Quantum interference and coherence lead to many interesting phenomenon and applications in quantum optics. In this dissertation, we study the quantum coherent properties in the following systems and aspects. We first investigate the optical bistability in a combined cavity-cold atoms system. In such a system the atom-photon interaction provides an optical lattice to the atoms and affects the mechanical motion of the atoms while atoms induce a position dependent phase shift on the cavity field. This highly nonlinearity induces optical bistability of intra-cavity photon number with respect to the pumping light added along the cavity axis. We show that the presence of this bistability can be controlled by a second pumping field added perpendicular to the cavity axis. It is also found that the critical input intensity of switching from one branch of bistability to the other depends on the the way of the field being added. This behavior is similar to the anomalous switching of the dispersive optical bistability of atomic media in the cavity. We also study the effect of counter-rotating terms in the control of spontaneous emission. We make use of a unitary transformation method and investigate the effect of dynamic energy shifts on the spontaneous emission modification via quantum interference in a four-level atomic system. We show that the counter-rotating terms, which are normally neglected in the usual investigation of atomic systems, do produce a significant influence on the evolution of the atomic amplitudes and the emission spectrum. This effect of counter-rotating terms can be observed in the time scale of the decay rate even when the dipole moments of the two upper levels are orthogonal to each other. The effect of counter-rotating terms on the spontaneous emission in a 3-D anisotropic photonic crystal is also discussed. It is shown that the behavior of the emission is similar to the case making rotating wave approximation, i.e., the localized and propagating fields are also separated by two characteristic atomic transition frequencies. However, the two characteristic frequencies are shifted due to the full Lamb shift which is obtained with counter-rotating terms being included in the Hamiltonian. We also utilize the unitary transformation method to show how the Lamb shift in a multi-level atom can be controlled by a driving field. Finally, we propose a subwavelength atom localization scheme for an atom located in a standing-wave field. The strategy is based on the observation that the photon statistics of resonance fluorescence depends on the position-dependent Rabi frequency.
Quantum interference and coherence lead to many interesting phenomenon and applications in quantum optics. In this dissertation, we study the quantum coherent properties in the following systems and aspects. We first investigate the optical bistability in a combined cavity-cold atoms system. In such a system the atom-photon interaction provides an optical lattice to the atoms and affects the mechanical motion of the atoms while atoms induce a position dependent phase shift on the cavity field. This highly nonlinearity induces optical bistability of intra-cavity photon number with respect to the pumping light added along the cavity axis. We show that the presence of this bistability can be controlled by a second pumping field added perpendicular to the cavity axis. It is also found that the critical input intensity of switching from one branch of bistability to the other depends on the the way of the field being added. This behavior is similar to the anomalous switching of the dispersive optical bistability of atomic media in the cavity. We also study the effect of counter-rotating terms in the control of spontaneous emission. We make use of a unitary transformation method and investigate the effect of dynamic energy shifts on the spontaneous emission modification via quantum interference in a four-level atomic system. We show that the counter-rotating terms, which are normally neglected in the usual investigation of atomic systems, do produce a significant influence on the evolution of the atomic amplitudes and the emission spectrum. This effect of counter-rotating terms can be observed in the time scale of the decay rate even when the dipole moments of the two upper levels are orthogonal to each other. The effect of counter-rotating terms on the spontaneous emission in a 3-D anisotropic photonic crystal is also discussed. It is shown that the behavior of the emission is similar to the case making rotating wave approximation, i.e., the localized and propagating fields are also separated by two characteristic atomic transition frequencies. However, the two characteristic frequencies are shifted due to the full Lamb shift which is obtained with counter-rotating terms being included in the Hamiltonian. We also utilize the unitary transformation method to show how the Lamb shift in a multi-level atom can be controlled by a driving field. Finally, we propose a subwavelength atom localization scheme for an atom located in a standing-wave field. The strategy is based on the observation that the photon statistics of resonance fluorescence depends on the position-dependent Rabi frequency.
Quantum interference in spontaneous emission from a four-level atom is investigated with the counter-rotating terms and the energy shifts included. The atom has two upper levels which are coupled to a common lower level by the same vacuum modes and are driven by a coherent field to an auxiliary level. The effect of the counter-rotating terms in the coupling through the vacuum modes is taken into account by a unitary transformation method. We show how the quantum interference due to the energy shifts affects the spontaneous emission.
