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Rydberg-Mediated Atomic Ensemble Entanglement and Hyperfine Qubit Detection

Minho Kwon

Published Jan 1, 2019• 1 citation
OpenAlex

Abstract

This thesis reports progress towards using hyperfine-encoded neutral atomic ensembles for quantum information applications. Ensemble qubits are alternative building blocks to process quantum information, while circumventing the challenges preparing a low-entropy single-atom qubit register. While ensemble approach inherits the single-atom quantum gate protocols, cooperative atom-light interaction makes it favorable platform to implement atom-photon interface, such as quantum memory. We have demonstrated semi-deterministic preparation of W-state, which we use as an ensemble qubit. Observed 50–60% preparation fidelity shows discrepancy to expected > 80% fidelity including known imperfections. We suspect Ground-Rydberg and Rydberg-Rydberg molecular interactions within the ensemble modify the dynamics. State tomography and Ramsey experiment clearly identified that majority of constituents in an ensemble are indeed entangled. We report the first measurement of W-state coherence time as 2.6ms for 7.6 atoms, which is long enough to perform 2600 Rydberg-mediated quantum gate operations. The first demonstration of Rydberg blockade between two ensembles happened in the same apparatus. We observe blockade fidelity of 0.89 (uncorrected) and near unity when post-selected on successful N = 1 Fock state preparation of Control ensemble. For weakly blockaded cases, Target ensemble remained as a perturber inhibiting Control ensemble from de-excitation. We discuss the efficacy of optical lattice insertion to suppress molecular interactions that might have been affecting the Rydberg dynamics. High fidelity, parallel, low loss fluorescence detection of hyperfine ground state of rubidium atoms is presented. Enforced cycling transition scattering minimally alters the internal states. We achieve mean state detection fidelity of 97% (uncorrected) and 98.7% (SPAM error corrected), with atom loss rate < 2% and hyperfine-changing rate < 2%. This scalable technique is also compatible with ensemble qubits and error correcting schemes. Technical developments on apparatus, lasers, supporting hardware and software are discussed. Automatic beam alignment system is implemented to correct long term drift of tightly focused addressing beams. Achieved pointing stability of 60 nm. Two home-made, high performing, cavity-enhanced frequency doubling systems were constructed to meet experimental demand. We observe 960/480 system output as high as 180 mW with 600 mW fundamental, and 1540/770 system output as high as 13.97 W from 19 W fundamental.

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Coherent control of addressable Rydberg atoms for hybrid quantum information processing

Craig Picken, Remy Legaie, Katie McDonnell +1 more

Neutral atoms provide an excellent resource for quantum information processing, combining the long atomic coherence times of the hyperfine ground-state with strong dipole-dipole interactions of highly excited Rydberg states for generating deterministic entanglement between qubits separated by < 10 µm [1]. Scalable long-range interactions can be obtained by coupling the atomic array to a superconducting microwave cavity enabling hybrid quantum information processing where the cavity-mediated entanglement allows atoms to be coupled over cm length scales. We present the first steps towards such an experiment incorporating high fidelity readout using an sCMOS camera [2] and the ability to drive fast, optically addressable rotations of the hyperfine-encoded qubits to the Rydberg state. Using our sub-kHz cavitystabilised laser system [3] we demonstrate coherent control of single Rydberg atoms, performing Ramsey spectroscopy to determine coherence time and to generate entanglement between a pair of atoms separated by 6 µm. Combining this excitation scheme with our ground-state Raman lasers we show progress towards the implementation of a mesoscopic Rydberg gate based on electromagnetically induced transparency (EIT) offering robust entanglement of multi-atom ensembles [4].

•Jul 25, 2018•0 citations

Rydberg Excitation of Single Atoms for Applications in Quantum Information and Metrology

