Neutral atoms provide an excellent resource for quantum information processing, combining the long atomic coherence times of the hyperfine ground-state with strong dipole-dipole interactions of highly excited Rydberg states for generating deterministic entanglement between qubits separated by < 10 µm [1]. Scalable long-range interactions can be obtained by coupling the atomic array to a superconducting microwave cavity enabling hybrid quantum information processing where the cavity-mediated entanglement allows atoms to be coupled over cm length scales. We present the first steps towards such an experiment incorporating high fidelity readout using an sCMOS camera [2] and the ability to drive fast, optically addressable rotations of the hyperfine-encoded qubits to the Rydberg state. Using our sub-kHz cavitystabilised laser system [3] we demonstrate coherent control of single Rydberg atoms, performing Ramsey spectroscopy to determine coherence time and to generate entanglement between a pair of atoms separated by 6 µm. Combining this excitation scheme with our ground-state Raman lasers we show progress towards the implementation of a mesoscopic Rydberg gate based on electromagnetically induced transparency (EIT) offering robust entanglement of multi-atom ensembles [4].
Neutral atoms provide an excellent resource for quantum information processing, combining the long atomic coherence times of the hyperfine ground-state with strong dipole-dipole interactions of highly excited Rydberg states for generating deterministic entanglement between qubits separated by < 10 µm [1]. Scalable long-range interactions can be obtained by coupling the atomic array to a superconducting microwave cavity enabling hybrid quantum information processing where the cavity-mediated entanglement allows atoms to be coupled over cm length scales. We present the first steps towards such an experiment incorporating high fidelity readout using an sCMOS camera [2] and the ability to drive fast, optically addressable rotations of the hyperfine-encoded qubits to the Rydberg state. Using our sub-kHz cavitystabilised laser system [3] we demonstrate coherent control of single Rydberg atoms, performing Ramsey spectroscopy to determine coherence time and to generate entanglement between a pair of atoms separated by 6 µm. Combining this excitation scheme with our ground-state Raman lasers we show progress towards the implementation of a mesoscopic Rydberg gate based on electromagnetically induced transparency (EIT) offering robust entanglement of multi-atom ensembles [4].
This thesis reports progress towards using hyperfine-encoded neutral atomic ensembles for quantum information applications. Ensemble qubits are alternative building blocks to process quantum information, while circumventing the challenges preparing a low-entropy single-atom qubit register. While ensemble approach inherits the single-atom quantum gate protocols, cooperative atom-light interaction makes it favorable platform to implement atom-photon interface, such as quantum memory. We have demonstrated semi-deterministic preparation of W-state, which we use as an ensemble qubit. Observed 50–60% preparation fidelity shows discrepancy to expected > 80% fidelity including known imperfections. We suspect Ground-Rydberg and Rydberg-Rydberg molecular interactions within the ensemble modify the dynamics. State tomography and Ramsey experiment clearly identified that majority of constituents in an ensemble are indeed entangled. We report the first measurement of W-state coherence time as 2.6ms for 7.6 atoms, which is long enough to perform 2600 Rydberg-mediated quantum gate operations. The first demonstration of Rydberg blockade between two ensembles happened in the same apparatus. We observe blockade fidelity of 0.89 (uncorrected) and near unity when post-selected on successful N = 1 Fock state preparation of Control ensemble. For weakly blockaded cases, Target ensemble remained as a perturber inhibiting Control ensemble from de-excitation. We discuss the efficacy of optical lattice insertion to suppress molecular interactions that might have been affecting the Rydberg dynamics. High fidelity, parallel, low loss fluorescence detection of hyperfine ground state of rubidium atoms is presented. Enforced cycling transition scattering minimally alters the internal states. We achieve mean state detection fidelity of 97% (uncorrected) and 98.7% (SPAM error corrected), with atom loss rate < 2% and hyperfine-changing rate < 2%. This scalable technique is also compatible with ensemble qubits and error correcting schemes. Technical developments on apparatus, lasers, supporting hardware and software are discussed. Automatic beam alignment system is implemented to correct long term drift of tightly focused addressing beams. Achieved pointing stability of 60 nm. Two home-made, high performing, cavity-enhanced frequency doubling systems were constructed to meet experimental demand. We observe 960/480 system output as high as 180 mW with 600 mW fundamental, and 1540/770 system output as high as 13.97 W from 19 W fundamental.
