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arXiv:2411.06607 · Physical Review A

High-fidelity individual addressing of single atoms in quantum registers at three-photon laser excitation of Rydberg states

Nikolai N. Bezuglov, Ilya I. Beterov, A. Cinins, K. Miculis, Vasily M. Entin, P. I. Betleni, G. Suliman, V. V. Gromyko, Denis B. Tretyakov, Elena A. Yakshina, I. I. Ryabtsev

Published Oct 17, 2025• 2 citations
arXivHTMLPDF

Abstract

Precise individual addressing of single atoms in quantum registers formed by optical trap arrays is essential to achieve high-fidelity quantum gates in neutral-atom quantum computers and simulators. Two-qubit quantum gates are typically implemented using coherent two-photon laser excitation of atoms to strongly interacting Rydberg states. However, two-photon excitation encounters challenges in individual addressing with tightly focused laser beams due to atom position uncertainty and the spatial inhomogeneity in both Rabi frequencies and light shifts. In this work, we theoretically demonstrate that the fidelity of individual addressing is significantly enhanced by employing coherent three-photon laser excitation of Rydberg states. For a specific example of $5{s}_{1/2}\stackrel{{\mathrm{\ensuremath{\Omega}}}_{1}}{\ensuremath{\rightarrow}}5{p}_{3/2}\stackrel{{\mathrm{\ensuremath{\Omega}}}_{2}}{\ensuremath{\rightarrow}}7{s}_{1/2}\stackrel{{\mathrm{\ensuremath{\Omega}}}_{3}}{\ensuremath{\rightarrow}}np$ excitation in $^{87}\mathrm{Rb}$ atoms, we find that upon strong laser coupling in the second step (Rabi frequency ${\mathrm{\ensuremath{\Omega}}}_{2}$) and moderate coupling in the first and third steps (Rabi frequencies ${\mathrm{\ensuremath{\Omega}}}_{1}$ and ${\mathrm{\ensuremath{\Omega}}}_{3}$), the three-photon Rabi frequency is given by $\mathrm{\ensuremath{\Omega}}={\mathrm{\ensuremath{\Omega}}}_{1}{\mathrm{\ensuremath{\Omega}}}_{3}/{\mathrm{\ensuremath{\Omega}}}_{2}$. If the spatial distributions of $({\mathrm{\ensuremath{\Omega}}}_{1}{\mathrm{\ensuremath{\Omega}}}_{3})$ and ${\mathrm{\ensuremath{\Omega}}}_{2}$ are arranged to be identical, $\mathrm{\ensuremath{\Omega}}$ becomes independent of atom position, even within very tightly focused laser beams. This approach dramatically improves individual addressing of Rydberg excitation for neighboring atoms in trap arrays compared to conventional two-photon excitation schemes. Our findings are crucial for large-scale quantum registers of neutral atoms, where distances between adjacent atoms should be minimized to ensure stronger Rydberg interactions and compact arrangement of atom arrays.

