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arXiv:1201.6597 · Physical Review Letters

Ultrafast Spin-Motion Entanglement and Interferometry with a Single Atom

Jonathan Mizrahi, Crystal Senko, Brian Neyenhuis, K. G. Johnson, Wesley C. Campbell, C. W. S. Conover, Christopher R. Monroe

Published May 13, 2013• 89 citations
arXivHTMLPDF

Abstract

We report entanglement of a single atom's hyperfine spin state with its motional state in a time scale of less than 3 ns. We engineer a short train of intense laser pulses to impart a spin-dependent momentum transfer of ± 2 ħk. Using pairs of momentum kicks, we create an atomic interferometer and demonstrate collapse and revival of spin coherence as the motional wave packet is split and recombined. The revival after a pair of kicks occurs only when the second kick is delayed by an integer multiple of the harmonic trap period, a signature of entanglement and disentanglement of the spin with the motion. Such quantum control opens a new regime of ultrafast entanglement in atomic qubits.

DOI
10.1103/physrevlett.110.203001

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We report entanglement of a single atom's hyperfine spin state with its motional state in a time scale of less than 3 ns. We engineer a short train of intense laser pulses to impart a spin-dependent momentum transfer of ± 2 ħk. Using pairs of momentum kicks, we create an atomic interferometer and demonstrate collapse and revival of spin coherence as the motional wave packet is split and recombined. The revival after a pair of kicks occurs only when the second kick is delayed by an integer multiple of the harmonic trap period, a signature of entanglement and disentanglement of the spin with the motion. Such quantum control opens a new regime of ultrafast entanglement in atomic qubits.
Trapped atomic ions are a promising medium for quantum computing, due to their long coherence times and potential for scalability. Current methods of en-tangling ions rely on addressing individual modes of motion within the trap and applying qubit state dependent forces with external fields. This approach can limit the speed of entangling gates and make them vulnerable to decoherence due to coupling to unwanted modes or ion heating. This thesis is directed towards demon-strating novel entanglement schemes which are not limited by the trap frequency, and can be made almost arbitrarily fast. Towards this goal, I report here on the first experiments using ultrafast laser pulses to control the internal and external states of a single trapped ion. I begin with experiments in ultrafast spin control, showing how a single laser pulse can be used to completely control both spin degrees of freedom of the ion qubit in tens of picoseconds. I also show how a train of weak pulses can be used to drive Raman transitions based on a frequency comb. I then discuss exper-iments using pulses to rapidly entangle the spin with the motion, and how careful spectral redistribution allows a single pulse to execute a spin-dependent momentum kick. Finally, I explain how these spin-dependent momentum kicks can be used in the future to create an ultrafast entangling gate. I go over how such a gate would work, and present experimentally realizable timing sequences which would create a maximally entangled state of two ions in a time faster than the period of motion in the trap.
Trapped atomic ions are a promising medium for quantum computing, due to their long coherence times and potential for scalability. Current methods of entangling ions rely on addressing individual modes of motion within the trap and applying qubit state dependent forces with external fields. This approach can limit the speed of entangling gates and make them vulnerable to decoherence due to coupling to unwanted modes or ion heating. This thesis is directed towards demonstrating novel entanglement schemes which are not limited by the trap frequency, and can be made almost arbitrarily fast. Towards this goal, I report here on the first experiments using ultrafast laser pulses to control the internal and external states of a single trapped ion. I begin with experiments in ultrafast spin control, showing how a single laser pulse can be used to completely control both spin degrees of freedom of the ion qubit in tens of picoseconds. I also show how a train of weak pulses can be used to drive Raman transitions based on a frequency comb. I then discuss experiments using pulses to rapidly entangle the spin with the motion, and how careful spectral redistribution allows a single pulse to execute a spin-dependent momentum kick. Finally, I explain how these spin-dependent momentum kicks can be used in the future to create an ultrafast entangling gate. I go over how such a gate would work, and present experimentally realizable timing sequences which would create a maximally entangled state of two ions in a time faster than the period of motion in the trap.
Pulsed lasers offer significant advantages over continuous wave (CW) lasers in the coherent control of qubits. Here we review the theoretical and experimental aspects of controlling the internal and external states of individual trapped atoms with pulse trains. Two distinct regimes of laser intensity are identified. When the pulses are sufficiently weak that the Rabi frequency Ω is much smaller than the trap frequency ω trap, sideband transitions can be addressed and atom-atom entanglement can be accomplished in much the same way as with CW lasers. By contrast, if the pulses are very strong Ω ≫ω trap, impulsive spin-dependent kicks can be combined to create entangling gates which are much faster than a trap period. These fast entangling gates should work outside of the Lamb-Dicke regime and be insensitive to thermal atomic motion. © 2013 Springer-Verlag Berlin Heidelberg.
We perform entanglement of spin and motional degrees of freedom of a single, ground-state trapped ion through the application of a 16ps16\phantom{\rule{0.28em}{0ex}}\mathrm{ps}16ps laser pulse. The duration of the interaction is significantly shorter than both the motional timescale ($30\phantom{\rule{0.28em}{0ex}}\textmu{}\text{s}$) and spin precession timescale (1ns1\phantom{\rule{0.28em}{0ex}}\text{ns}1ns), demonstrating that neither sets a fundamental speed limit on this operation for quantum information processing. Entanglement is demonstrated through the collapse and revival of spin coherence as the spin components of the wave function separate and recombine in phase space. We infer the fidelity of these single-qubit operations to be $({97}_{\ensuremath{-}4}^{+3})%$.
We demonstrate single-qubit operations on a trapped atom hyperfine qubit using a single ultrafast pulse from a mode-locked laser. We shape the pulse from the laser and perform a π rotation of the qubit in less than 50 ps with a population transfer exceeding 99% and negligible effects from spontaneous emission or ac Stark shifts. The gate time is significantly shorter than the period of atomic motion in the trap (Ω(Rabi)/ν(trap)>10(4)), demonstrating that this interaction takes place deep within the strong excitation regime.
Ultrafast spin-phonon entanglement based on spin-dependent momentum kicks (SDKs) provides an approach to realize fast entangling gates with intrinsic robustness and scalability for trapped ion quantum computing. Such SDKs so far have been implemented on a nanosecond timescale by off-resonant Raman transitions where each laser pulse is split into a sequence of perturbation pulses with carefully designed temporal patterns. Here we report an experimental realization of ultrafast qubit manipulation and spin-phonon entanglement in picoseconds using SDKs from single resonant laser pulses on the magnetic-field-insensitive hyperfine qubit states. This experiment demonstrates a convenient approach to ultrafast SDKs on noise-insensitive ion-spin qubits, with improvement in its speed by more than an order of magnitude. It removes the need to engineer the pattern of a sequence of perturbation pulses and is less vulnerable to noise, simplifying the approach to large-scale trapped-ion quantum computing based on fast quantum gates with SDKs.