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arXiv:1406.5080 · Physical Review A

Single-atom addressing in microtraps for quantum-state engineering using Rydberg atoms

Henning Labuhn, Sylvain Ravets, Daniel Barredo, Lucas Béguin, Florence Nogrette, Thierry Lahaye, Antoine Browaeys

Published Aug 22, 2014• 92 citations
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Abstract

We report on the selective addressing of an individual atom in a pair of single-atom microtraps separated by $3\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}$m. Using a tunable light shift, we render the selected atom off-resonant with a global Rydberg excitation laser which is resonant with the other atom, making it possible to selectively block this atom from being excited to the Rydberg state. Furthermore we demonstrate the controlled manipulation of a two-atom entangled state by using the addressing beam to induce a phase shift onto one component of the wave function of the system, transferring it to a dark state for the Rydberg excitation light. Our results are an important step towards implementing quantum information processing and quantum simulation with large arrays of Rydberg atoms.

DOI
10.1103/physreva.90.023415

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We report on the selective addressing of an individual atom in a pair of single-atom microtraps separated by 3\ensuremathμ3\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}3\ensuremathμm. Using a tunable light shift, we render the selected atom off-resonant with a global Rydberg excitation laser which is resonant with the other atom, making it possible to selectively block this atom from being excited to the Rydberg state. Furthermore we demonstrate the controlled manipulation of a two-atom entangled state by using the addressing beam to induce a phase shift onto one component of the wave function of the system, transferring it to a dark state for the Rydberg excitation light. Our results are an important step towards implementing quantum information processing and quantum simulation with large arrays of Rydberg atoms.
We report on the local control of the transition frequency of a spin 1/2 encoded in two Rydberg levels of an individual atom by applying a state-selective light shift using an addressing beam. With this tool, we first study the spectrum of an elementary system of two spins, tuning it from a nonresonant to a resonant regime, where "bright" (super-radiant) and "dark" (subradiant) states emerge. We observe the collective enhancement of the microwave coupling to the bright state. We then show that after preparing an initial single spin excitation and letting it hop due to the spin-exchange interaction, we can freeze the dynamics at will with the addressing laser, while preserving the coherence of the system. In the context of quantum simulation, this scheme opens exciting prospects for engineering inhomogeneous XY spin Hamiltonians or preparing spin-imbalanced initial states.
Abstract Neutral atom arrays are particularly promising for large-scale quantum computing because it is possible to prepare large-scale qubit arrays. An unsolved issue is how to selectively excite one qubit deep in a 3D atomic array to Rydberg states. In this work, we show two methods for this purpose. The first method relies on a well-known result: in a dipole transition between two quantum states driven by two off-resonant fields of equal strength but opposite detunings ±Δ, the transition is characterized by two counter-rotating Rabi frequencies Ω e ± i Δ t (or ± Ω e ± i Δ t if the two fields have a π -phase difference). This pair of detuned fields lead to a time-dependent Rabi frequency 2 Ω cos ( Δ t ) (or 2 i Ω sin ( Δ t ) ), so that a full transition between the two levels is recovered. We show that when the two detuned fields are sent in different directions, one atom in a 3D optical lattice can be selectively addressed for Rydberg excitation, and when its state is restored, the state of any nontarget atoms irradiated in the light path is also restored. Moreover, we find that the Rydberg excitation by this method can significantly suppress the fundamental blockade error of a Rydberg gate, paving the way for a high-fidelity entangling gate with a commonly used quasi-rectangular pulse that is easily obtained by pulse pickers. Along the way, we find a second method for single-site Rydberg addressing in 3D, where a selected target atom can be excited to the Rydberg state while preserving the state of any nontarget atom due to a spin-echo sequence. The capability to selectively address a target atom in 3D atomic arrays for Rydberg excitation makes it possible to design a large-scale neutral-atom information processor based on the Rydberg blockade.
Neutral atoms trapped and manipulated by laser light provide experimentally well accessible quantum systems allowing for a high degree of control over external and internal degrees of freedom. Arrays of dipole traps in which the atoms are confined individually in a configurable geometry constitute a versatile platform for quantum simulation and information applications. By exciting these atoms into Rydberg states, interactions of variable strength and range can be introduced into the system, allowing for the implementation of entangling gate operations or spin Hamiltonians. A crucial requirement for these schemes to function in a reliable way is the ability to create defect-free arrays of single atoms. This is generally a challenge in these types of systems, as common atom loading schemes are limited to roughly 50% probability of filling each site. In this work, a technique for the rearrangement of atoms within a scalable architecture based on micro-optical lens arrays was developed and implemented, resulting in the creation of uniformly filled regions containing more than 100 atoms, which represent the largest defect-free structures realized so far in systems of this kind. This was accomplished by filling the empty traps in a pre-defined pattern with an atom one by one using an optical tweezer. Thus, structures with up to 5 x 5 atoms could be rendered defect-free in more than 99% of attempts. Although the success rate drops below unity for larger clusters, a value of 3.1% for a 100-atom structure is still viable for experiments working with post-selection methods. The filling fraction of even the largest examined structures was observed to be higher than 88%, surpassing common loading schemes by a significant margin. The measurements presented in this thesis build on a