The author of this thesis concentrates his attention on quantum optical properties of some artificial electromagnetic media, such as quantum coherent atomic vapors (various multilevel electromagnetically induced transparency vapors) and negative refractive index materials, and suggests some possible ways to manipulate wave propagations inside the artificial electromagnetic materials based on quantum coherence and quantum vacuum effects. In Chapters 1 and 2, the author reviews the previous papers on quantum coherence as well as the relevant work such as electromagnetically induced transparency (EIT), atomic population trapping and their various applications. The basic concepts of quantum coherence (atomic phase coherence, quantum interferences within atomic energy levels) and quantum vacuum are introduced, and the theoretical formulations for treating wave propagations in quantum coherent media are presented. In Chapter 3, the author considers three topics on the manipulation of light propagations via quantum coherence and quantum interferences: i) the evolutional optical behaviors (turn-on dynamics) of a four-level N-configuration atomic system is studied and the tunable optical behavior that depends on the intensity ratio of the signal field to the control field is considered. Some typical photonic logic gates (e.g. NOT and NOR gates) are designed based on the tunable four-level optical responses of the N-configuration atomic system; ii) the destructive and constructive quantum interferences between two control transitions (driven by the control fields) in a tripod-type four-level system is suggested. The double-control quantum interferences can be utilized to realize some photonic devices such as the logic-gate devices, e.g., NOT, OR, NOR and EXNOR gates; iii) some new quantum coherent schemes (using EIT and dressed-state mixed-parity transitions) for realizing negative refractive indices are proposed. The most remarkable characteristic (and advantage) of the present scenarios is such that the isotropic left-handed media (with microscopic structure units at the atomic level) in the optical frequency band can be achieved. Quantum vacuum (the ground state of quantized fields) can exhibit many interesting effects. In Chapter 4, we investigate two quantum-vacuum effects in artificial materials: i) the anisotropic distribution of quantum-vacuum momentum density in a moving electromagnetic medium; ii) the angular momentum transfer between quantum vacuum and anisotropic medium. Such quantum-vacuum macroscopic mechanical effects could be detected by current technology, e.g., the so-called fiber optical sensor that can measure motion with nanoscale sensitivity. We expect that these vacuum effects could be utilized to develop sensitive sensor techniques or to design new quantum optical and photonic devices.In Chapter 5, the author suggests some interesting effects due to the combination of quantum coherence and quantum vacuum, i.e., the quantum coherent effects, in which the quantum-vacuum fluctuation field is involved. Two topics are addressed: i) spontaneous emission inhibition due to quantum interference in a three-level system; ii) quantum light-induced guiding potentials for coherent manipulation of atomic matter waves (containing multilevel atoms). These quantum guiding potentials could be utilized to cool and trap atoms, and may be used for the development of new techniques of atom fibers and atom chips, where the coherent manipulation of atomic matter waves is needed.In Chapter 6, we conclude this thesis with some remarks, briefly discuss new work that deserves further consideration in the future, and present a guide to the previously published papers by us.
Optical response of an active medium can substantially be modified when coherent superpositions of states are excited, that is, when systems display quantum coherence and interference. This has led to fascinating applications in atomic and molecular systems. Examples include coherent population trapping, lasing without inversion, electromagnetically induced transparency, cooperative spontaneous emission, and quantum entanglement. \n \nWe study quantum coherence effects in several quantum optical systems and find interesting applications. We show that quantum coherence can lead to transient Raman lasing and lasing without inversion in short wavelength spectral regions--extreme ultraviolet and x-ray--without the requirement of incoherent pumping. For example, we demonstrate transient Raman lasing at 58.4 nm in Helium atom and transient lasing without inversion at 6.1 nm in Helium-like Boron (triply-ionized Boron). We also investigate dynamical properties of a collective superradiant state prepared by absorption of a single photon when the size of the sample is larger than the radiation wavelength. We show that for large number of atoms such a state, to a good approximation, decays exponentially with a rate proportional to the number of atoms. We also find that the collective frequency shift resulting from repeated emission and reabsorption of short-lived virtual photons is proportional to the number of species in the sample. Furthermore, we examine how a position-dependent excitation phase affects the evolution of entanglement between two dipole-coupled qubits. It turns out that the coherence induced by position-dependent excitation phase slows down the otherwise fast decay of the two-qubit entanglement. We also show that it is possible to entangle two spatially separated and uncoupled qubits via interaction with correlated photons in a cavity quantum electrodynamics setup. Finally, we analyze how quantum coherence can be used to generate continuous-variable entanglement in quantum-beat lasers in steady state and propose possible implementation in quantum lithography.
We analyze the absorptive and hybrid absorptive–dispersive double-cavity optical bistability behavior in a four-level N-type atomic system driven by two optical fields circulating inside two independently unidirectional ring cavities and a trigger field outside the cavities. In this system, the two-photon absorption and cross Kerr nonlinearity play significant roles in the formation of bistability and can be controlled efficiently due to the quantum interference effect, and then the resulting nonlinear behavior exhibits different features from the two/three-level schemes. It is shown that the threshold values and hysteresis cycle width of the bistable curve can be manipulated via the adjustment of the system parameters. Meanwhile, we also obtain double-beam optical multistability. When adding positive and negative pulses to the cavity input, all-optical steady-state switching for the two cavity outputs can be achieved simultaneously. Therefore, the proposed scheme may have potential applications in all-optical communication and computing.
Optical bistability (OB) and optical multi-stability (OM) of a four-level Λ-type atomic system with two fold lower levels inside a unidirectional ring cavity is investigated. The effect of quantum interference arising from spontaneous emission and incoherent pumping on OB and OM is discussed. It is found that the threshold of OB and OM can be controlled by quantum interference mechanisms. In addition intensity of coupling field and the rate of an incoherent pumping field on behavior of OB and OM are then discussed.
Abstract We describe the linear and nonlinear optical properties of a four-level atomic system, after reducing it to an effective two-level atomic model under the condition of adiabatic shifting of resonances driven by two coherent off-resonant fields. The reduced form of the Hamiltonian corresponding to the two-level system is obtained by employing an adiabatic elimination procedure in the rate equations of the probability amplitudes for the proposed four-level model. For a weak probe field operating in the system, the nonlinear dependence of complex susceptibility on the Rabi frequencies and the detuning parameters of the off-resonant driving fields makes it possible to exhibit coherent control of single-photon and two-photon absorption and transparency, the evolution of enhanced Self-Kerr nonlinearity and noticeable dispersive switching. We have shown how the quantum interference results in the generic four-level model at the adiabatic limit. The present scheme describes the appearance of single-photon transparency without invoking any exact two-photon resonance.