Aaron M. Hankin

With the advent of laser cooling and trapping, neutral atoms have become a foundational source of accuracy for applications in metrology and are showing great potential for their use as qubits in quantum information. In metrology, neutral atoms provide the most accurate references for the measurement of time and acceleration. The unsurpassed stability provided by these systems make neutral atoms an attractive avenue to explore applications in quantum information and computing. However, to fully investigate the field of quantum information, we require a method to generate entangling interactions between neutral-atom qubits. Recent progress in the use of highly-excited Rydberg states for strong dipolar interactions has shown great promise for controlled entanglement using the Rydberg blockade phenomenon. I report the use of singly-trapped cesium atoms as qubits for applications in metrology and quantum information. Each atom provides a physical basis for a single qubit by encoding the required information into the ground-state hyperfine structure of cesium. Through the manipulation of these qubits with microwave and optical frequency sources, we demonstrate the capacity for arbitrary single-qubit control by driving qubit rotations in three orthogonal directions on the Bloch sphere. With this control, we develop an atom interferometer that far surpasses the force sensitivity of other approaches by applying the well-established technique of light-pulsed atom-matterwave interferometry to single atoms. Following this, we focus on two-qubit interactions using highly-excited Rydberg states. Through the development of a unique single-photon approach to Rydberg excitation using an ultraviolet laser at 319 nm, we observe the Rydberg blockade interaction between atoms separated by 6.6(3) microns. Motivated by the observation of Rydberg blockade, we study the application of Rydberg-dressed states for a quantum controlled-phase gate. Using a realistic simulation of the dressed-state dynamics, we calculate a controlled-phase gate fidelity of 94% that is primarily limited by Doppler frequency shifts. Finally, we employ our single-photon excitation laser to measure the Rydberg-dressed interaction, thus demonstrating the viability of this approach.

•Jan 28, 2015•2 citations

A Cavity-Coupled Rydberg Atom Array for Quantum Science and Quantum Computing

Beili Hu

Neutral atom arrays have rapidly emerged as a leading platform for quantum computing, boasting scalable, configurable arrays of single atoms trapped in optical tweezers, fast, high-fidelity entangling gates through Rydberg interactions, and programmable, parallelized control of qubit operations. Coupling an atom array to an optical cavity opens a new frontier. Leveraging enhanced light-atom interactions in cavity quantum electrodynamics, cavity- coupled atom arrays acquire capabilities that can further expand the neutral atom toolbox, including cavity-enhanced atom readouts, atom-photon entanglement, and photon-mediated interactions between distant atoms. This thesis presents a quantum hardware platform that integrates an array of neutral atoms with a high-finesse optical cavity. After describing the design and development of the experimental apparatus, I demonstrate high-fidelity atom state readout through the cavity, achieving improved speed and atom survival compared to conventional free-space imaging methods. I then introduce a new technique for selectively controlling atom-cavity coupling on arbitrary subsets of the array, using local AC Stark shifts on the excited states of the atoms. Building on these tools, I demonstrate fast, non-destructive cavity-based readout of atom arrays, a crucial bottleneck of atom array platforms. I also showcase real-time measurement and feedback capabilities with a demonstration of classical error correction, using a register of atomic bits. Finally, I describe progress toward implementing single- and two-qubit gates within the cavity-coupled system. By combining coherent control, tunable interactions, and high-fidelity, non-destructive readout integrated and real-time feedback, the cavity-coupled Rydberg atom array offers a promising path toward fault-tolerant quantum computing.

•May 1, 2025•0 citations

Fast Preparation and Detection of a Rydberg Qubit Using Atomic Ensembles

Wenchao Xu, Aditya V. Venkatramani, Sergio Cantu +4 more

We demonstrate a new approach for fast preparation, manipulation, and collective readout of an atomic Rydberg-state qubit. By making use of Rydberg blockade inside a small atomic ensemble, we prepare a single qubit within $3\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$ with a success probability of ${F}_{p}=0.93\ifmmode\pm\else\textpm\fi{}0.02$, rotate it, and read out its state in $6\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$ with a single-shot fidelity of ${F}_{d}=0.92\ifmmode\pm\else\textpm\fi{}0.04$. The ensemble-assisted detection is ${10}^{3}$ times faster than imaging of a single atom with the same optical resolution, and enables fast repeated nondestructive measurement. We observe qubit coherence times of $15\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$, much longer than the $\ensuremath{\pi}$ rotation time of 90 ns. Potential applications ranging from faster quantum information processing in atom arrays to efficient implementation of quantum error correction are discussed.

