Ultrafast spin-phonon entanglement based on spin-dependent momentum kicks (SDKs) provides an approach to realize fast entangling gates with intrinsic robustness and scalability for trapped ion quantum computing. Such SDKs so far have been implemented on a nanosecond timescale by off-resonant Raman transitions where each laser pulse is split into a sequence of perturbation pulses with carefully designed temporal patterns. Here we report an experimental realization of ultrafast qubit manipulation and spin-phonon entanglement in picoseconds using SDKs from single resonant laser pulses on the magnetic-field-insensitive hyperfine qubit states. This experiment demonstrates a convenient approach to ultrafast SDKs on noise-insensitive ion-spin qubits, with improvement in its speed by more than an order of magnitude. It removes the need to engineer the pattern of a sequence of perturbation pulses and is less vulnerable to noise, simplifying the approach to large-scale trapped-ion quantum computing based on fast quantum gates with SDKs.
Ultrafast spin-phonon entanglement based on spin-dependent momentum kicks (SDKs) provides an approach to realize fast entangling gates with intrinsic robustness and scalability for trapped ion quantum computing. Such SDKs so far have been implemented on a nanosecond timescale by off-resonant Raman transitions where each laser pulse is split into a sequence of perturbation pulses with carefully designed temporal patterns. Here we report an experimental realization of ultrafast qubit manipulation and spin-phonon entanglement in picoseconds using SDKs from single resonant laser pulses on the magnetic-field-insensitive hyperfine qubit states. This experiment demonstrates a convenient approach to ultrafast SDKs on noise-insensitive ion-spin qubits, with improvement in its speed by more than an order of magnitude. It removes the need to engineer the pattern of a sequence of perturbation pulses and is less vulnerable to noise, simplifying the approach to large-scale trapped-ion quantum computing based on fast quantum gates with SDKs.
Trapped atomic ions are a promising medium for quantum computing, due to their long coherence times and potential for scalability. Current methods of entangling ions rely on addressing individual modes of motion within the trap and applying qubit state dependent forces with external fields. This approach can limit the speed of entangling gates and make them vulnerable to decoherence due to coupling to unwanted modes or ion heating. This thesis is directed towards demonstrating novel entanglement schemes which are not limited by the trap frequency, and can be made almost arbitrarily fast. Towards this goal, I report here on the first experiments using ultrafast laser pulses to control the internal and external states of a single trapped ion. I begin with experiments in ultrafast spin control, showing how a single laser pulse can be used to completely control both spin degrees of freedom of the ion qubit in tens of picoseconds. I also show how a train of weak pulses can be used to drive Raman transitions based on a frequency comb. I then discuss experiments using pulses to rapidly entangle the spin with the motion, and how careful spectral redistribution allows a single pulse to execute a spin-dependent momentum kick. Finally, I explain how these spin-dependent momentum kicks can be used in the future to create an ultrafast entangling gate. I go over how such a gate would work, and present experimentally realizable timing sequences which would create a maximally entangled state of two ions in a time faster than the period of motion in the trap.
Excitation of trapped-ion hyperfine qubits with fast optical Raman pulses enables faster-than-trap-period entangling gates with qubits of long coherence time for practical quantum computation. Achieving high-fidelity fast two-qubit gates requires high-quality spin-dependent kicks (SDKs), which form their fundamental building blocks. Here, we characterize the control parameters (including Raman frequency difference, pulse arrival times, Lamb--Dicke parameter, temperature, pulse width, and SDK time) that maximize the performance of single-ion SDKs for protocols compatible with performed experiments involving a small number of fast pulses. We demonstrate through analytical methods and numerical simulations that, within the model commonly used for infidelity optimization, finite pulse duration is the dominant source of error, exceeding the contribution of secular motion by orders of magnitude for nanosecond-scale SDKs. Low infidelities -- below 10−3 for schemes with ≳10 fixed-amplitude, equispaced, picosecond pulses -- are achievable in SDK times on the order of nanoseconds. These results provide quantitative design rules for achieving competitive SDK fidelities with current pulsed-laser technology, laying the foundation for sub-microsecond trapped-ion quantum entangling operations.