We report results of a ground-state entanglement protocol for a pair of Cs atoms separated by 6 μ m, combining the Rydberg blockade mechanism with a two-photon Raman transition to prepare the Bell state with a loss-corrected fidelity of 0.81(5), equal to the best demonstrated fidelity for atoms trapped in optical tweezers but without the requirement for dynamically adjustable interatomic spacing. Qubit state coherence is also critical for quantum information applications, and we characterise both ground-state and ground-Rydberg dephasing rates using Ramsey spectroscopy. We demonstrate transverse dephasing times ms and s for the qubit levels and achieve long ground-Rydberg coherence times of as required for implementing high-fidelity multi-qubit gate sequences where a control atom remains in the Rydberg state while applying local operations on neighbouring target qubits.
We show that an array of polar molecules interacting with Rydberg atoms is a promising hybrid system for scalable quantum computation.Quantum information is stored in long-lived hyperfine or rotational states of molecules, which interact indirectly through resonant dipole-dipole interactions with Rydberg atoms.A two-qubit gate based on this interaction has a duration of 1 μs and an achievable fidelity of 99.9%.The gate has little sensitivity to the motional states of the particles-the molecules can be in thermal states, the atoms do not need to be trapped during Rydberg excitation, the gate does not heat the molecules, and heating of the atoms has a negligible effect.Within a large, static array, the gate can be applied to arbitrary pairs of molecules separated by tens of micrometres, making the scheme highly scalable.The molecule-atom interaction can also be used for rapid qubit initialization and efficient, nondestructive qubit readout, without driving any molecular transitions.Single-qubit gates are driven using microwave pulses alone, exploiting the strong electric dipole transitions between rotational states.Thus, all operations required for large-scale quantum computation can be done without moving the molecules or exciting them out of their ground electronic states.
The advent of digital neutral-atom quantum computers relies on the development of fast and robust protocols for high-fidelity quantum operations. In this work, we introduce a novel scheme for entangling gates using four atomic levels per atom: a ground-state qubit and two Rydberg states. A laser field couples the qubit to one of the two Rydberg states, while a microwave field drives transitions between the two Rydberg states, enabling a resonant dipole-dipole interaction between different atoms. We show that controlled- Z gates can be realized in this scheme without requiring optical phase modulation and relying solely on a microwave field with time-dependent phase and amplitude. We demonstrate that such gates are faster and less sensitive to Rydberg decay than state-of-the-art Rydberg gates based on van der Waals interactions. Moreover, we systematically stabilize our protocol against interatomic distance fluctuations and analyze its performance in realistic setups with rubidium or cesium atoms. Our results open up new avenues to the use of microwave-driven dipolar interactions for quantum computation with neutral atoms.
We report the implementation of universal two- and three-qubit entangling gates on neutral-atom qubits encoded in long-lived hyperfine ground states. The gates are mediated by excitation to strongly interacting Rydberg states and are implemented in parallel on several clusters of atoms in a one-dimensional array of optical tweezers. Specifically, we realize the controlled-phase gate, enacted by a novel, fast protocol involving only global coupling of two qubits to Rydberg states. We benchmark this operation by preparing Bell states with fidelity F≥95.0(2)%, and extract gate fidelity ≥97.4(3)%, averaged across five atom pairs. In addition, we report a proof-of-principle implementation of the three-qubit Toffoli gate, in which two control atoms simultaneously constrain the behavior of one target atom. These experiments demonstrate key ingredients for high-fidelity quantum information processing in a scalable neutral-atom platform.
Neutral atom arrays have rapidly emerged as a leading platform for quantum computing, boasting scalable, configurable arrays of single atoms trapped in optical tweezers, fast, high-fidelity entangling gates through Rydberg interactions, and programmable, parallelized control of qubit operations. Coupling an atom array to an optical cavity opens a new frontier. Leveraging enhanced light-atom interactions in cavity quantum electrodynamics, cavity- coupled atom arrays acquire capabilities that can further expand the neutral atom toolbox, including cavity-enhanced atom readouts, atom-photon entanglement, and photon-mediated interactions between distant atoms. This thesis presents a quantum hardware platform that integrates an array of neutral atoms with a high-finesse optical cavity. After describing the design and development of the experimental apparatus, I demonstrate high-fidelity atom state readout through the cavity, achieving improved speed and atom survival compared to conventional free-space imaging methods. I then introduce a new technique for selectively controlling atom-cavity coupling on arbitrary subsets of the array, using local AC Stark shifts on the excited states of the atoms. Building on these tools, I demonstrate fast, non-destructive cavity-based readout of atom arrays, a crucial bottleneck of atom array platforms. I also showcase real-time measurement and feedback capabilities with a demonstration of classical error correction, using a register of atomic bits. Finally, I describe progress toward implementing single- and two-qubit gates within the cavity-coupled system. By combining coherent control, tunable interactions, and high-fidelity, non-destructive readout integrated and real-time feedback, the cavity-coupled Rydberg atom array offers a promising path toward fault-tolerant quantum computing.