum phases. \nBut this long-standing ambition to push for models with tailorable interaction potentials can bring with it also considerable challenges in their theoretical description, since sponta- neous symmetry breaking transitions in many body lattice systems coupled to dynamical light-fields with single-photon character occur in the presence of drive and dissipation for the photonic force carriers. This clearly calls for model systems where the above men- tioned interplay of interactions, drive, dissipation and cooperative many-body behaviour can be theoretically studied to provide simple, experimentally verifiable predictions. \nThe Dicke model is, through its simplicity (an exactly solved ferromagnet with infinite range atom-atom interactions mediated by a single cavity mode), an exceptionally well- suited candidate. As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.
When placing an ultracold atomic gas inside a cavity, the light-matter coupling is enhanced and nonlinear atomic dynamics is generated, offering a promising platform for quantum simulation of models with short- and long-range interactions. Recently, superradiant self-organized phases for ultracold atomic gases inside a cavity, pumped by a blue detuned optical lattice, have been observed. Here, we explore the formation of quantum many-body phases of bosonic atoms inside an optical cavity, subject to transverse blue detuned pumping. We investigate the strongly interacting regime, which can be reached by tuning the s-wave scattering length using external fields. We analyze the interplay between superradiant self-organization with superfluid and Mott insulator phases, without the need of including higher lying bands, as the Wannier functions are dynamically linked to the cavity light via backaction. We observe different kinds of structural phase transitions driven by the light inside the cavity and the interplay with atomic collisions. We observe the mode softening at the critical points in the quantum phase transitions which can be measured in future experiments. We obtain our results within a full self-consistent theoretical framework, the light-matter density matrix renormalization group (DMRG), which employs the computation of light dependent Wannier functions for the full quantum optical lattice in combination with DMRG for the atomic dynamics. The methods introduced here can be used to analyze the effects of strong quantum correlations in strongly interacting light-matter systems.
This dissertation contains a study of ultracold atoms in optical cavities. We particularly focus on two aspects of the coupled atom-cavity systems. In the first aspect, we implement the quantum nature of the light field to probe the quantum state of the atoms. This is interesting due to the nondestructive nature of the characterization of many-body atomic states. In the second aspect we study the cavity optomechanics that investigates the coupling of mechanical and optical degrees of freedom via radiation pressure. The optomechanical cavity provides an interesting nonlinear system to study the coupling between atoms and the intracavity field.In the context of cavity quantum electrodynamics we study the reflection of two counter-propagating modes of the light field in a high-Q ring cavity by ultracold atoms either in the Mott insulator state or in the superfluid state of an optical lattice. We find that the dynamics of the reflected light strongly depends on both the lattice spacing and the state of the matter-wave field. By using the Monte Carlo wave-function method to account for the cavity damping we also determine the two-time correlation function and the time-dependent physical spectrum of theretroreflected field. We find that the light field and the atoms become entangled if the latter are in a superfluid state. We also analyze quantitatively the entanglement between the atoms and the light.In cavity optomechanics the mechanical effect can either comes from a vibrating macroscopic oscillator or a collective density excitation of a Bose-Einstein condensate. First we use a Fabry-Perot-type cavity to study the opto-mechanically-induced bistable quantum phase transitions between superfluid and a Mott insulator states of an ultracold bosonic gases trapped inside the cavity. Secondly, we study the symmetricand antisymmetric collective density side modes of the BEC which results from the optomechanical effects of the light fields in a ring cavity.