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arXiv:1306.2205 · Physical Review A

Observation of Rb two-photon absorption directly excited by an erbium-fiber-laser-based optical frequency comb via spectral control

Jiutao Wu, Dong Hou, Zhengyu Qin, Zhigang Zhang, Jianye Zhao

Published Apr 14, 2014• 10 citations

Abstract

We present the observation of the Rb two-photon spectrum directly excited by an Er:fiber laser comb in a hot atomic vapor system. The influences of the atomic velocity distribution on direct and sequential two-photon transitions are discussed respectively and a combination of corresponding spectral control techniques is developed to eliminate the Doppler broadening background. A direct frequency comb spectroscopy is obtained with high-resolution two-photon transition lines. These techniques would benefit spectroscopy measurement in hot atomic vapor systems, and pave the way for establishing a high-stability optical frequency comb in 1.5 $\ensuremath{\mu}$m optical communication bands based on the Rb two-photon transitions.

DOI: 10.1103/physreva.89.041402

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arXiv:1706.03237•Physical Review A•Aug 31, 2017•3 citations

We present the observation of the Rb two-photon spectrum directly excited by an Er:fiber laser comb in a hot atomic vapor system. The influences of the atomic velocity distribution on direct and sequential two-photon transitions are discussed respectively and a combination of corresponding spectral control techniques is developed to eliminate the Doppler broadening background. A direct frequency comb spectroscopy is obtained with high-resolution two-photon transition lines. These techniques would benefit spectroscopy measurement in hot atomic vapor systems, and pave the way for establishing a high-stability optical frequency comb in 1.5

\ensuremath{\mu}

m optical communication bands based on the Rb two-photon transitions.

We demonstrate the direct frequency comb spectroscopy of Rb 5S→5D two-photon transitions directly excited by an optical frequency comb (OFC) in 1.5 μm fiber communication bands. A chain of comb spectral manipulation and quantum coherence control is implemented to enhance the efficiency of second harmonic OFC generation and eliminate the Doppler-broadening background. The direct frequency comb spectroscopy with clearly resolved transition lines is obtained. Our scheme provides a potential approach to realize the OFC at ~1.5 μm with high stability and accuracy.

We demonstrate an approach to create a stable erbium-fiber-based frequency comb at communication band by directly locking the combs to two rubidium atomic transitions resonances (electromagnetically induced transparency absorption and two-photon absorption), respectively. This approach directly transfers the precision and stability of the atomic transitions to the comb. With its distinguishing feature of compactness by removing the conventional octave-spanning spectrum and f-to-2f beating facilities and the ability to directly control the comb's frequency at the atomic transition frequency, this stable optical comb can be widely used in optical communication, frequency standard, and optical spectroscopy and microscopy.

The two-photon transition $5S\ensuremath{-}5P\ensuremath{-}5D$ in rubidium vapor is investigated by detecting the fluorescence from the

6{P}_{3/2}

state when the atomic system is excited by the combined action of a cw diode laser and a frequency comb. The cw laser plays a role as a velocity-selective filter and allows for sub-Doppler spectroscopy over a large spectral range including the

5{D}_{3/2}

and

5{D}_{5/2}

states. For a counterpropagating beam configuration, the response of each atomic velocity group is well characterized within the Doppler profile and the excited hyperfine levels are clearly resolved. The contribution of the optical pumping to the direct two-photon process is also revealed. The results are well described in a frequency domain picture by considering the interaction of each velocity group with the cw laser and the modes of the frequency comb.