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Mott transitions, topology, and magnetism of interacting fermions in confined geometries.

Karla Jana Baumann

Published Aug 28, 2020• 0 citations
OpenAlex

Abstract

This thesis reports original research on strongly interacting fermions described by Hubbard-like models which can be realized with ultracold atom experiments. In particular, two main directions have been pursued: (i) the control of magnetic and topological properties in a honeycomb lattice through a suitable tuning of the trapping potential, and (ii) the possibility to observe orbital-selective Mott physics in a multicomponent Fermi system where the SU(N) symmetry is broken in a controlled way. The first line of research is based on the idea that increasing the strength of a trapping potential, one can trap a strongly interacting fermions in a limited portion of space, thereby changing their average density and the related magnetic properties. In particular it was demonstrated that this confinement protocol can be used to designeffective “nanoflakes” which are reminiscent of a solid-state proposal [1]. The second step was to extend the same philosophy to the so-called Kane-Mele model, a spinful version of the paradigmatic model proposed by Haldane which presents quantum Hall states. This model can be realized with cold-atom systems using artificial gauge fields. In this thesis we consider a Kane-Mele-Hubbard model where the electronic structure of the Kane-Mele model is supplemented by the onsite Hubbard interaction, allowing us to study the interplay between the correlations and magnetism induced by the repulsion, with the non-trivial topological properties. Also for this model, we follow the strategy discussed above, namely the possibility to engineer an effective “nanoflake” by tuning the lattice potential. The final outcome in this case is even reacher, because it leads, among other results, to a situation where the effective flake hosts an inhomogeneous state which presents at the same time topologically non-trivial properties and magnetism, realizing a spin-Chern insulator [2]. Besides the remarkable application for topological matter, artificial gauge fields, which rely on the coupling of spin states, offer also great insides into mutli-orbital physics. In the second main research line reported in the thesis we study in collaboration with the experimental group of Leonardo Fallani, the controlled symmetry breaking on a 173Yb many-body system, where coupling between spin states is exploited to simulate the mechanism relevant for the physics of multi-orbital materials, such as iron-based superconductors. In order to reveal this mechanism in cold atoms we focus on interacting SU(3) lattice fermions where the SU(3) spin symmetry is explicitly broken by a Raman coupling between the spin states. Combining experiments and theory, we demonstrate that this setup reveals orbital-selective physics and it shows that the SU(3)-symmetry-breaking Raman coupling favours Mott localization and selective properties [3]. Our results show a clear evidence of orbital-selective correlations, which reflect in contrasting transport properties in different orbitals, the extreme case being an orbital-selective Mott state where only some of the orbitals are Mott localized while others remain metallic. Moreover, the coupling between spin states favors Mott localization with respect to the symmetric case, hence it reduces the critical interaction needed for a full Mott localization.

