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Advanced Sensor Systems and Applications

Miniaturized atomic magnetometer employing pump-beam modulation

Ziqian Yue, Junjian Tang, Yueyang Zhai

Published Oct 11, 2024• 0 citations
Publisher

Abstract

Atomic magnetometers with magnetic field modulation have emerged as pivotal sensors for biomagnetic measurements. However, challenges such as crosstalk between adjacent modulation fields and the complexity of signal circuitry become increasingly serious in the development of array-based equipment with the magnetometers, especially in the miniaturized atomic magnetometer. This paper proposes an all-optical, fully integrated fiber-coupled atomic magnetometer that employs pump beam modulation. A miniaturized atomic magnetometer with a volume of 10 cm³ has been designed, incorporating an active measurement area of 3 × 3 × 3 mm3. The magnetometer operates in the spinexchange relaxation-free (SERF) regime with an 87Rb vapor cell. An amplitude-modulated pump beam directly modulates the rubidium atomic ensembles, rather than the magnetic field modulation. The optical rotation angle is detected by an unmodulated probe beam oriented orthogonally to the pump beam. In light of the discontinuous pumping characteristics, we developed a modified theoretical model to clarify the output response of the proposed atomic magnetometer. The experimental results demonstrate that the new design achieves the same sensitivity as conventional magnetometer configurations with a smaller volume and without crosstalk of the magnetic field. This research highlights the significant potential for advancing the development of highly sensitive, miniaturized atomic magnetometers, making them particularly suitable for applications in magnetocardiography (MCG) and magnetoencephalography (MEG).

