Two-Dimensional Mott-Hubbard Electrons in an Artificial Honeycomb Lattice
Achintya Singha, Marco Gibertini, B. Karmakar, Shengjun Yuan, Marco Polini, Giovanni Vignale, Mikhail I. Katsnelson, Aron Pinczuk, Loren N. Pfeiffer, K. W. West, V. Pellegrini
Artificial crystal lattices can be used to tune repulsive Coulomb interactions between electrons. We trapped electrons, confined as a two-dimensional gas in a gallium arsenide quantum well, in a nanofabricated lattice with honeycomb geometry. We probed the excitation spectrum in a magnetic field, identifying collective modes that emerged from the Coulomb interaction in the artificial lattice, as predicted by the Mott-Hubbard model. These observations allow us to determine the Hubbard gap and suggest the existence of a Coulomb-driven ground state.
Artificial crystal lattices can be used to tune repulsive Coulomb interactions between electrons. We trapped electrons, confined as a two-dimensional gas in a gallium arsenide quantum well, in a nanofabricated lattice with honeycomb geometry. We probed the excitation spectrum in a magnetic field, identifying collective modes that emerged from the Coulomb interaction in the artificial lattice, as predicted by the Mott-Hubbard model. These observations allow us to determine the Hubbard gap and suggest the existence of a Coulomb-driven ground state.
We create an artificial graphene system with tunable interactions and study the crossover from metallic to Mott insulating regimes, both in isolated and coupled two-dimensional honeycomb layers. The artificial graphene consists of a two-component spin mixture of an ultracold atomic Fermi gas loaded into a hexagonal optical lattice. For strong repulsive interactions, we observe a suppression of double occupancy and measure a gapped excitation spectrum. We present a quantitative comparison between our measurements and theory, making use of a novel numerical method to obtain Wannier functions for complex lattice structures. Extending our studies to time-resolved measurements, we investigate the equilibration of the double occupancy as a function of lattice loading time.
This thesis reports original research on strongly interacting fermions described by Hubbard-like models which can be realized with ultracold atom experiments. In particular, two main directions have been pursued: (i) the control of magnetic and topological properties in a honeycomb lattice through a suitable tuning of the trapping potential, and (ii) the possibility to observe orbital-selective Mott physics in a multicomponent Fermi system where the SU(N) symmetry is broken in a controlled way. The first line of research is based on the idea that increasing the strength of a trapping potential, one can trap a strongly interacting fermions in a limited portion of space, thereby changing their average density and the related magnetic properties. In particular it was demonstrated that this confinement protocol can be used to designeffective “nanoflakes” which are reminiscent of a solid-state proposal [1]. The second step was to extend the same philosophy to the so-called Kane-Mele model, a spinful version of the paradigmatic model proposed by Haldane which presents quantum Hall states. This model can be realized with cold-atom systems using artificial gauge fields. In this thesis we consider a Kane-Mele-Hubbard model where the electronic structure of the Kane-Mele model is supplemented by the onsite Hubbard interaction, allowing us to study the interplay between the correlations and magnetism induced by the repulsion, with the non-trivial topological properties. Also for this model, we follow the strategy discussed above, namely the possibility to engineer an effective “nanoflake” by tuning the lattice potential. The final outcome in this case is even reacher, because it leads, among other results, to a situation where the effective flake hosts an inhomogeneous state which presents at the same time topologically non-trivial properties and magnetism, realizing a spin-Chern insulator [2]. Besides the remarkable application for topological matter, artificial gauge fields, which rely on the coupling of spin states, offer also great insides into mutli-orbital physics. In the second main research line reported in the thesis we study in collaboration with the experimental group of Leonardo Fallani, the controlled symmetry breaking on a 173Yb many-body system, where coupling between spin states is exploited to simulate the mechanism relevant for the physics of multi-orbital materials, such as iron-based superconductors. In order to reveal this mechanism in cold atoms we focus on interacting SU(3) lattice fermions where the SU(3) spin symmetry is explicitly broken by a Raman coupling between the spin states. Combining experiments and theory, we demonstrate that this setup reveals orbital-selective physics and it shows that the SU(3)-symmetry-breaking Raman coupling favours Mott localization and selective properties [3]. Our results show a clear evidence of orbital-selective correlations, which reflect in contrasting transport properties in different orbitals, the extreme case being an orbital-selective Mott state where only some of the orbitals are Mott localized while others remain metallic. Moreover, the coupling between spin states favors Mott localization with respect to the symmetric case, hence it reduces the critical interaction needed for a full Mott localization.