arXiv:2105.11050•Physical Review Letters•Jul 27, 2021•63 citations

Rydberg Atoms: A Collective Platform for Quantum Information Science

Y. Li

Quantum information is a rapidly developing field that merges the principles of quantum mechanics with information theory to explore new ways of processing and transmitting information. Qubits, which utilize superposition and entanglement, offer the potential for exponentially faster computation and secure communication methods that are fundamentally different from classical systems. This thesis contributes to the future of quantum information by studying two key platforms using neutral atoms: atomic arrays and atomic ensembles. It summarizes essential theoretical and experimental methods in the field and discusses key findings. To achieve entanglement among atomic qubits, Rydberg interactions are utilized, with two main effects discussed in this thesis. The Rydberg blockade effect is introduced where atoms trapped in an ensemble can form a two-level superatom. A state-insensitive optical lattice is used to achieve long coherence time for both the ground and Rydberg states. Long-lived Rabi oscillations and Ramsey interference are reported to demonstrate the collective enhancement of √N in a superatom. Furthermore, Rydberg dephasing is separated from Rydberg blockade and is investigated as a method to generate single photons from multiply excited states. This thesis presents both theoretical models and temporal evolution measurements of Rydberg dephasing from an initially unentangled Rydberg spinwave into an entangled single photon state. Additionally, this thesis examines the collective atomic dipole moment of a superatom, ⟨E⟩. Theoretical and experimental work are conducted to study the dipole moment when the phase-matched emission is combined with a coherent field in a homodyne detection method. This work advances our understanding of Rydberg interactions and collective dipole moments, contributing to the rapidly developing field of quantum information. The goal is to pave the way for the next era of quantum information through collaborative efforts and innovative research.

•Jan 1, 2024•0 citations

Single-qubit detection by collective phase imprinting

Kritsana Srakaew, Pascal Weckesser, Daniel Adler +4 more

The amplification of quantum information carried by a single quantum excitation is a recurring challenge across diverse quantum platforms. The coupling between a single qubit and a mesoscopic ensemble of spins, for example, can be leveraged to realize non-destructive detection of the qubit state. However, realizing robust couplings between such systems is experimentally challenging and typically requires programmable quantum gates or native long-range interactions. Here, we introduce a platform that couples a single qubit, encoded in the ground-to-Rydberg transition of a control atom, to a Rydberg-dressed target ensemble of ground-state atoms trapped in an optical lattice. We show that the state of the control qubit can be coherently mapped onto the ensemble via a qubit-controlled collective phase shift. By Rydberg-dressing the ensemble, the controlled phase shift per target atom becomes independent of the number of target atoms, making the protocol intrinsically insensitive to atom-number fluctuations and atom loss, which are the dominant experimental imperfections in our system. Exploiting the collective response of up to eight target spins, we demonstrate the efficacy of the scheme by realizing non-destructive detection of a single Rydberg excitation with a state-assignment fidelity of $\mathcal{F} = 99.81^{+0.17}_{-1.47}\,\%$. Our approach demonstrates the key ingredients for high-fidelity transfer of quantum information from a single qubit to a mesoscopic ensemble, opening a route to non-destructive mid-circuit readout of Rydberg states and to efficient interfaces between single qubits and photonic modes.