DOI
10.1117/12.3035399

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Atomic magnetometers with magnetic field modulation have emerged as pivotal sensors for biomagnetic measurements. However, challenges such as crosstalk between adjacent modulation fields and the complexity of signal circuitry become increasingly serious in the development of array-based equipment with the magnetometers, especially in the miniaturized atomic magnetometer. This paper proposes an all-optical, fully integrated fiber-coupled atomic magnetometer that employs pump beam modulation. A miniaturized atomic magnetometer with a volume of 10 cm³ has been designed, incorporating an active measurement area of 3 × 3 × 3 mm3. The magnetometer operates in the spinexchange relaxation-free (SERF) regime with an 87Rb vapor cell. An amplitude-modulated pump beam directly modulates the rubidium atomic ensembles, rather than the magnetic field modulation. The optical rotation angle is detected by an unmodulated probe beam oriented orthogonally to the pump beam. In light of the discontinuous pumping characteristics, we developed a modified theoretical model to clarify the output response of the proposed atomic magnetometer. The experimental results demonstrate that the new design achieves the same sensitivity as conventional magnetometer configurations with a smaller volume and without crosstalk of the magnetic field. This research highlights the significant potential for advancing the development of highly sensitive, miniaturized atomic magnetometers, making them particularly suitable for applications in magnetocardiography (MCG) and magnetoencephalography (MEG).
Abstract The chip-scale hybrid optical pumping spin-exchange relaxation-free (SERF) atomic magnetometer with a single-beam arrangement has prominent applications in biomagnetic measurements because of its outstanding features, including ultrahigh sensitivity, an enhanced signal-to-noise ratio, homogeneous spin polarization and a much simpler optical configuration than other devices. In this work, a miniaturized single-beam hybrid optical pumping SERF atomic magnetometer based on a microfabricated atomic vapor cell is demonstrated. Although the optically thin Cs atoms are spin-polarized, the dense Rb atoms determine the experimental results. The enhanced signal strength and narrowed resonance linewidth are experimentally proven, which shows the superiority of the proposed magnetometer scheme. By using a differential detection scheme, we effectively suppress optical noise with an approximate five-fold improvement. Moreover, the cell temperature markedly affects the performance of the magnetometer. We systematically investigate the effects of temperature on the magnetometer parameters. The theoretical basis for these effects is explained in detail. The developed miniaturized magnetometer has an optimal magnetic sensitivity of 20 fT/Hz 1/2 . The presented work provides a foundation for the chip-scale integration of ultrahighly sensitive quantum magnetometers that can be used for forward-looking magnetocardiography (MCG) and magnetoencephalography (MEG) applications.
In recent years, arrayed atomic magnetometers have been continuously applied in biomagnetic scenarios. However, the crosstalk between adjacent sensors introduced by the modulated magnetic fields significantly compromises the imaging accuracy of arrayed atomic magnetometers. To solve this problem, a detuned square-wave optical modulation zero-field atomic magnetometer configuration is developed and we provide an analytical solution of this method. In this scheme, the circularly polarized pump light is used to polarize alkali metal atoms longitudinally, and a beam of detuned square-wave modulated circularly polarized light is applied transversely to generate a light-shift modulation instead of the coil-generated modulated magnetic field. Then the transverse magnetic field is measured by the optical absorption method of longitudinally circularly polarized pump light. This scheme maintains the inherent advantage of high sensitivity in spinexchange relaxation-free (SERF) atomic magnetometers. Additionally, the all-optical configuration eliminates the need for additional modulated magnetic fields or radio frequency (RF) fields, thereby mitigating crosstalk issues associated with modulated magnetic fields in array applications. Consequently, this scheme exhibits great potential for arraying and is expected to be employed in magnetocardiography (MCG) and magnetoencephalography (MEG).
A self-oscillating magnetometer based on nonlinear magneto-optical rotation using amplitude-modulated pump light and unmodulated probe light (AM-NMOR) in 87Rb has been constructed and tested towards a goal of airborne detection of magnetic anomalies. In AM-NMOR, stroboscopic optical pumping via amplitude modulation of the pump beam creates alignment of the ground electronic state of the rubidium atoms. The Larmor precession causes an ac rotation of the polarization of a separate probe beam; the polarization rotation frequency provides a measure of the magnetic field. An anti-relaxation coating on the walls of the atomic vapor cell results in a long lifetime of 56 ms for the alignment, which enables precise measurement of the precession frequency. Light is delivered to the magnetometer by polarization-maintaining optical fibers. Tests of the sensitivity include directly measuring the beat frequency between the magnetometer and a commercial instrument and measurements of Earth's field under magnetically quiet conditions, indicating a sensitivity of at least 5 pT/νHz. Rotating the sensor indicates a heading error of less than 1 nT, limited in part by residual magnetism of the sensor.
Functional imaging equipment based on miniaturized atomic magnetometers with array arrangement exhibits promising prospects in biomagnetic scenarios. However, crosstalk from the modulated magnetic field between adjacent sensors degrades the imaging accuracy. To address this issue, this study proposes an all-optical dual-axis zero-field atomic magnetometer using light-shift modulation. We utilize an acousto-optic modulator to modulate a detuned circularly polarized beam for pumping the atomic spin ensembles. This beam allows for the optical modulation of spin polarization and meanwhile generates a light-shift modulation, effectively replacing the conventional magnetic field modulation. By using a probe beam to detect the optical rotation angle perpendicular to the direction of the pump beam, we construct an all-optical configuration of a longitudinally modulated atomic magnetometer, enabling dual-axis magnetic field measurements. Experimental results demonstrate dual-axis sensitivities of 29 and 15fT/Hz1/2, respectively. This method eliminates the need for conventional coil-based magnetic field modulation, thereby paving the way for potential applications in magnetocardiography and magnetoencephalography.Received 3 August 2023Revised 13 November 2023Accepted 4 December 2023DOI:https://doi.org/10.1103/PhysRevApplied.21.014023© 2024 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasMagneto-optical effectMagnetometryOptical pumpingStark effectPhysical SystemsAlkali metalsAtomic gasesTechniquesOptically detected magnetic resonancePrecision measurementsAtomic, Molecular & OpticalCondensed Matter, Materials & Applied Physics
Abstract High-sensitivity triaxial magnetic field measurements are crucial in various scientific and industrial applications, with spin-exchange relaxation-free (SERF) atomic magnetometers (AMs) standing out for their exceptional sensitivity. However, conventional methods for achieving triaxial measurements in SERF magnetometers typically involve multiple modulated magnetic fields, which introduce crosstalk challenges in array-based configurations. We propose a static bias magnetic field assisted optical modulation triaxial AM to address this limitation. In this configuration, the detuned circularly polarized light is utilized to achieve synchronous modulation of the fictitious magnetic field and pumping rate while incorporating a static bias magnetic field to generate a transverse projection component. We develop a comprehensive triaxial response model that fully considers the effects of the longitudinal spin polarization deflection. Building upon this model, we derive the relationship between the transverse spin component and the triaxial magnetic field and introduce parameter optimization methods to obtain optimal parameters, thus enabling triaxial measurements of 12 fT Hz −1/2 , 10 fT Hz −1/2 , and 15 fT Hz −1/2 along the x-, y -, and z -axes. Our approach offers significant advantages over existing methods, particularly in minimizing crosstalk and mitigating spin-exchange relaxation introduced by multiple modulated magnetic fields. Moreover, the effective detection of simulated magnetocardiography signals highlights the practical applicability and reliability of the proposed method in real-world scenarios.
Emerging quantum sensing devices namely atomic magnetometers have become promising candidate for future biomagnetism imaging. However, the limitation of detection bandwidth exists a major drawback for devices of this kind. Conventional approaches, including transverse magnetic field modulation and close-loop control, have seen challenging tradeoffs between size, resolution and bandwidths. In this study, a wide bandwidth zero-field magnetometer with a miniaturized light source has been developed for alternating current (AC) magnetic field detection. A dual-beam Spin-Exchange Relaxation-Free (SERF) magnetometer employing a 4×4×4mm3 alkali metal vapor cell achieves a bandwidth of 188 Hz. This represents a threefold increase in bandwidth compared to non-modulated mode. The sensitivity under modulated mode demonstrated a sensitivity of 55fT/Hz1/2within the frequency range of 10-188Hz. Our results also demonstrated that the sensitivity is constrained by relaxation induced by the modulation of pumping source, so possible tradeoffs can be made based on various applications. The proposed method provides novel approach for bandwidth extension of atomic magnetometers which further pave the way for future applications including magnetoencephalography (MEG), particularly in reducing magnetic noise crosstalk and enhancing spatial resolution.