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arXiv:1412.6167 · Nuclear Instruments and Methods in Physics Research Section A Accelerators Spectrometers Detectors and Associated Equipment

Diffusive transfer of polarized 3He gas through depolarizing magnetic gradients

J. Maxwell, Charles Epstein, R. Milner

Published Jan 9, 2015• 7 citations
arXivHTMLPDF
DOI
10.1016/j.nima.2015.01.004

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We carried out experiments on a spin polarized 3He- 4He mixture with 3He concentration x 3 = 6.26 × 10−4, and on pure 3He liquid. Spin polarization affects the transport properties of these Fermi systems. The effect on momentum transport was studied by using a vibrating-wire viscometer to measure viscosity of the 3He-4He mixture over the temperature range 6.09 mK–100 mK in 7.96 T and 1.00 T magnetic fields. A large viscosity increase was observed upon application of the 7.96 T magnetic field for temperature T < TF(TF = 19.5 mK is the Fermi temperature). The observed viscosity is in very good agreement with theoretical calculations for a dilute Fermi gas by Jeon and Mullin [1988, 1989] and Mullin and Jeon [1992]. The polarization effect on spin transport was investigated by measuring the transverse diffusion coefficient D ⊥ in pure 3He liquid at saturated vapor pressure and at 15.85 bar over the temperature range 4.5 mK–159 mK in a 7.96 T magnetic field. We used a pulsed NMR spin echo technique in a field gradient of 16.0 G/cm to do the measurements and fits to the Leggett equations [1970] to obtain D⊥. For T < 20 mK, we found D⊥ is less than measured in earlier experiments at lower magnetic fields. D⊥ does not increase with decreasing temperature as 1/T2, but appears to approach a constant as T → 0 while it is expected that the longitudinal spin diffusion coefficient D∥ ∝ 1/ T2. This is called spin diffusion anisotropy and it was observed for the first time in our 3He liquid experiments. The anisotropy temperature we determined for 3He liquid was Ta = 16.4 ± 2.2 mK at saturated vapor pressure and in a 7.96 T magnetic field. The transverse spin diffusion in 3 He results agree qualitatively with theories proposed by Meyerovich and Musaeflan [1992, 1994]. They also agree qualitatively with theories proposed by Golosov and Ruckenstein [1995, 1998] by extrapolation of the dilute theory to a strongly interacting system.

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The general results obtained in the preceding article are applied to the study of transport phenomena in a spin polarized gas at low temperatures, with particular emphasis on the particle indistinguishability effects in collisions. The effects of the nuclear orientation M are treated exactly (no M expansion). First, a simple theory of spin diffusion is presented and the response of the gas to a spin orientation gradient is calculated. The spin coherences and their evolution due to the « identical-spin rotation effect » are taken into account; it is found that they can play an important role, especially in the low temperature limit. The hydrodynamic equations of evolution of M are non-linear and anisotropic. Particle indistinguishability effects give an oscillatory character to the evolution of the transverse components of M (spin oscillations). Then, a more elaborate variational method is used to study the coupling between spin diffusion and heat conduction. This effect is, again, a sheer consequence of quantum interference phenomena introduced by particle indistinguishability. Finally, isotopic mixtures of 3He and 4He are considered In addition to coupling between isotopic diffusion and heat conduction, which exists for classical systems, quantum collision effects introduce a coupling between these two modes and spin diffusion.

Journal de physique•Jan 1, 1982•129 citations
We carried out experiments on a spin polarized 3He- 4He mixture with 3He concentration x 3 = 6.26 × 10−4, and on pure 3He liquid. Spin polarization affects the transport properties of these Fermi systems. The effect on momentum transport was studied by using a vibrating-wire viscometer to measure viscosity of the 3He-4He mixture over the temperature range 6.09 mK–100 mK in 7.96 T and 1.00 T magnetic fields. A large viscosity increase was observed upon application of the 7.96 T magnetic field for temperature T < TF(TF = 19.5 mK is the Fermi temperature). The observed viscosity is in very good agreement with theoretical calculations for a dilute Fermi gas by Jeon and Mullin [1988, 1989] and Mullin and Jeon [1992]. The polarization effect on spin transport was investigated by measuring the transverse diffusion coefficient D ⊥ in pure 3He liquid at saturated vapor pressure and at 15.85 bar over the temperature range 4.5 mK–159 mK in a 7.96 T magnetic field. We used a pulsed NMR spin echo technique in a field gradient of 16.0 G/cm to do the measurements and fits to the Leggett equations [1970] to obtain D⊥. For T < 20 mK, we found D⊥ is less than measured in earlier experiments at lower magnetic fields. D⊥ does not increase with decreasing temperature as 1/T2, but appears to approach a constant as T → 0 while it is expected that the longitudinal spin diffusion coefficient D∥ ∝ 1/ T2. This is called spin diffusion anisotropy and it was observed for the first time in our 3He liquid experiments. The anisotropy temperature we determined for 3He liquid was Ta = 16.4 ± 2.2 mK at saturated vapor pressure and in a 7.96 T magnetic field. The transverse spin diffusion in 3 He results agree qualitatively with theories proposed by Meyerovich and Musaeflan [1992, 1994]. They also agree qualitatively with theories proposed by Golosov and Ruckenstein [1995, 1998] by extrapolation of the dilute theory to a strongly interacting system.
This article gives a theoretical study of the effects of weak magnetic field gradients on the spin relaxation of a dilute atomic gas. The theory is valid for low or moderate values of the field (the relevant correlation time of the gas is then the diffusion time across the container) as well as for high fields (the intercollision time then plays the most important role). Quantum effects due to particle indistinguishability are included. No consequences of the divergence of the atomic mean free path in a polarized gas at zero temperature are found, in contrast to the situation for viscosity and heat conductivity. On the other hand, substantial effects due to « identical spin rotation effects » are predicted.
The general results obtained in the preceding article are applied to the study of transport phenomena in a spin polarized gas at low temperatures, with particular emphasis on the particle indistinguishability effects in collisions. The effects of the nuclear orientation M are treated exactly (no M expansion). First, a simple theory of spin diffusion is presented and the response of the gas to a spin orientation gradient is calculated. The spin coherences and their evolution due to the « identical-spin rotation effect » are taken into account; it is found that they can play an important role, especially in the low temperature limit. The hydrodynamic equations of evolution of M are non-linear and anisotropic. Particle indistinguishability effects give an oscillatory character to the evolution of the transverse components of M (spin oscillations). Then, a more elaborate variational method is used to study the coupling between spin diffusion and heat conduction. This effect is, again, a sheer consequence of quantum interference phenomena introduced by particle indistinguishability. Finally, isotopic mixtures of 3He and 4He are considered In addition to coupling between isotopic diffusion and heat conduction, which exists for classical systems, quantum collision effects introduce a coupling between these two modes and spin diffusion.