Trapped atomic ions are a promising medium for quantum computing, due to their long coherence times and potential for scalability. Current methods of en-tangling ions rely on addressing individual modes of motion within the trap and applying qubit state dependent forces with external fields. This approach can limit the speed of entangling gates and make them vulnerable to decoherence due to coupling to unwanted modes or ion heating. This thesis is directed towards demon-strating novel entanglement schemes which are not limited by the trap frequency, and can be made almost arbitrarily fast. Towards this goal, I report here on the first experiments using ultrafast laser pulses to control the internal and external states of a single trapped ion. I begin with experiments in ultrafast spin control, showing how a single laser pulse can be used to completely control both spin degrees of freedom of the ion qubit in tens of picoseconds. I also show how a train of weak pulses can be used to drive Raman transitions based on a frequency comb. I then discuss exper-iments using pulses to rapidly entangle the spin with the motion, and how careful spectral redistribution allows a single pulse to execute a spin-dependent momentum kick. Finally, I explain how these spin-dependent momentum kicks can be used in the future to create an ultrafast entangling gate. I go over how such a gate would work, and present experimentally realizable timing sequences which would create a maximally entangled state of two ions in a time faster than the period of motion in the trap.
We propose high-fidelity single-qubit spin-dependent kicks (SDKs) for trapped ions using nanosecond Raman pulses via amplitude modulation of a continuous-wave laser with a tunable beat frequency. We develop a general method for maintaining SDK performance in the presence of micromotion by identifying optimal choices of the RF phase and frequency that suppress unwanted backward kicks. The proposed scheme enables SDK infidelities as low as 10−9 in the absence of micromotion, and below 10−5 with micromotion. This study lays the foundation for the realization of sub-trap-period and high-fidelity two-qubit gates based on SDKs.
One of the major problems in building a quantum computer is the development of scalable and robust methods to entangle many qubits. Quantum computers based on trapped atomic ions are one of the most mature and promising platforms for quantum information processing, exhibiting excellent coherence properties, near-perfect qubit detection efficiency, and high-fidelity entangling gates. Entangling operations between multiple ions in a chain typically rely on qubit state-dependent forces that modulate their Coulomb-coupled normal modes of motion. However, scaling these operations to large qubit numbers in a single chain must account for the increasing complexity of the normal mode spectrum, and can result in a gate time slowdown or added complexity of the control forces. In this thesis, I present an alternative route to the scalability problem using optical interactions faster than any state evolution. The experiments shown here represent a proof of principle for quantum manipulation of atoms in the strong coupling regime. This work relies on spin dependent forces (SDK) with short laser pulses and use it as our fundamental building block for thermometry and non-trivial motional state preparation. Together with a robust stabilization of the ion trap and high light collection efficiency, we demonstrate two-ion entanglement with ten ultrafast pulses. Due to the nature of the interaction, the demonstrated entangling operation can be made arbitrarily fast only limited by laser engineering.
Since the dawn of quantum information science, laser-cooled trapped atomic ions have been one of the most compelling systems for the physical realization of a quantum computer. By applying qubit state dependent forces to the ions, their collective motional modes can be used as a bus to realize entangling quantum gates. Ultrafast state-dependent kicks [1] can provide a universal set of quantum logic operations, in conjunction with ultrafast single qubit rotations [2], which uses only ultrafast laser pulses. This may present a clearer route to scaling a trapped ion processor [3]. In addition to the role that spin-dependent kicks (SDKs) play in quantum computation, their utility in fundamental quantum mechanics research is also apparent. In this thesis, we present a set of experiments which demonstrate some of the principle properties of SDKs including ion motion independence (we demonstrate single ion thermometry from the ground state to near room temperature and the largest Schrodinger cat state ever created in an oscillator), high speed operations (compared with conventional atom-laser interactions), and multi-qubit entanglement operations with speed that is not fundamentally limited by the trap oscillation frequency. We also present a method to provide higher stability in the radial mode ion oscillation frequencies of a linear radiofrequency (rf) Paul trap--a crucial factor when performing operations on the rf-sensitive modes. Finally, we present the highest atomic position sensitivity measurement of an isolated atom to date of ~0.5 nm Hz^(-1/2) with a minimum uncertainty of 1.7 nm using a 0.6 numerical aperature (NA) lens system, along with a method to correct aberrations and a direct position measurement of ion micromotion (the inherent oscillations of an ion trapped in an oscillating rf field). This development could be used to directly image atom motion in the quantum regime, along with sensing forces at the yoctonewton [10^(-24) N)] scale for gravity sensing, and 3D imaging of atoms from static to higher frequency motion. These ultrafast atomic qubit manipulation tools demonstrate inherent advantages over conventional techniques, offering a fundamentally distinct regime of control and speed not previously achievable.