We consider an efficient scheme to simulate fermionic Hubbard models with nonlocal density-density interactions in two dimensions, based on bond-centered auxiliary-field quantum Monte Carlo. The simulations are shown to be sign-problem-free within a finite, restricted parameter range. Using this approach, we first study the Hubbard model on the half-filled square lattice bilayer, including an interlayer repulsion term in addition to the local repulsion, and present the ground-state phase diagram within the accessible parameter region. Starting from the antiferromagnetically ordered state in the absence of interlayer repulsion, the interlayer interactions are found to destabilize the antiferromagnetic order, leading to a band insulator state. Moreover, for sufficiently strong interlayer tunneling, we also observe the emergence of a direct dimer product state of mixed D-Mott and S-Mott character along the equal coupling line. We discuss the stability range of this state within strong-coupling perturbation theory. Furthermore, we consider the Hubbard model on the honeycomb lattice with next-nearest-neighbor interactions. Such an interaction is found to enhance both charge density and spin-current correlations within the semimetallic region. However, inside the accessible parameter region, they do not stabilize long-ranged charge density wave order nor a quantum spin Hall state, and the only insulating state that we observe exhibits long-range antiferromagnetism.
Interacting fermions on the half-filled honeycomb lattice with short-range repulsions have been suggested to host a variety of interesting many-body ground states, e.g., a topological Mott insulator. A number of recent studies of the spinless case in terms of exact diagonalization, the infinite density matrix renormalization group, and the functional renormalization group, however, indicate a suppression of the topological Mott insulating phase in the whole range of interaction parameters. Here, we complement the previous studies by investigating the quantum many-body instabilities of the physically relevant case of spin-1/2 fermions with onsite, nearest-neighbor, and second-nearest-neighbor repulsion. To this end, we employ the multipatch functional renormalization group for correlated fermions with refined momentum resolution observing the emergence of an antiferromagnetic spin-density wave and a charge-density wave for dominating onsite and nearest-neighbor repulsions, respectively. For dominating second-nearest neighbor interaction our results favor an ordering tendency towards a charge-modulated ground state over the topological Mott insulating state. The latter evades a stabilization as the leading instability by the additional onsite interaction.
The Hubbard model encapsulates the physics of strongly correlated quantum systems in its most basic form. It has been studied intensively in the context of the high-temperature superconductivity. A number of novel phases were recently proposed for Hubbard-like models on the honeycomb lattice, the structure of graphene. We analyzed the Hubbard model of spin- 21 fermions on the honeycomb lattice at half-filling using large-scale quantum Monte Carlo simulations. We find that the weak coupling semimetal and the antiferromagnetic Mott insulator at strong interaction are separated by an extended gapped phase in an intermediate coupling regime. Exploring excitation gaps, various correlation functions as well as probing for flux quantization, we conclude that a quantum spin liquid, lacking any conventional order, emerges with local charge and spin correlations, best described by a resonating valence bonds state.
We describe here a quantum simulator of extended bipartite Hubbard model with broken sublattice symmetry. The simulator consists of a structured lateral gate confining two-dimensional electrons in a quantum well into artificial minima arranged in a hexagonal lattice. The sublattice symmetry breaking is generated by forming an artificial triangular graphene quantum dot (ATGQD) with zigzag edges. The resulting extended Hubbard model generates tunable ratio of tunneling strength to electron-electron interactions and of sublattice symmetry with control over shape. The validity of the simulator is confirmed for small systems using mean-field and exact diagonalization many-body approaches which show that the ground state changes from a metallic to an antiferromagnetic (AF) phase by varying the distance between sites or depth of the confining potential. The one-electron spectrum of these triangular dots contains a macroscopically degenerate shell at the Fermi level. The shell persists at the mean-field level for weak interactions (metallic phase) but disappears for strong interactions in the AF phase. We determine the effects of electron-electron interactions on the ground state, the total spin, and the excitation spectrum as a function of filling of the ATGQD. We find that the half-filled charge neutral shell leads to a partially spin-polarized state in both metallic and AF regimes in accordance with Lieb's theorem. In both regimes a relatively large gap separates the spin-polarized ground state to the first excited many-body state at half-filling of the degenerate shell. By adding or removing an electron, this gap drops dramatically, and alternate total spin states emerge with energies nearly degenerate to a spin-polarized ground state.