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arXiv:2307.11287 · Physical Review A

Impulsive spin-motion entanglement for fast quantum computation and sensing

Randall Putnam, Adam West, Wesley C. Campbell, Paul Hamilton

Published Mar 18, 2024• 10 citations
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Abstract

We perform entanglement of spin and motional degrees of freedom of a single, ground-state trapped ion through the application of a $16\phantom{\rule{0.28em}{0ex}}\mathrm{ps}$ laser pulse. The duration of the interaction is significantly shorter than both the motional timescale ($30\phantom{\rule{0.28em}{0ex}}\textmu{}\text{s}$) and spin precession timescale ($1\phantom{\rule{0.28em}{0ex}}\text{ns}$), demonstrating that neither sets a fundamental speed limit on this operation for quantum information processing. Entanglement is demonstrated through the collapse and revival of spin coherence as the spin components of the wave function separate and recombine in phase space. We infer the fidelity of these single-qubit operations to be $({97}_{\ensuremath{-}4}^{+3})%$.

DOI
10.1103/physreva.109.032614

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We perform entanglement of spin and motional degrees of freedom of a single, ground-state trapped ion through the application of a 16ps16\phantom{\rule{0.28em}{0ex}}\mathrm{ps}16ps laser pulse. The duration of the interaction is significantly shorter than both the motional timescale (30\textmus30\phantom{\rule{0.28em}{0ex}}\textmu{}\text{s}30\textmus) and spin precession timescale (1ns1\phantom{\rule{0.28em}{0ex}}\text{ns}1ns), demonstrating that neither sets a fundamental speed limit on this operation for quantum information processing. Entanglement is demonstrated through the collapse and revival of spin coherence as the spin components of the wave function separate and recombine in phase space. We infer the fidelity of these single-qubit operations to be (97\ensuremath−4+3)({97}_{\ensuremath{-}4}^{+3})%(97\ensuremath−4+3​).
We report entanglement of a single atom's hyperfine spin state with its motional state in a time scale of less than 3 ns. We engineer a short train of intense laser pulses to impart a spin-dependent momentum transfer of ± 2 ħk. Using pairs of momentum kicks, we create an atomic interferometer and demonstrate collapse and revival of spin coherence as the motional wave packet is split and recombined. The revival after a pair of kicks occurs only when the second kick is delayed by an integer multiple of the harmonic trap period, a signature of entanglement and disentanglement of the spin with the motion. Such quantum control opens a new regime of ultrafast entanglement in atomic qubits.
Trapped atomic ions are a promising medium for quantum computing, due to their long coherence times and potential for scalability. Current methods of entangling ions rely on addressing individual modes of motion within the trap and applying qubit state dependent forces with external fields. This approach can limit the speed of entangling gates and make them vulnerable to decoherence due to coupling to unwanted modes or ion heating. This thesis is directed towards demonstrating novel entanglement schemes which are not limited by the trap frequency, and can be made almost arbitrarily fast. Towards this goal, I report here on the first experiments using ultrafast laser pulses to control the internal and external states of a single trapped ion. I begin with experiments in ultrafast spin control, showing how a single laser pulse can be used to completely control both spin degrees of freedom of the ion qubit in tens of picoseconds. I also show how a train of weak pulses can be used to drive Raman transitions based on a frequency comb. I then discuss experiments using pulses to rapidly entangle the spin with the motion, and how careful spectral redistribution allows a single pulse to execute a spin-dependent momentum kick. Finally, I explain how these spin-dependent momentum kicks can be used in the future to create an ultrafast entangling gate. I go over how such a gate would work, and present experimentally realizable timing sequences which would create a maximally entangled state of two ions in a time faster than the period of motion in the trap.
Trapped atomic ions are a promising medium for quantum computing, due to their long coherence times and potential for scalability. Current methods of en-tangling ions rely on addressing individual modes of motion within the trap and applying qubit state dependent forces with external fields. This approach can limit the speed of entangling gates and make them vulnerable to decoherence due to coupling to unwanted modes or ion heating. This thesis is directed towards demon-strating novel entanglement schemes which are not limited by the trap frequency, and can be made almost arbitrarily fast. Towards this goal, I report here on the first experiments using ultrafast laser pulses to control the internal and external states of a single trapped ion. I begin with experiments in ultrafast spin control, showing how a single laser pulse can be used to completely control both spin degrees of freedom of the ion qubit in tens of picoseconds. I also show how a train of weak pulses can be used to drive Raman transitions based on a frequency comb. I then discuss exper-iments using pulses to rapidly entangle the spin with the motion, and how careful spectral redistribution allows a single pulse to execute a spin-dependent momentum kick. Finally, I explain how these spin-dependent momentum kicks can be used in the future to create an ultrafast entangling gate. I go over how such a gate would work, and present experimentally realizable timing sequences which would create a maximally entangled state of two ions in a time faster than the period of motion in the trap.
