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arXiv:1207.2187 · Physical Review A

Dynamics of Feshbach molecules in an ultracold three-component mixture

Alexander Y. Khramov, Anders H. Hansen, Alan O. Jamison, William H. Dowd, Subhadeep Gupta

Published Sep 10, 2012• 16 citations
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Abstract

We present investigations of the formation rate and collisional stability of lithium Feshbach molecules in an ultracold three-component mixture composed of two resonantly interacting fermionic ${}^{6}$Li spin states and bosonic ${}^{174}$Yb. We observe long molecule lifetimes ($>100$ ms) even in the presence of a large ytterbium bath and extract reaction rate coefficients of the system. We find good collisional stability of the mixture in the unitary regime, opening new possibilities for studies and probes of strongly interacting quantum gases in contact with a bath species.

DOI
10.1103/physreva.86.032705

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Using a Feshbach resonance, we create ultracold fermionic molecules starting from a Bose-Fermi atom gas mixture. The resulting mixture of atoms and weakly bound molecules provides a rich system for studying few-body collisions because of the variety of atomic collision partners for molecules; either bosonic, fermionic, or distinguishable atoms. Inelastic loss of the molecules near the Feshbach resonance is dramatically affected by the quantum statistics of the colliding particles and the scattering length. In particular, we observe a molecule lifetime as long as 100 ms near the Feshbach resonance.
We describe the formation of fermionic NaLi Feshbach molecules from an ultracold mixture of bosonic 23{}^{23}23Na and fermionic 6{}^{6}6Li. Precise magnetic field sweeps across a narrow Feshbach resonance at 745 G result in a molecule conversion fraction of 55%5 for our experimental densities and temperatures, corresponding to a molecule number of $5\ifmmode\times\else\texttimes\fi{}{10}^{4}$. The observed molecular decay lifetime is 1.31.31.3 ms after removing free Li and Na atoms from the trap. Due to its extremely low reactivity, NaLi molecules in the ground state will have a much longer lifetime than KRb.
We report on the observation of magnetic Feshbach resonances in a Fermi-Fermi mixture of ultracold atoms with extreme mass imbalance and on their unique p-wave dominated three-body recombination processes.Our system consists of open-shell alkali-metal 6 Li and closed-shell 173 Yb atoms, both spin polarized and held at various temperatures between 1 and 20 μK.We confirm that Feshbach resonances in this system are solely the result of a weak separation-dependent hyperfine coupling between the electronic spin of 6 Li and the nuclear spin of 173 Yb.Our analysis also shows that three-body recombination rates are controlled by the identical fermion nature of the mixture, even in the presence of s-wave collisions between the two species and with recombination rate coefficients outside the Wigner threshold regime at our lowest temperature.Specifically, a comparison of experimental and theoretical line shapes of the recombination process indicates that the characteristic asymmetric line shape as a function of applied magnetic field and a maximum recombination rate coefficient that is independent of temperature can only be explained by triatomic collisions with nonzero, p-wave total orbital angular momentum.The resonances can be used to form ultracold doublet ground-state molecules and to simulate quantum superfluidity in mass-imbalanced mixtures.
We investigate the possibility of forming Li+Yb ultracold molecules by magnetoassociation in mixtures of ultracold atoms. We find that magnetically tunable Feshbach resonances exist, but are extremely narrow for even-mass ytterbium isotopes, which all have zero spin. For odd-mass Yb isotopes, however, there is a new mechanism due to hyperfine coupling between the electron spin and the Yb nuclear magnetic moment. This mechanism produces Feshbach resonances for fermionic Yb isotopes that can be more than 2 orders of magnitude larger than for the bosonic counterparts.
The topic of the present lecture notes are two-species quantum mixtures composed of a deeply degenerate Fermi gas and a second component, the latter being fermionic or bosonic. A key ingredient is the possibility to tune the sss-wave interaction between the different species by means of magnetically controlled Feshbach resonances, which allow us to investigate regimes of strong interactions. In two case studies, we review our experiments on mixtures of 6^66Li fermions with fermionic 40^{40}40K or bosonic 41^{41}41K atoms and on mixtures of fermionic 161^{161}161Dy with 40^{40}40K atoms. We cover various topics of fermionic quantum many-body physics, ranging from impurity physics and quasiparticles over phase separation to the formation of ultracold molecules and progress towards novel superfluids.