quant-pharXiv:2608.06970•Aug 10, 2026•0 citations
This thesis reports progress towards using hyperfine-encoded neutral atomic ensembles for quantum information applications. Ensemble qubits are alternative building blocks to process quantum information, while circumventing the challenges preparing a low-entropy single-atom qubit register. While ensemble approach inherits the single-atom quantum gate protocols, cooperative atom-light interaction makes it favorable platform to implement atom-photon interface, such as quantum memory. We have demonstrated semi-deterministic preparation of W-state, which we use as an ensemble qubit. Observed 50–60% preparation fidelity shows discrepancy to expected > 80% fidelity including known imperfections. We suspect Ground-Rydberg and Rydberg-Rydberg molecular interactions within the ensemble modify the dynamics. State tomography and Ramsey experiment clearly identified that majority of constituents in an ensemble are indeed entangled. We report the first measurement of W-state coherence time as 2.6ms for 7.6 atoms, which is long enough to perform 2600 Rydberg-mediated quantum gate operations. The first demonstration of Rydberg blockade between two ensembles happened in the same apparatus. We observe blockade fidelity of 0.89 (uncorrected) and near unity when post-selected on successful N = 1 Fock state preparation of Control ensemble. For weakly blockaded cases, Target ensemble remained as a perturber inhibiting Control ensemble from de-excitation. We discuss the efficacy of optical lattice insertion to suppress molecular interactions that might have been affecting the Rydberg dynamics. High fidelity, parallel, low loss fluorescence detection of hyperfine ground state of rubidium atoms is presented. Enforced cycling transition scattering minimally alters the internal states. We achieve mean state detection fidelity of 97% (uncorrected) and 98.7% (SPAM error corrected), with atom loss rate < 2% and hyperfine-changing rate < 2%. This scalable technique is also compatible with ensemble qubits and error correcting schemes. Technical developments on apparatus, lasers, supporting hardware and software are discussed. Automatic beam alignment system is implemented to correct long term drift of tightly focused addressing beams. Achieved pointing stability of 60 nm. Two home-made, high performing, cavity-enhanced frequency doubling systems were constructed to meet experimental demand. We observe 960/480 system output as high as 180 mW with 600 mW fundamental, and 1540/770 system output as high as 13.97 W from 19 W fundamental.
Neutral atoms provide an excellent resource for quantum information processing, combining the long atomic coherence times of the hyperfine ground-state with strong dipole-dipole interactions of highly excited Rydberg states for generating deterministic entanglement between qubits separated by < 10 µm [1]. Scalable long-range interactions can be obtained by coupling the atomic array to a superconducting microwave cavity enabling hybrid quantum information processing where the cavity-mediated entanglement allows atoms to be coupled over cm length scales. We present the first steps towards such an experiment incorporating high fidelity readout using an sCMOS camera [2] and the ability to drive fast, optically addressable rotations of the hyperfine-encoded qubits to the Rydberg state. Using our sub-kHz cavitystabilised laser system [3] we demonstrate coherent control of single Rydberg atoms, performing Ramsey spectroscopy to determine coherence time and to generate entanglement between a pair of atoms separated by 6 µm. Combining this excitation scheme with our ground-state Raman lasers we show progress towards the implementation of a mesoscopic Rydberg gate based on electromagnetically induced transparency (EIT) offering robust entanglement of multi-atom ensembles [4].
With the advent of laser cooling and trapping, neutral atoms have become a foundational source of accuracy for applications in metrology and are showing great potential for their use as qubits in quantum information. In metrology, neutral atoms provide the most accurate references for the measurement of time and acceleration. The unsurpassed stability provided by these systems make neutral atoms an attractive avenue to explore applications in quantum information and computing. However, to fully investigate the field of quantum information, we require a method to generate entangling interactions between neutral-atom qubits. Recent progress in the use of highly-excited Rydberg states for strong dipolar interactions has shown great promise for controlled entanglement using the Rydberg blockade phenomenon. I report the use of singly-trapped cesium atoms as qubits for applications in metrology and quantum information. Each atom provides a physical basis for a single qubit by encoding the required information into the ground-state hyperfine structure of cesium. Through the manipulation of these qubits with microwave and optical frequency sources, we demonstrate the capacity for arbitrary single-qubit control by driving qubit rotations in three orthogonal directions on the Bloch sphere. With this control, we develop an atom interferometer that far surpasses the force sensitivity of other approaches by applying the well-established technique of light-pulsed atom-matterwave interferometry to single atoms. Following this, we focus on two-qubit interactions using highly-excited Rydberg states. Through the development of a unique single-photon approach to Rydberg excitation using an ultraviolet laser at 319 nm, we observe the Rydberg blockade interaction between atoms separated by 6.6(3) microns. Motivated by the observation of Rydberg blockade, we study the application of Rydberg-dressed states for a quantum controlled-phase gate. Using a realistic simulation of the dressed-state dynamics, we calculate a controlled-phase gate fidelity of 94% that is primarily limited by Doppler frequency shifts. Finally, we employ our single-photon excitation laser to measure the Rydberg-dressed interaction, thus demonstrating the viability of this approach.