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This thesis reports original research on strongly interacting fermions described by Hubbard-like models which can be realized with ultracold atom experiments. In particular, two main directions have been pursued: (i) the control of magnetic and topological properties in a honeycomb lattice through a suitable tuning of the trapping potential, and (ii) the possibility to observe orbital-selective Mott physics in a multicomponent Fermi system where the SU(N) symmetry is broken in a controlled way. The first line of research is based on the idea that increasing the strength of a trapping potential, one can trap a strongly interacting fermions in a limited portion of space, thereby changing their average density and the related magnetic properties. In particular it was demonstrated that this confinement protocol can be used to designeffective “nanoflakes” which are reminiscent of a solid-state proposal [1]. The second step was to extend the same philosophy to the so-called Kane-Mele model, a spinful version of the paradigmatic model proposed by Haldane which presents quantum Hall states. This model can be realized with cold-atom systems using artificial gauge fields. In this thesis we consider a Kane-Mele-Hubbard model where the electronic structure of the Kane-Mele model is supplemented by the onsite Hubbard interaction, allowing us to study the interplay between the correlations and magnetism induced by the repulsion, with the non-trivial topological properties. Also for this model, we follow the strategy discussed above, namely the possibility to engineer an effective “nanoflake” by tuning the lattice potential. The final outcome in this case is even reacher, because it leads, among other results, to a situation where the effective flake hosts an inhomogeneous state which presents at the same time topologically non-trivial properties and magnetism, realizing a spin-Chern insulator [2]. Besides the remarkable application for topological matter, artificial gauge fields, which rely on the coupling of spin states, offer also great insides into mutli-orbital physics. In the second main research line reported in the thesis we study in collaboration with the experimental group of Leonardo Fallani, the controlled symmetry breaking on a 173Yb many-body system, where coupling between spin states is exploited to simulate the mechanism relevant for the physics of multi-orbital materials, such as iron-based superconductors. In order to reveal this mechanism in cold atoms we focus on interacting SU(3) lattice fermions where the SU(3) spin symmetry is explicitly broken by a Raman coupling between the spin states. Combining experiments and theory, we demonstrate that this setup reveals orbital-selective physics and it shows that the SU(3)-symmetry-breaking Raman coupling favours Mott localization and selective properties [3]. Our results show a clear evidence of orbital-selective correlations, which reflect in contrasting transport properties in different orbitals, the extreme case being an orbital-selective Mott state where only some of the orbitals are Mott localized while others remain metallic. Moreover, the coupling between spin states favors Mott localization with respect to the symmetric case, hence it reduces the critical interaction needed for a full Mott localization.
The present thesis is devoted to the study of physical phenomena emerging from strong correlations in strongly interacting quantum many-body systems with several components. Hubbard models are widely used as minimal models which take into account the interactions between particles and they have been studied in relation to phenomena such as Mott localization, unconventional superconductivity, quantum magnetism and many others. All of these striking phenomena share their origin from the strong correlations among fermions induced by their mutual interactions. Furthermore, condensed matter models are usually realized only in an approximate fashion in actual solid-state systems, making the situation all the more puzzling and hard to be treated analytically or numerically. Therefore, a great effort has been performed to simulate Hubbard models in a system of atoms cooled down to ultra low temperatures and trapped in optical lattices. The most peculiar feature of cold atoms experiments consists in the possibility of tuning relevant physical parameters of the systems, as the density or the interactions among atoms, using laser and/or magnetic fields. This paved the way to the observation of fundamental quantum states of matter as the weakly interacting Bose-Einstein condensate, the super fluid to Mott insulator transition, the super fluid BEC-BCS crossover, the Mott transition in systems of composite fermions and so on. Hence, it is considered of great interest establishing connections between the quantum simulations cold atomic toolbox and systems realized in solid-state physics...
In recent years, topology has become increasingly prevalent in condensed matter physics. It has allowed us to understand, and even predict, a variety of striking and remarkable physical phenomena. The study of strongly interacting systems has similarly lavished us with a diverse range of exotic phases and unconventional transitions, many of which are still poorly understood. In this thesis we will explore the interplay between topology and interactions in an effort to uncover new and novel phases. First we study how interactions impact the quantum phase transition between a topologically non-trivial phase and a trivial phase. The combination of interactions and the low-energy degrees of freedom associated with the transition leads to the emergence of a dome of lattice-symmetry breaking nematic order. Such behaviour is reminiscent of a number of strongly correlated electronic systems. We move on to study the strongly interacting limit of one of the earliest and best-known non-interacting topological phases, Haldane's model of a Chern insulator. Recently realized with ultracold atoms in a shaken optical lattice, the model has a non-trivial topological invariant associated with its band structure. In the strongly interacting limit the spin degrees of freedom are all that survive and we find a rich phase diagram of magnetically ordered phases, using a combination of both classical and quantum techniques. Supplementing the model with an additional term we can `quantum-melt' one of these ordered states to produce a disordered, liquid state that we positively identify as a chiral spin liquid, a highly entangled state of matter with fractionalised excitations. We generalise this mechanism to other two dimensional lattices, uncovering a possible unifying framework with which to understand the emergence of chiral spin liquids in lattice spin models. Finally, motivated by groundbreaking experiments in the ultracold atoms community, we investigate a model of two-component bosons with an artificial spin-orbit coupling. The interplay between the lattice, interactions and spin-orbit coupling produces a variety of unusual superfluid phases. Using a novel Monte Carlo technique we reveal the finite temperature phase diagram that appears close to the Mott transition.
