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arXiv:1408.3384 · Nature Photonics

All-optical coherent control of vacuum Rabi oscillations

Ranojoy Bose, Tao Cai, Kaushik Roy Choudhury, Glenn S. Solomon, Edo Waks A

Published Oct 3, 2014• 78 citations
arXivHTMLPDF
DOI
10.1038/nphoton.2014.224

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Vacuum Rabi oscillation is a damped oscillation in which energy can transfer between an atomic excitation and a photon when an atom is strongly coupled to a photonic cavity. This process is challenging to be coherently controlled due to the fact that interaction between the atom and the electromagnetic resonator needs to be modulated in a quick manner compared to vacuum Rabi frequency. This control has been achieved at microwave frequencies, but has remained challenging to be implemented in the optical domain. Here we demonstrated coherent control of energy transfer in a semiconductor quantum dot strongly coupled to a photonic crystal molecule by manipulating the vacuum Rabi oscillation of the system. Instead of using a single photonic crystal cavity, we utilized a photonic crystal molecule consisting two coupled photonic crystal defect cavities to obtain both strong quantum dot-cavity coupling and cavityenhanced AC stark shift. In our system the AC stark shift modulates the coupling interaction between the quantum dot and the cavity by shifting the quantum dot resonance, on timescales (picosecond) shorter than the vacuum Rabi period. We demonstrated the ability to transfer excitation between a quantum dot and cavity, and performed coherent control of light-matter states. Our results provides an ultra-fast approach for probing and controlling light-matter interactions in an integrated nanophotonic device, and could pave the way for gigahertz rate synthesis of arbitrary quantum states of light at optical frequencies.
We study the all-optical time control of the strong coupling between a single cascade three-level quantum emitter and a microcavity. We find that only specific arrival times of the control pulses succeed in switching off the Rabi oscillations. Depending on the arrival times of control pulses, a variety of exotic nonadiabatic cavity quantum electrodynamics effects can be observed. We show that control pulses with specific arrival times, performing which-path and quantum-eraser operations, are able to suddenly switch-off and on first-order coherence of cavity photons, without affecting their strong coupling population dynamics.