We present a theoretical study of fast all-to-all entangling gates in trapped-ion quantum processors, based on impulsive excitation of spin-dependent motion with broadband laser pulses. Previous studies have shown that such fast gate schemes are highly scalable and naturally performant outside the Lamb-Dicke regime, however, are limited to nearest-neighbor operations. Here we demonstrate that impulsive spin-dependent excitation can be used to perform high-fidelity nonlocal entangling operations in quasiuniform chains of up to 40 ions. We identify a regime of phonon-mediated entanglement between arbitrary pairs of ions in the chain, where any two pairs of ions in the chain can be entangled in approximately 1.3-2 center-of-mass oscillation periods. We assess the experimental feasibility of the proposed gate schemes, which reveals pulse error requirements that are weakly dependent on the length of the ion chain and the distance between the target qubits. These results suggest entangling gates based on impulsive spin-dependent excitation present new possibilities for large-scale computation in near-term ion-trap devices.
One of the major problems in building a quantum computer is the development of scalable and robust methods to entangle many qubits. Quantum computers based on trapped atomic ions are one of the most mature and promising platforms for quantum information processing, exhibiting excellent coherence properties, near-perfect qubit detection efficiency, and high-fidelity entangling gates. Entangling operations between multiple ions in a chain typically rely on qubit state-dependent forces that modulate their Coulomb-coupled normal modes of motion. However, scaling these operations to large qubit numbers in a single chain must account for the increasing complexity of the normal mode spectrum, and can result in a gate time slowdown or added complexity of the control forces. In this thesis, I present an alternative route to the scalability problem using optical interactions faster than any state evolution. The experiments shown here represent a proof of principle for quantum manipulation of atoms in the strong coupling regime. This work relies on spin dependent forces (SDK) with short laser pulses and use it as our fundamental building block for thermometry and non-trivial motional state preparation. Together with a robust stabilization of the ion trap and high light collection efficiency, we demonstrate two-ion entanglement with ten ultrafast pulses. Due to the nature of the interaction, the demonstrated entangling operation can be made arbitrarily fast only limited by laser engineering.
Since the dawn of quantum information science, laser-cooled trapped atomic ions have been one of the most compelling systems for the physical realization of a quantum computer. By applying qubit state dependent forces to the ions, their collective motional modes can be used as a bus to realize entangling quantum gates. Ultrafast state-dependent kicks [1] can provide a universal set of quantum logic operations, in conjunction with ultrafast single qubit rotations [2], which uses only ultrafast laser pulses. This may present a clearer route to scaling a trapped ion processor [3]. In addition to the role that spin-dependent kicks (SDKs) play in quantum computation, their utility in fundamental quantum mechanics research is also apparent. In this thesis, we present a set of experiments which demonstrate some of the principle properties of SDKs including ion motion independence (we demonstrate single ion thermometry from the ground state to near room temperature and the largest Schrodinger cat state ever created in an oscillator), high speed operations (compared with conventional atom-laser interactions), and multi-qubit entanglement operations with speed that is not fundamentally limited by the trap oscillation frequency. We also present a method to provide higher stability in the radial mode ion oscillation frequencies of a linear radiofrequency (rf) Paul trap--a crucial factor when performing operations on the rf-sensitive modes. Finally, we present the highest atomic position sensitivity measurement of an isolated atom to date of ~0.5 nm Hz^(-1/2) with a minimum uncertainty of 1.7 nm using a 0.6 numerical aperature (NA) lens system, along with a method to correct aberrations and a direct position measurement of ion micromotion (the inherent oscillations of an ion trapped in an oscillating rf field). This development could be used to directly image atom motion in the quantum regime, along with sensing forces at the yoctonewton [10^(-24) N)] scale for gravity sensing, and 3D imaging of atoms from static to higher frequency motion. These ultrafast atomic qubit manipulation tools demonstrate inherent advantages over conventional techniques, offering a fundamentally distinct regime of control and speed not previously achievable.