DOI
10.1103/s918-nqsp

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Neutral atoms trapped and manipulated by laser light provide experimentally well accessible quantum systems allowing for a high degree of control over external and internal degrees of freedom. Arrays of dipole traps in which the atoms are confined individually in a configurable geometry constitute a versatile platform for quantum simulation and information applications. By exciting these atoms into Rydberg states, interactions of variable strength and range can be introduced into the system, allowing for the implementation of entangling gate operations or spin Hamiltonians. A crucial requirement for these schemes to function in a reliable way is the ability to create defect-free arrays of single atoms. This is generally a challenge in these types of systems, as common atom loading schemes are limited to roughly 50% probability of filling each site. In this work, a technique for the rearrangement of atoms within a scalable architecture based on micro-optical lens arrays was developed and implemented, resulting in the creation of uniformly filled regions containing more than 100 atoms, which represent the largest defect-free structures realized so far in systems of this kind. This was accomplished by filling the empty traps in a pre-defined pattern with an atom one by one using an optical tweezer. Thus, structures with up to 5 x 5 atoms could be rendered defect-free in more than 99% of attempts. Although the success rate drops below unity for larger clusters, a value of 3.1% for a 100-atom structure is still viable for experiments working with post-selection methods. The filling fraction of even the largest examined structures was observed to be higher than 88%, surpassing common loading schemes by a significant margin. The measurements presented in this thesis build on a region of the array containing 361 sites, being limited by available laser power. In contrast, the addressable range of the optical tweezer includes more than 1500 sites and microlens arrays with up to a million lenses are commercially available. By implementing coherent Rydberg excitation of this assembled atom array, significant progress toward a universal quantum computer or flexible quantum simulator has been made. Using a two-photon excitation scheme, coherent dynamics between the ground and Rydberg state could be observed simultaneously in a 5 x 5 region of the array, with two-photon Rabi frequencies on the order of Omega = 2Pi x 500kHz measured for a Rydberg laser beam waist of w_0,B = 18.7(10) µm. The choice of an appropriate Rydberg state and interatomic spacing led to the presence of strong nearest-neighbor interactions and allowed for the demonstration of the Rydberg blockade effect by observing a collective enhancement of the Rabi frequency consistent with the expected scaling ~ sqrt(N) as well as the suppression of multiple excitations. This mechanism represents the fundamental constituent of a two-qubit gate operation. The architecture introduced in this work offers a scalability unique among quantum simulation platforms and the presented results underpin its potential to propel the atom-optical approach for quantum information processing beyond the threshold of quantum supremacy. Different approaches for scaling up the system have been explored, indicating that defect-free structures of more than 1000 atoms are within range with feasible experimental improvements. Through a detailed analysis of the factors limiting the coherence of the observed dynamics, strategies for future experimental improvements have been developed. Among these, increasing the coupling strength to the Rydberg state into the megahertz regime by increasing laser power and implementing single-site addressing represents the most straight-forward and promising approach.
Scalable quantum computers and quantum networks require the combination of quantum processing nodes with efficient light-matter interfaces to distribute quantum information in local or long-distance quantum networks. Neutral-atom arrays have both been coupled to Rydberg states to enable high-fidelity quantum gates in universal processing architectures, and to optical cavities to realize interfaces to photons. However, combining these two capabilities and coupling atom arrays to highly excited Rydberg states in the mode of an optical cavity has been an outstanding challenge. Here we present a novel cavity-coupled Rydberg array that achieves this long-standing goal. We prepare, detect, and control individual atoms in a scalable optical tweezer array, couple them strongly to the optical mode of a high-finesse optical cavity and excite them in a controlled way to Rydberg states. We show that high-cooperativity coupling to an optical cavity -- demonstrated via the dispersive shift of the resonance of the cavity in presence of the atoms -- and strong Rydberg interactions -- demonstrated via the collective enhancement of Rydberg coupling in the atomic array -- can be achieved in our setup at the same spatial location. Our presented experimental platform opens the path to several new directions, including the realization of quantum network nodes, quantum simulation of long-range interacting, open quantum systems and photonic-state engineering leveraging high-fidelity Rydberg control.
