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arXiv:1309.5915 · Physical Review A

Quantum input-output theory for optical cavities with arbitrary coupling strength: Application to two-photon wave-packet shaping

Michael G. Raymer, Colin J. McKinstrie

Published Oct 11, 2013• 29 citations
arXivHTMLPDF

Abstract

We develop quantum-optical input-output theory for resonators with arbitrary coupling strength, and for input fields whose spectrum can be wider than the cavity free-spectral range, while ensuring that the field-operator commutator relations in space-time variables are correct. The cavity-field commutator exhibits a series of space-time ``echoes,'' representing causal connections of certain space-time points by light propagation. We apply the theory to two-photon wave-packet shaping by cavity reflection, which displays a remarkable illustration of dispersion cancellation. We also show that the theory is amenable to inclusion of intracavity absorbing and emitting atoms, allowing, for example, dissipative losses within the cavity to be incorporated in a quantum mechanically correct way.

DOI
10.1103/physreva.88.043819

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•Jan 1, 2006•0 citations
We develop quantum-optical input-output theory for resonators with arbitrary coupling strength, and for input fields whose spectrum can be wider than the cavity free-spectral range, while ensuring that the field-operator commutator relations in space-time variables are correct. The cavity-field commutator exhibits a series of space-time ``echoes,'' representing causal connections of certain space-time points by light propagation. We apply the theory to two-photon wave-packet shaping by cavity reflection, which displays a remarkable illustration of dispersion cancellation. We also show that the theory is amenable to inclusion of intracavity absorbing and emitting atoms, allowing, for example, dissipative losses within the cavity to be incorporated in a quantum mechanically correct way.
We study theoretically the interaction between two photons in a nonlinear cavity. The photons are absorbed into the cavity by an effective tuning of its input-output coupling via external control of a coupling to a second, strongly output-coupled cavity mode. Such ``dynamically coupled'' cavities, which can be implemented using bulk ${\ensuremath{\chi}}^{(2)}$ and ${\ensuremath{\chi}}^{(3)}$ nonlinearities, enable incoming photon wave packets to be absorbed into the cavity with high fidelity when the duration of the control is similar to that of the wave packets. Further, this configuration can be used to avoid limitations in the photon-photon interaction time set by the delay-bandwidth product of passive cavities and enables the elimination of wave-packet distortions caused by dispersive cavity transmission and reflection. We consider three kinds of nonlinearities, two arising from ${\ensuremath{\chi}}^{(2)}$ and ${\ensuremath{\chi}}^{(3)}$ materials and one due to an interaction with a two-level emitter. To analyze the input and output of few-photon wave packets, we use a Schr\"odinger-picture formalism in which traveling-wave fields are discretized into infinitesimal time bins. We suggest that dynamically coupled cavities provide a very useful tool for improving the performance of quantum devices relying on cavity-enhanced light-matter interactions such as single-photon sources and atomlike quantum memories with photon interfaces. As an example, we present simulation results showing that high-fidelity two-qubit entangling gates may be constructed using any of the considered nonlinear interactions.
Being able to reliably transfer the quantum state from one system to another is crucial to developing quantum networks. A standard way to accomplish this transfer of information is by making use of an intermediate information carrier (e.g., a photon) that is emitted by the first system and absorbed by the second. For such a scenario one can develop an effective description by eliminating the intermediate degrees of freedom, which yields an effective direct coupling between the two systems. If, however, the spectral properties of the two systems are different, the photon's time-frequency shape needs to be appropriately modified before it reaches the second system. We study here the effective description that results when we thus manipulate the intermediate photon. We examine a unitary transformation UUU that time reverses, frequency translates, and stretches the photon wave packet. We find that the concomitant modifications to the effective description can best be understood in terms of a change to the state's time argument $\ensuremath{\rho}(t)={\ensuremath{\rho}}_{1}(\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{t})\ensuremath{\bigotimes}{\ensuremath{\rho}}_{2}(t)$, where $\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{t}$ is a fictitious time for the first system that is stretched and runs backward. We apply this theory to three-level $\mathrm{\ensuremath{\Lambda}}$ systems inside optical cavities, and we numerically illustrate how performing the unitary transformation UUU results in improved quantum state transfer.
The purpose of this paper is to compare two unitary, deterministic approaches to the study of the interaction of quantized fields with atomic systems in optical cavities. In particular it is shown that the ``modes of the universe'' approach, in which each mode has both an intracavity and an outside part, is formally equivalent, in an appropriate limit, to the better known ``input-output'' formalism in its unitary (i.e., Hermitian-Hamiltonian based) form; the latter may be called a ``quasimode'' theory, since it treats the field inside the cavity as a separate degree of freedom. Differences that arise between the two approaches for numerical calculations involving a finite set of discrete modes are also pointed out. The formalism is illustrated with an in-depth discussion of the explicit solution for a single-photon pulse, of arbitrary shape and detuning, incident on a cavity containing a two-level atom.
Within the framework of exact quantization of the electromagnetic field in dispersing and absorbing media the input-output problem of a high-QQQ cavity is studied, with special emphasis on the absorption losses in the coupling mirror. As expected, the cavity modes are found to obey quantum Langevin equations, which could be also obtained from quantum noise theories, by appropriately coupling the cavity modes to dissipative systems, including the effect of the mirror-assisted absorption losses. On the contrary, the operator input-output relations obtained in this way would be incomplete in general, as the exact calculation shows. On the basis of the operator input-output relations the problem of extracting the quantum state of an initially excited cavity mode is studied and input-output relations for the sss-parametrized phase-space function are derived, with special emphasis on the relation between the Wigner functions of the quantum states of the outgoing field and the cavity field.
We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultrastrong light-matter coupling regime, in which the vacuum Rabi frequency is a significant fraction of the active electronic transition frequency and the antiresonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. In the case of a time-independent vacuum Rabi frequency, exact analytical expressions for the operators are obtained, which allows us to characterize the quantum dissipative response of the cavity to an arbitrary initial condition (vacuum, coherent field, thermal excitation). For a vacuum input in both the photonic and electronic polarization modes, the ground state of the cavity system is a two-mode squeezed vacuum state with a finite population in both photonic and electronic modes. These excitations are, however, virtual and cannot escape from the cavity: for a vacuum input, a vacuum output is found, without any trace of the intracavity squeezing. For a coherent photonic input the linear optical response spectra (reflectivity, absorption, transmission) have been studied, and signatures of the ultrastrong coupling have been identified in the asymmetric and peculiar anticrossing of the polaritonic eigenmodes. Finally, we have calculated the electroluminescence spectra in the case of an incoherent electronic input: the emission intensity in the ultrastrong coupling regime results in being significantly enhanced as compared to the case of an isolated quantum well without a surrounding cavity.
We present a full quantum theory for the dissipative dynamics of an optical cavity in the ultra-strong light-matter coupling regime, in which the vacuum Rabi frequency is comparable to the electronic transition frequency and the anti-resonant terms of the light-matter coupling play an important role. In particular, our model can be applied to the case of intersubband transitions in doped semiconductor quantum wells embedded in a microcavity. The coupling of the intracavity photonic mode and of the electronic polarization to the external, frequency-dependent, dissipation baths is taken into account by means of quantum Langevin equations in the input-output formalism. Observable spectra (reflection, absorption, transmission and electroluminescence) are calculated analytically in the case of a time-independent vacuum Rabi frequency.