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arXiv:1404.0374 · Review of Scientific Instruments

An optically modulated zero-field atomic magnetometer with suppressed spin-exchange broadening

Ricardo Jiménez-Martínez, Svenja A. Knappe, John E. Kitching

Published Apr 1, 2014• 51 citations
arXivHTMLPDF

Abstract

We demonstrate an optically pumped (87)Rb magnetometer in a microfabricated vapor cell based on a zero-field dispersive resonance generated by optical modulation of the (87)Rb ground state energy levels. The magnetometer is operated in the spin-exchange relaxation-free regime where high magnetic field sensitivities can be achieved. This device can be useful in applications requiring array-based magnetometers where radio frequency magnetic fields can induce cross-talk among adjacent sensors or affect the source of the magnetic field being measured.

DOI
10.1063/1.4872075

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Advanced Sensor Systems and Applications•Oct 11, 2024•0 citations
We demonstrate an optically pumped (87)Rb magnetometer in a microfabricated vapor cell based on a zero-field dispersive resonance generated by optical modulation of the (87)Rb ground state energy levels. The magnetometer is operated in the spin-exchange relaxation-free regime where high magnetic field sensitivities can be achieved. This device can be useful in applications requiring array-based magnetometers where radio frequency magnetic fields can induce cross-talk among adjacent sensors or affect the source of the magnetic field being measured.
Spin-exchange relaxation free alkali-metal magnetometers typically operate in the regime of high optical density, presenting challenges for simple and efficient optical pumping and detection. We describe a high-sensitivity Rb magnetometer using a single elliptically polarized off-resonant laser beam. Circular component of the light creates relatively uniform spin polarization while the linear component is used to measure optical rotation generated by the atoms. Modulation of the atomic spin direction with an oscillating magnetic field shifts the detected signal to high frequencies. Using a fiber-coupled distributed feedback laser, we achieve magnetic field sensitivity of 7 fT/Hz7\text{ }\text{fT}/\sqrt{\text{Hz}}7 fT/Hz​ with a miniature $5\ifmmode\times\else\texttimes\fi{}5\ifmmode\times\else\texttimes\fi{}5\text{ }\text{mm}\text{ }\text{Rb}$ vapor cell.
We report on the development of a microfabricated atomic magnetic gradiometer based on optical spectroscopy of alkali atoms in the vapor phase. The gradiometer, which operates in the spin-exchange relaxation free regime, has a length of 60 mm and cross sectional diameter of 12 mm, and consists of two chip-scale atomic magnetometers which are interrogated by a common laser light. The sensor can measure differences in magnetic fields, over a 20 mm baseline, of 10 fT/[Formula: see text] at frequencies above 20 Hz. The maximum rejection of magnetic field noise is 1000 at 10 Hz. By use of a set of compensation coils wrapped around the sensor, we also measure the sensor sensitivity at several external bias field strengths up to 150 mG. This device is useful for applications that require both sensitive gradient field information and high common-mode noise cancellation.
In recent years, arrayed atomic magnetometers have been continuously applied in biomagnetic scenarios. However, the crosstalk between adjacent sensors introduced by the modulated magnetic fields significantly compromises the imaging accuracy of arrayed atomic magnetometers. To solve this problem, a detuned square-wave optical modulation zero-field atomic magnetometer configuration is developed and we provide an analytical solution of this method. In this scheme, the circularly polarized pump light is used to polarize alkali metal atoms longitudinally, and a beam of detuned square-wave modulated circularly polarized light is applied transversely to generate a light-shift modulation instead of the coil-generated modulated magnetic field. Then the transverse magnetic field is measured by the optical absorption method of longitudinally circularly polarized pump light. This scheme maintains the inherent advantage of high sensitivity in spinexchange relaxation-free (SERF) atomic magnetometers. Additionally, the all-optical configuration eliminates the need for additional modulated magnetic fields or radio frequency (RF) fields, thereby mitigating crosstalk issues associated with modulated magnetic fields in array applications. Consequently, this scheme exhibits great potential for arraying and is expected to be employed in magnetocardiography (MCG) and magnetoencephalography (MEG).
Spin polarized atomic magnetometers involve the preparation of atomic spins and their detection for monitoring magnetic fields. Due to the fact that magnetic fields are ubiquitous in our world, spin polarized atomic magnetometers are used in a wide range of applications from the detection of magnetic fields generated by the human heart and brain to the detection of nuclear magnetic resonance. In this thesis we developed microfabricated spin polarized atomic magnetometers. These sensors are based on optical pumping and spin-exchange collisions between alkali atoms and noble gases contained in microfabricated millimeter-scale vapor cells. In the first part of the thesis, we improved different features of current microfabricated optical magnetometers. Specifically, we improved the bandwidth of these devices, without degrading their magnetic field sensitivity, by broadening their magnetic resonance through spin-exchange collisions between alkali atoms. We also implemented all-optical excitation techniques to avoid problems, such as the magnetic perturbation of the environment, induced by the radio-frequency fields used in some of these sensors. In the second part of the thesis we demonstrated a microfluidic chip for the optical production and detection of hyperpolarized Xe gas through spin-exchange collisions with optically pumped Rb atoms. These devices are critical for the widespread use of spin polarized atomic magnetometers in applications requiring simple, compact, low-cost, and portable instrumentation.
Abstract We present a design for a multi-channel optically pumped zero-field magnetometer utilizing a 200-μm-thick Rubidium vapor cell. The vapor cell and its housing are designed to reduce the minimal distance between a magnetic sample and the sensing volume to about 1 mm, to optimize the effective spatial resolution. The thin vapor cell, filled with 2 atm of nitrogen as a buffer gas reduces the volume across which the magnetic field is averaged. The vapor cell is fully illuminated by a single laser beam, and the transmitted light is imaged onto a 4 x 4 photodiode array, allowing for simultaneous measurement of a magnetic field distribution with up to 16 channels. The performance of the magnetometer is studied for all channels. It is shown that the sensor can operate in the spin-exchange relaxation-free regime with a projected photon-shot noise limited noise floor of about 1 pT/Hz1/2 for a sensitive voxel size of approximately 600 μm x 600 μm x 200 μm.
Atomic magnetometers with magnetic field modulation have emerged as pivotal sensors for biomagnetic measurements. However, challenges such as crosstalk between adjacent modulation fields and the complexity of signal circuitry become increasingly serious in the development of array-based equipment with the magnetometers, especially in the miniaturized atomic magnetometer. This paper proposes an all-optical, fully integrated fiber-coupled atomic magnetometer that employs pump beam modulation. A miniaturized atomic magnetometer with a volume of 10 cm³ has been designed, incorporating an active measurement area of 3 × 3 × 3 mm3. The magnetometer operates in the spinexchange relaxation-free (SERF) regime with an 87Rb vapor cell. An amplitude-modulated pump beam directly modulates the rubidium atomic ensembles, rather than the magnetic field modulation. The optical rotation angle is detected by an unmodulated probe beam oriented orthogonally to the pump beam. In light of the discontinuous pumping characteristics, we developed a modified theoretical model to clarify the output response of the proposed atomic magnetometer. The experimental results demonstrate that the new design achieves the same sensitivity as conventional magnetometer configurations with a smaller volume and without crosstalk of the magnetic field. This research highlights the significant potential for advancing the development of highly sensitive, miniaturized atomic magnetometers, making them particularly suitable for applications in magnetocardiography (MCG) and magnetoencephalography (MEG).