Abstract Neutral atom arrays are particularly promising for large-scale quantum computing because it is possible to prepare large-scale qubit arrays. An unsolved issue is how to selectively excite one qubit deep in a 3D atomic array to Rydberg states. In this work, we show two methods for this purpose. The first method relies on a well-known result: in a dipole transition between two quantum states driven by two off-resonant fields of equal strength but opposite detunings ±Δ, the transition is characterized by two counter-rotating Rabi frequencies Ω e ± i Δ t (or ± Ω e ± i Δ t if the two fields have a π -phase difference). This pair of detuned fields lead to a time-dependent Rabi frequency 2 Ω cos ( Δ t ) (or 2 i Ω sin ( Δ t ) ), so that a full transition between the two levels is recovered. We show that when the two detuned fields are sent in different directions, one atom in a 3D optical lattice can be selectively addressed for Rydberg excitation, and when its state is restored, the state of any nontarget atoms irradiated in the light path is also restored. Moreover, we find that the Rydberg excitation by this method can significantly suppress the fundamental blockade error of a Rydberg gate, paving the way for a high-fidelity entangling gate with a commonly used quasi-rectangular pulse that is easily obtained by pulse pickers. Along the way, we find a second method for single-site Rydberg addressing in 3D, where a selected target atom can be excited to the Rydberg state while preserving the state of any nontarget atom due to a spin-echo sequence. The capability to selectively address a target atom in 3D atomic arrays for Rydberg excitation makes it possible to design a large-scale neutral-atom information processor based on the Rydberg blockade.
Individually trapped neutral atoms are a promising candidate for use in quantum computing and simulation applications. They are highly scalable, have long coherence times and can be entangled via strong dipole-dipole interactions by driving to highly excited Rydberg states. However, the fidelity of single atom operations as well as two-atom entangling operations is limited by intrinsic sources of decoherence such as atomic motion, as well as technical sources of noise such as laser intensity fluctuations and phase/frequency fluctuations. We study the effect of these factors on single atom Rabi oscillations and two-atom Rydberg blockaded Rabi oscillations, using perturbation theory and numerical simulation. We develop a window function approach which helps us qualitatively understand the significance of the different spectral components of the noise as well as quantitatively understand the dependence of the Rabi oscillation fidelity on Rabi frequency. This allows us to predict the maximum experimentally achievable fidelities using independent measurements of experimental parameters such as noise spectra and atomic temperature. Turning to the question of near-term scalability of the experimental system, we prototype and test a method of generating a ’ladder’ configuration of optical tweezers utilizing two independent lasers. Our setup allows us to fully tune the geometry of the ladder, namely the separation between the two rows, the angle between them, and their relative position along the axis of the ladder. This pseudo-2D configuration enables us to reach larger system sizes in the near future and allows us to access beyond 1D physics.
Neutral atoms in optical tweezer arrays have emerged as a leading platform for quantum information processing. The fidelity of entangling gates mediated by Rydberg interactions has improved rapidly and is increasingly constrained by blackbody-radiation-induced transitions, which shorten Rydberg lifetimes and create contaminant states that can cause correlated errors. Cryogenic environments can suppress these transition rates by more than an order of magnitude. However, realizing a universal gate set in such an environment has remained an outstanding challenge. Here, we demonstrate a universal quantum gate set in a cryogenic 133^{133}133Cs atom array, with a single-qubit gate fidelity of 99.970(2)% and a raw two-qubit entangling-gate fidelity of 99.76(8)%, within the range of leading room-temperature implementations. The entangling gate uses direct single-photon coupling between the electronic ground state and a Rydberg PPP state, avoiding scattering and light shifts associated with two-photon coupling. The gate operates at a modest Rabi frequency of 2π×4.32π\times4.32π×4.3 MHz. The measured fidelity agrees with our error model dominated by atomic motion, indicating a straightforward route to higher fidelity through improved cooling, while the fundamental error contribution from Rydberg decay is below 3×10−43\times10^{-4}3×10−4. These results establish a path to entangling-gate fidelities substantially beyond the current state of the art through cryogenic suppression of Rydberg decay, reducing the overhead for fault-tolerant computation.
We have numerically simulated a two-qubit CZ gate for ultracold neutral atoms based on Rydberg blockade, utilizing three-photon excitation to Rydberg states. The three-photon laser excitation overcomes lack of individual addressability for entangling gates in atomic arrays, which is a key limitation of conventional schemes of quantum information processing with neutral atoms. This is achieved by mitigating sensitivity to laser intensity fluctuations caused by spatial motion of atoms in optical tweezers. Our goal is to investigate the gate performance when three-photon laser excitation is used. We considered Levine-Pichler gate which applies an abrupt phase jump at the center of the control laser pulse. Our simulation accounts for the influence of spontaneous decay of intermediate and Rydberg states and finite Rydberg excitation energies. We obtained the maximum fidelity of the CZ gate around 99.7% for the model based on probability amplitudes and 99.72% for the model based on density matrices. This value exceeds the threshold required for the application of quantum error correction protocols, demonstrating the promise of this gate for experimental realization. This work was supported by BASIS foundation Grant No. № 25-1-1-57-5