Neutral atom arrays have rapidly emerged as a leading platform for quantum computing, boasting scalable, configurable arrays of single atoms trapped in optical tweezers, fast, high-fidelity entangling gates through Rydberg interactions, and programmable, parallelized control of qubit operations. Coupling an atom array to an optical cavity opens a new frontier. Leveraging enhanced light-atom interactions in cavity quantum electrodynamics, cavity- coupled atom arrays acquire capabilities that can further expand the neutral atom toolbox, including cavity-enhanced atom readouts, atom-photon entanglement, and photon-mediated interactions between distant atoms. This thesis presents a quantum hardware platform that integrates an array of neutral atoms with a high-finesse optical cavity. After describing the design and development of the experimental apparatus, I demonstrate high-fidelity atom state readout through the cavity, achieving improved speed and atom survival compared to conventional free-space imaging methods. I then introduce a new technique for selectively controlling atom-cavity coupling on arbitrary subsets of the array, using local AC Stark shifts on the excited states of the atoms. Building on these tools, I demonstrate fast, non-destructive cavity-based readout of atom arrays, a crucial bottleneck of atom array platforms. I also showcase real-time measurement and feedback capabilities with a demonstration of classical error correction, using a register of atomic bits. Finally, I describe progress toward implementing single- and two-qubit gates within the cavity-coupled system. By combining coherent control, tunable interactions, and high-fidelity, non-destructive readout integrated and real-time feedback, the cavity-coupled Rydberg atom array offers a promising path toward fault-tolerant quantum computing.
We demonstrate a new approach for fast preparation, manipulation, and collective readout of an atomic Rydberg-state qubit. By making use of Rydberg blockade inside a small atomic ensemble, we prepare a single qubit within $3\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$ with a success probability of ${F}_{p}=0.93\ifmmode\pm\else\textpm\fi{}0.02$, rotate it, and read out its state in $6\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$ with a single-shot fidelity of ${F}_{d}=0.92\ifmmode\pm\else\textpm\fi{}0.04$. The ensemble-assisted detection is 103{10}^{3}103 times faster than imaging of a single atom with the same optical resolution, and enables fast repeated nondestructive measurement. We observe qubit coherence times of $15\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$, much longer than the $\ensuremath{\pi}$ rotation time of 90 ns. Potential applications ranging from faster quantum information processing in atom arrays to efficient implementation of quantum error correction are discussed.
Quantum information is a rapidly developing field that merges the principles of quantum mechanics with information theory to explore new ways of processing and transmitting information. Qubits, which utilize superposition and entanglement, offer the potential for exponentially faster computation and secure communication methods that are fundamentally different from classical systems. This thesis contributes to the future of quantum information by studying two key platforms using neutral atoms: atomic arrays and atomic ensembles. It summarizes essential theoretical and experimental methods in the field and discusses key findings. To achieve entanglement among atomic qubits, Rydberg interactions are utilized, with two main effects discussed in this thesis. The Rydberg blockade effect is introduced where atoms trapped in an ensemble can form a two-level superatom. A state-insensitive optical lattice is used to achieve long coherence time for both the ground and Rydberg states. Long-lived Rabi oscillations and Ramsey interference are reported to demonstrate the collective enhancement of √N in a superatom. Furthermore, Rydberg dephasing is separated from Rydberg blockade and is investigated as a method to generate single photons from multiply excited states. This thesis presents both theoretical models and temporal evolution measurements of Rydberg dephasing from an initially unentangled Rydberg spinwave into an entangled single photon state. Additionally, this thesis examines the collective atomic dipole moment of a superatom, ⟨E⟩. Theoretical and experimental work are conducted to study the dipole moment when the phase-matched emission is combined with a coherent field in a homodyne detection method. This work advances our understanding of Rydberg interactions and collective dipole moments, contributing to the rapidly developing field of quantum information. The goal is to pave the way for the next era of quantum information through collaborative efforts and innovative research.
The amplification of quantum information carried by a single quantum excitation is a recurring challenge across diverse quantum platforms. The coupling between a single qubit and a mesoscopic ensemble of spins, for example, can be leveraged to realize non-destructive detection of the qubit state. However, realizing robust couplings between such systems is experimentally challenging and typically requires programmable quantum gates or native long-range interactions. Here, we introduce a platform that couples a single qubit, encoded in the ground-to-Rydberg transition of a control atom, to a Rydberg-dressed target ensemble of ground-state atoms trapped in an optical lattice. We show that the state of the control qubit can be coherently mapped onto the ensemble via a qubit-controlled collective phase shift. By Rydberg-dressing the ensemble, the controlled phase shift per target atom becomes independent of the number of target atoms, making the protocol intrinsically insensitive to atom-number fluctuations and atom loss, which are the dominant experimental imperfections in our system. Exploiting the collective response of up to eight target spins, we demonstrate the efficacy of the scheme by realizing non-destructive detection of a single Rydberg excitation with a state-assignment fidelity of F=99.81−1.47+0.17 %\mathcal{F} = 99.81^{+0.17}_{-1.47}\,\%F=99.81−1.47+0.17​%. Our approach demonstrates the key ingredients for high-fidelity transfer of quantum information from a single qubit to a mesoscopic ensemble, opening a route to non-destructive mid-circuit readout of Rydberg states and to efficient interfaces between single qubits and photonic modes.