Abstract A large repulsion between particles in a quantum system can lead to their localization, an effect responsible for the Mott insulator phases in strongly correlated materials. In a system with multiple orbitals, an orbital-selective Mott insulator can form, where electrons in some orbitals are predicted to localize while others remain itinerant. Here we demonstrate a more general version of this phenomenon by observing flavour-selective localization in an atom-based quantum simulator. Our experiment realizes Fermi–Hubbard models with an SU(3) symmetry that can be broken using a tunable coupling between flavours. We observe an enhancement of the localization associated with a selective Mott transition and the emergence of flavour-dependent correlations. Our realization of flavour-selective Mott physics demonstrates the potential of cold atoms to simulate interacting multicomponent materials such as superconductors and topological insulators.
We study strongly interacting ultracold spin-1/21/21/2 fermions in a honeycomb lattice in the presence of a harmonic trap. Tuning the strength of the harmonic trap we show that it is possible to confine the fermions in artificial structures reminiscent of graphene nanoflakes in solid state. The confinement on small structures induces magnetic effects which are absent in a large graphene sheet. Increasing the strength of the harmonic potential we are able to induce different magnetic states, such as a N\'eel-like antiferromagnetic or ferromagnetic state, as well as mixtures of these basic states. The realization of different magnetic patterns is associated with the terminations of the artificial structures, in turn controlled by the confining potential.
The present thesis studies a variety of cold atomic systems in artificial gauge fields. In the first part we focus on fractional quantum Hall effects, asking whether interesting topological states can be realized with cold atoms. We start by making a close connection to solid-state systems and first consider fermionic atoms with dipolar interactions. Assuming the system to be in the Laughlin state, we evaluate the energy gap in the thermodynamic limit as a measure for the robustness of the state. We show that it can be increased by additionally applying a non-Abelian gauge field squeezing the Landau levels. We then switch to bosonic systems with repulsive contact interactions. Artificial magnetic fields for cold bosons have extensively been discussed before in the context of rotating Bose gases. We follow a different approach where the gauge field is due to an atom-laser coupling. Thus, transitions between different dressed states have to be included. They are shown to break the cylindrical symmetry of the system. Modifying the Laughlin state and the Moore-Read state accordingly, we determine the parameter regimes where they are good representations for the ground state of the system obtained via exact diagonalization. One of the most interesting feature of fractional quantum Hall states is the anyonic behavior of their excitations. We therefore also study quasiholes in the Laughlin state and the modified Laughlin state. They are shown to posses anyonic properties, which become manifest even in small systems. Moreover, the dynamics of a single quasihole causes visible traces in the density of the system which allow to clearly distinguish the Laughlin regime from less correlated phases. In the latter, a sequence of collapses and revivals of the quasihole can be observed, which is absent in the Laughlin regime. Extending our study to bosonic systems with a pesudospin-1/2 degree of freedom, we discuss the formation of strongly correlated spin singlets. Strikingly, at filling v=4/3, the system is described by a state with non-Abelian excitations, which is constructed as the zero-energy ground state of repulsive three-body contact interactions. Systems with internal degrees of freedom also allow for implementing artificial spin-orbit coupling. It is shown to give rise to a variety of incompressible states. In the second part of the thesis, we concentrate on condensed system. Bose-Einstein condensates with spin-orbit coupling are shown to have a degeneracy on the mean-field level, which is lifted by quantum and thermal fluctuations. The system becomes experimentally feasible in three dimensions, where the condensate depletion remains finite, and thus allow for an experimental observation of this order-by-disorder mechanism. Finally, we study the influence of Abelian and non-Abelian gauge fields on the quantum phase transitions of bosons in a square optical lattice. Re-entrant superfluid phases and superfluids at finite momenta are interesting properties featured by such systems.
Complex quantum many-body systems are ubiquitous in nature, yet their behaviour often remains very challenging to predict with analytical or numerical calculations.In this thesis a different approach is presented, using ultracold fermionic 40 K atoms in a lattice with a flexible geometry, formed by interfering laser beams.This system constitutes a precisely tunable, yet very accessible complex system, which can be used to probe -or "quantum simulate" -phenomena predicted for condensed-matter systems.We demonstrate, theoretically and experimentally, how a periodically modulated system can be described by an effective Hamiltonian on longer time-scales.This approach based on Floquet theory applies even when driving the system far from equilibrium.Using oscillating magnetic field gradients, we create an effectively spin-dependent lattice, where the tunnelling rate for different internal atomic states can be freely tuned.The flexible geometry of the lattice is used to create a honeycomb lattice and study the linear band crossings -known as Dirac cones -characteristic of its band structure.We distort the lattice and use momentum-resolved interband transitions probe the deformation and movement of the Dirac cones and their eventual disappearance when moving towards a square or dimerised geometry.We show that circular modulation of a honeycomb lattice induces imaginary next-nearest neighbour tunnelling, which breaks time-reversal symmetry.In addition, a tunable site-offset is used to break inversion symmetry.We thereby realize a model proposed by F.D.M. Haldane in 1988 and study the predicted topological transition from a trivial to a Chern-insulating regime, characterised by a closing band gap.Furthermore, effects of the Berry curvature are observed in both regimes, using transverse drifts of a driven atomic cloud.Using a mixture of two internal states with tunable scattering between them, we study the Hubbard model on a variety of geometries and with a range of observables.The crossover between metal, Mott-insulator and band insulator in a two-and threedimensional Honeycomb lattice is probed by observing the double occupancy, compressibility and excitation spectrum.The addition of a site-offset leads to the appearance of a competing type of density order -an explicit charge-density wave -which is directly probed and leads to new types of excitations.At lower temperatures, magnetic correlations appear.By freezing out the dynamics of the system and adiabatically merging neighbouring sites,the probability to find singlet or triplet states on different patterns of bonds is directly probed.Using this method we study the dependence of magnetic correlations on geometry in seven different lattice structures, and crossovers between them.We find that lower connectivity quantum effects enhance short-range correlations and compare our results to sophisticated numerical approximations.Ramping the lattice from one geometry to another allows for probing the quantum dynamics of re-distributing magnetic correlations, from the sudden to the adiabatic regime.v