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arXiv:1104.0238 · Nature Communications

Violation of a Leggett–Garg inequality with ideal non-invasive measurements

George C. Knee, Stephanie Simmons, Erik M. Gauger, John J. L. Morton, Helge P. Riemann, Nikolai V. Abrosimov, Peter Becker, Hans-Joachim Pohl, Kohei M. Itoh, Mike L. W. Thewalt, G. Andrew D. Briggs, Simon C. Benjamin

Published Jan 3, 2012• 259 citations
arXivHTMLPDF

Abstract

The quantum superposition principle states that an entity can exist in two different states simultaneously, counter to our 'classical' intuition. Is it possible to understand a given system's behaviour without such a concept? A test designed by Leggett and Garg can rule out this possibility. The test, originally intended for macroscopic objects, has been implemented in various systems. However to date no experiment has employed the 'ideal negative result' measurements that are required for the most robust test. Here we introduce a general protocol for these special measurements using an ancillary system, which acts as a local measuring device but which need not be perfectly prepared. We report an experimental realization using spin-bearing phosphorus impurities in silicon. The results demonstrate the necessity of a non-classical picture for this class of microscopic system. Our procedure can be applied to systems of any size, whether individually controlled or in a spatial ensemble. Quantum mechanics predicts that objects can simultaneously exist in a superposition of two states. Kneeet al.propose and demonstrate experimentally a protocol which fully confirms this prediction, by testing the so-called Leggett–Garg inequality in a non-invasive manner.