region of the array containing 361 sites, being limited by available laser power. In contrast, the addressable range of the optical tweezer includes more than 1500 sites and microlens arrays with up to a million lenses are commercially available. By implementing coherent Rydberg excitation of this assembled atom array, significant progress toward a universal quantum computer or flexible quantum simulator has been made. Using a two-photon excitation scheme, coherent dynamics between the ground and Rydberg state could be observed simultaneously in a 5 x 5 region of the array, with two-photon Rabi frequencies on the order of Omega = 2Pi x 500kHz measured for a Rydberg laser beam waist of w_0,B = 18.7(10) µm. The choice of an appropriate Rydberg state and interatomic spacing led to the presence of strong nearest-neighbor interactions and allowed for the demonstration of the Rydberg blockade effect by observing a collective enhancement of the Rabi frequency consistent with the expected scaling ~ sqrt(N) as well as the suppression of multiple excitations. This mechanism represents the fundamental constituent of a two-qubit gate operation. The architecture introduced in this work offers a scalability unique among quantum simulation platforms and the presented results underpin its potential to propel the atom-optical approach for quantum information processing beyond the threshold of quantum supremacy. Different approaches for scaling up the system have been explored, indicating that defect-free structures of more than 1000 atoms are within range with feasible experimental improvements. Through a detailed analysis of the factors limiting the coherence of the observed dynamics, strategies for future experimental improvements have been developed. Among these, increasing the coupling strength to the Rydberg state into the megahertz regime by increasing laser power and implementing single-site addressing represents the most straight-forward and promising approach.
Precise individual addressing of single atoms in quantum registers formed by optical trap arrays is essential to achieve high-fidelity quantum gates in neutral-atom quantum computers and simulators. Two-qubit quantum gates are typically implemented using coherent two-photon laser excitation of atoms to strongly interacting Rydberg states. However, two-photon excitation encounters challenges in individual addressing with tightly focused laser beams due to atom position uncertainty and the spatial inhomogeneity in both Rabi frequencies and light shifts. In this work, we theoretically demonstrate that the fidelity of individual addressing is significantly enhanced by employing coherent three-photon laser excitation of Rydberg states. For a specific example of $5{s}_{1/2}\stackrel{{\mathrm{\ensuremath{\Omega}}}_{1}}{\ensuremath{\rightarrow}}5{p}_{3/2}\stackrel{{\mathrm{\ensuremath{\Omega}}}_{2}}{\ensuremath{\rightarrow}}7{s}_{1/2}\stackrel{{\mathrm{\ensuremath{\Omega}}}_{3}}{\ensuremath{\rightarrow}}np$ excitation in 87Rb^{87}\mathrm{Rb}87Rb atoms, we find that upon strong laser coupling in the second step (Rabi frequency ${\mathrm{\ensuremath{\Omega}}}_{2}$) and moderate coupling in the first and third steps (Rabi frequencies ${\mathrm{\ensuremath{\Omega}}}_{1}$ and ${\mathrm{\ensuremath{\Omega}}}_{3}$), the three-photon Rabi frequency is given by $\mathrm{\ensuremath{\Omega}}={\mathrm{\ensuremath{\Omega}}}_{1}{\mathrm{\ensuremath{\Omega}}}_{3}/{\mathrm{\ensuremath{\Omega}}}_{2}$. If the spatial distributions of $({\mathrm{\ensuremath{\Omega}}}_{1}{\mathrm{\ensuremath{\Omega}}}_{3})$ and ${\mathrm{\ensuremath{\Omega}}}_{2}$ are arranged to be identical, $\mathrm{\ensuremath{\Omega}}$ becomes independent of atom position, even within very tightly focused laser beams. This approach dramatically improves individual addressing of Rydberg excitation for neighboring atoms in trap arrays compared to conventional two-photon excitation schemes. Our findings are crucial for large-scale quantum registers of neutral atoms, where distances between adjacent atoms should be minimized to ensure stronger Rydberg interactions and compact arrangement of atom arrays.
Neutral atoms provide an excellent resource for quantum information processing, combining the long atomic coherence times of the hyperfine ground-state with strong dipole-dipole interactions of highly excited Rydberg states for generating deterministic entanglement between qubits separated by < 10 µm [1]. Scalable long-range interactions can be obtained by coupling the atomic array to a superconducting microwave cavity enabling hybrid quantum information processing where the cavity-mediated entanglement allows atoms to be coupled over cm length scales. We present the first steps towards such an experiment incorporating high fidelity readout using an sCMOS camera [2] and the ability to drive fast, optically addressable rotations of the hyperfine-encoded qubits to the Rydberg state. Using our sub-kHz cavitystabilised laser system [3] we demonstrate coherent control of single Rydberg atoms, performing Ramsey spectroscopy to determine coherence time and to generate entanglement between a pair of atoms separated by 6 µm. Combining this excitation scheme with our ground-state Raman lasers we show progress towards the implementation of a mesoscopic Rydberg gate based on electromagnetically induced transparency (EIT) offering robust entanglement of multi-atom ensembles [4].
Ultracold atoms confined in microtrap array is a highly versatile platform for quantum many-body physics, quantum simulation and quantum computation because of the easy scalability, long coherence time, single site addressability and controllable interactions, e.g. using Rydberg states. Here, we demonstrate an novel method to prepare versatile arrays of atomic ensembles by transferring them from a pancake shaped optical reservoir to an array of optical tweezers produced via direct projection of light patterns produced via a digital micromirror device. The size of each ensemble is smaller than the Rydberg blockade radius, such that each one can carry either 0 or 1 (collective) excitations which can then strongly interact with the neighbouring ensembles. Finally I will discuss a recent proposal to use such Rydberg arrays to realise programmable quantum systems in the form of quantum cellular automata (QCA). This opens a path to study many-body quantum dynamics in quantum and classical regimes, to engineer highly entangled quantum states and toward an inherently scalable approach to quantum information processing and computing.