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arXiv:1410.1650 · Physical Review A

Quantum dynamics of a two-level emitter with a modulated transition frequency

Mihai Macovei, Christoph H. Keitel

Published Oct 20, 2014• 16 citations
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Abstract

The resonant quantum dynamics of an excited two-level emitter is investigated via classical modulation of its transition frequency while simultaneously the radiator interacts with a broadband electromagnetic field reservoir. The frequency of modulation is selected to be of the order of the bare-state spontaneous decay rate. In this way, one can induce quantum interference effects, and consequently, quantum coherences among multiple decaying transition pathways. Depending on the modulation depth and its absolute phase, both the spontaneous emission and the frequency shift may be conveniently modified and controlled.

DOI
10.1103/physreva.90.043838

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•Dec 12, 2013•0 citations
The resonant quantum dynamics of an excited two-level emitter is investigated via classical modulation of its transition frequency while simultaneously the radiator interacts with a broadband electromagnetic field reservoir. The frequency of modulation is selected to be of the order of the bare-state spontaneous decay rate. In this way, one can induce quantum interference effects, and consequently, quantum coherences among multiple decaying transition pathways. Depending on the modulation depth and its absolute phase, both the spontaneous emission and the frequency shift may be conveniently modified and controlled.
We investigate the spontaneous emission spectrum of a three-level atom coherently driven by a microwave field. The microwave excitation establishes a coherent link between the bottom two levels, and as a consequence induces the quantum interference of previously independent decay pathways. As the decay pathways differ from one another by an odd number of stimulated emission processes, the spontaneous emission spectrum acquires a dependence on the phase of the excitation field, a feature that is absent in other resonance fluorescence phenomena.
The spontaneous emission of radiation from two two-level atoms in a Fabry–Perot cavity is considered. The transition frequency of the atoms is assumed to be modulated. It is shown that the frequency modulation leads to radical change of the spontaneous emission dynamics, including the decoherence properties of the entangled atomic states. Two ingredients are necessary in order to achieve this. Firstly, the modulation should be able to periodically detune the atoms from the resonance with the cavity. Secondly, the dynamics of spontaneous emission is efficiently modified if a resonant condition between the modulation frequency and modulation depth is fulfilled. Thus, frequency modulation can be used to dynamically control the collective effects in spontaneous emission in cavities.
We discuss quantum interference effects in the resonance fluorescence spectrum of a \ensuremath{\Lambda} three-level atom when the lower-level doublet is driven by a coherent field. The interfering pathways that lead to the same final state involve both spontaneous decays and stimulated transitions, and differ from one another by an odd number of stimulated processes induced by the driving field. As a consequence, the interference structures depend upon the phase of the coherent field, an effect that is absent in other resonance fluorescence phenomena. The phase dependence of the quantum interference contribution is especially significant when the level splitting of the driven doublet is comparable to the spontaneous decay rates of the competing optical paths.
We investigate the effect of an intense low-frequency field on the population decay of an excited two-level atom, where the two states are connected by a dipole-forbidden transition. In addition to the natural two-photon spontaneous decay, the low-frequency field gives rise to induced two-photon processes, where one of the two photons is spontaneous. Due to the low frequency of the applied field, the induced decay pathways may interfere with each other. We show how varying the parameters of the applied field allows switching between constructive and destructive interference, thereby increasing or decreasing the induced transition rate as compared to the rate without interference. As all relevant competing transitions are of the same multiphoton order, the system is a promising candidate to verify the idea of spontaneous-emission interference induced by multiphoton pathways experimentally.
Quantum interference and coherence lead to many interesting phenomenon and applications in quantum optics. In this dissertation, we study the quantum coherent properties in the following systems and aspects. We first investigate the optical bistability in a combined cavity-cold atoms system. In such a system the atom-photon interaction provides an optical lattice to the atoms and affects the mechanical motion of the atoms while atoms induce a position dependent phase shift on the cavity field. This highly nonlinearity induces optical bistability of intra-cavity photon number with respect to the pumping light added along the cavity axis. We show that the presence of this bistability can be controlled by a second pumping field added perpendicular to the cavity axis. It is also found that the critical input intensity of switching from one branch of bistability to the other depends on the the way of the field being added. This behavior is similar to the anomalous switching of the dispersive optical bistability of atomic media in the cavity. We also study the effect of counter-rotating terms in the control of spontaneous emission. We make use of a unitary transformation method and investigate the effect of dynamic energy shifts on the spontaneous emission modification via quantum interference in a four-level atomic system. We show that the counter-rotating terms, which are normally neglected in the usual investigation of atomic systems, do produce a significant influence on the evolution of the atomic amplitudes and the emission spectrum. This effect of counter-rotating terms can be observed in the time scale of the decay rate even when the dipole moments of the two upper levels are orthogonal to each other. The effect of counter-rotating terms on the spontaneous emission in a 3-D anisotropic photonic crystal is also discussed. It is shown that the behavior of the emission is similar to the case making rotating wave approximation, i.e., the localized and propagating fields are also separated by two characteristic atomic transition frequencies. However, the two characteristic frequencies are shifted due to the full Lamb shift which is obtained with counter-rotating terms being included in the Hamiltonian. We also utilize the unitary transformation method to show how the Lamb shift in a multi-level atom can be controlled by a driving field. Finally, we propose a subwavelength atom localization scheme for an atom located in a standing-wave field. The strategy is based on the observation that the photon statistics of resonance fluorescence depends on the position-dependent Rabi frequency.