DOI
10.1038/ncomms1614

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The quantum superposition principle states that an entity can exist in two different states simultaneously, counter to our 'classical' intuition. Is it possible to understand a given system's behaviour without such a concept? A test designed by Leggett and Garg can rule out this possibility. The test, originally intended for macroscopic objects, has been implemented in various systems. However to date no experiment has employed the 'ideal negative result' measurements that are required for the most robust test. Here we introduce a general protocol for these special measurements using an ancillary system, which acts as a local measuring device but which need not be perfectly prepared. We report an experimental realization using spin-bearing phosphorus impurities in silicon. The results demonstrate the necessity of a non-classical picture for this class of microscopic system. Our procedure can be applied to systems of any size, whether individually controlled or in a spatial ensemble. Quantum mechanics predicts that objects can simultaneously exist in a superposition of two states. Kneeet al.propose and demonstrate experimentally a protocol which fully confirms this prediction, by testing the so-called Leggett–Garg inequality in a non-invasive manner.
When a physical object is in a quantum superposition, interference among the possible quantum paths affects the outcomes of a measurement. Gaining knowledge about the system with an intermediate measurement smears out, if not completely destroys, the resulting interference pattern. Based on this idea, Leggett and Garg formulated an inequality relating two-time correlation measurements, which establishes a quantitative criterion for discerning quantum superposition on a fundamental ground. Originally proposed to test realism of macroscopic physical objects, the inequality is here used to prove the non-classicality of the motion of a cesium atom, which propagates on a space-time discrete lattice. Making use of ideal negative measurements to test the atom's motion, we obtain a 6 sigma experimental violation of the Leggett-Garg inequality. From a broader perspective, our findings provide rigorous validation of the idea that quantum transport experiments cannot be interpreted in terms of classical trajectories.
"According to the quantum superposition principle, quantum mechanics at the macroscopic scale predicts that a macroscopic system can be in more than one distinct state at the same time. Such an extrapolation of quantum mechanics contradicts our everyday instinct, summarized by Leggett and Garg (LG) under the heading of macrorealism (MR) [1]. To resolve the conflict and to determine whether MR or quantum mechanics is the right description of macroscopic objects, in 1985, Leggett and Garg [1] proposed the temporal Bell's inequality (TBI). If a macorealist description is possible, the inequality is satisfied - quantum mechanics, on the other hand, predicts a violation. Thereafter, people were motivated to engineer macroscopic quantum systems and to test the TBI. In the TBI, one of the most critical postulates is that of the noninvasive measurability (NIM) : it is in principle possible to determine which state the system is in with an arbitrarily small e ect on the subsequent system dynamics. To satisfy the NIM postulate in the TBI experiment, the implementation of the ""ideal negative result"" (INR) measurement was also proposed by LG [1]. In a two-state system, an INR measurement is designed to interact (in each run) with only one of two system states. Only runs where the measurement reported no outcome are kept. Although in the last few years there have been tests of the TBI on microscopic systems with the use of INR measurements [4] and on macroscopic systems using weak measurement [5], no one has ever implemented INR measurements on macroscopic systems in TBI tests so far. In addition, the NIM postulate was simply assumed, and not veri ed by an ancillary test [9, 3]. With these considerations in mind, there are two main tasks in this thesis: the rst one is to analyze the realization of an INR measurement on a macroscopic object. I propose an experiment based on coupling a flux-qubit to a dcSQUID, which mirrors the approach of Knee et al. [4], where the system of interest is coupled to another quantum system which acts as a measuring device. In order to accomplish the first task, we analyze the escape dynamics of a flux-qubit SQUID composite system in various limits and discuss the prospects of operating in a regime realizing a von Neumann (""projective"")-like measurement onto the qubit flux basis. Later in the thesis, I discuss current feasibility of the proposed experiment based on the possible measurement error (the ""venality"" [4]) of our INR measurement. The second task is to analyze experimental tests of measurement invasiveness. I propose a concrete protocol, ancillary to the main TBI experiment, which may narrow some loopholes in the test of MR [3]. I generalize the approach of Wilde and Mizel [3], using the behavior of the two-time correlator of a system as an indicator of measurement invasiveness. The measured invasivities can be used to give a improved lower bound for the TBI."
In contrast to the spatial Bell's inequalities which probe entanglement between spatially separated systems, the Leggett–Garg inequalities test the correlations of a single system measured at different times. Violation of a genuine Leggett–Garg test implies either the absence of a realistic description of the system or the impossibility of measuring the system without disturbing it. Quantum mechanics violates the inequalities on both accounts and the original motivation for these inequalities was as a test for quantum coherence in macroscopic systems. The last few years has seen a number of experimental tests and violations of these inequalities in a variety of microscopic systems such as superconducting qubits, nuclear spins, and photons. In this article, we provide an introduction to the Leggett–Garg inequalities and review these latest experimental developments. We discuss important topics such as the significance of the non-invasive measurability assumption, the clumsiness loophole, and the role of weak measurements. Also covered are some recent theoretical proposals for the application of Leggett–Garg inequalities in quantum transport, quantum biology and nano-mechanical systems.
The Leggett–Garg (LG) test of macroscopic realism involves a series of dichotomic non-invasive measurements that are used to calculate a function which has a fixed upper bound for a macrorealistic system and a larger upper bound for a quantum system. The quantum upper bound depends on both the details of the measurement and the dimension of the system. Here we present an LG experiment on a three-level quantum system, which produces a larger theoretical quantum upper bound than that of a two-level quantum system. The experiment is carried out in nuclear magnetic resonance and consists of the LG test as well as a test of the ideal assumptions associated with the experiment, such as measurement non-invasiveness. The non-invasive measurements are performed via the modified ideal negative result measurement scheme on a three-level system. Once these assumptions are tested, the violation becomes small, despite the fact that the LG value itself is large. Our results showcase the advantages of using the modified measurement scheme that can reach higher LG values, since these leave a larger margin for violating the inequality in the face of experimental imperfections.
The Leggett-Garg inequality is a widely used test of the "quantumness" of a system, and involves correlations between measurements realized at different times. According to its widespread interpretation, a violation of the Legget-Garg inequality disproves macroscopic realism and non-invasiveness. Nevertheless, recent results point out that macroscopic realism is a model dependent notion and that one should always be able to attribute to invasiveness a violation of a Legget-Garg inequality. This opens some natural questions: how to provide such an attribution in a systematic way? How can apparent macroscopic realism violation be recast into a dimensional independent invasiveness model? The present work answers these questions by introducing an operational model where the effects of invasiveness are controllable through a parameter associated with what is called the measurability of the physical system. Such a parameter leads to different generalized measurements that can be associated with the dimensionality of a system, to measurement errors or to back action.
Investigating the boundary between a quantum mechanical description and a classical realistic view is of fundamental importance. The Leggett-Garg (LG) inequality provides a criterion to distinguish between quantum systems and classical systems, and can be used to prove the macroscopic superposition state. A larger upper bound of the LG function can be obtained in a multilevel system. Here, we present an experimental violation of the Leggett-Garg inequality in a three-level system using a nitrogen-vacancy center in diamond by ideal negative result measurements. The experimental maximum value of the Leggett-Garg function is ${K}_{3}^{\text{expt}}=1.625\ifmmode\pm\else\textpm\fi{}0.022$, which exceeds the L\"uders bound with a $5\ensuremath{\sigma}$ level of confidence.