We show how to create long-range interactions between alkali atoms in different hyperfine ground states, with the goal of coherent quantum transport. The scheme uses off-resonant dressing with atomic Rydberg states. We demonstrate coherent migration of electronic excitation through dressed dipole–dipole interaction by full solutions of models with four essential states per atom and give the structure of the spectrum of dressed states for a dimer. In addition, we present an effective (perturbative) Hamiltonian for the ground-state manifold and show that it correctly describes the full multi-state dynamics. We discuss excitation transport in detail for a chain of five atoms. In the presented scheme, the actual population in the Rydberg state is kept small. Dressing offers many advantages over the direct use of Rydberg levels: it reduces ionization probabilities and provides an additional tuning parameter for lifetimes and interaction strengths.
We show how to create long-range interactions between alkali atoms in different hyperfine ground states, with the goal of coherent quantum transport. The scheme uses off-resonant dressing with atomic Rydberg states. We demonstrate coherent migration of electronic excitation through dressed dipole–dipole interaction by full solutions of models with four essential states per atom and give the structure of the spectrum of dressed states for a dimer. In addition, we present an effective (perturbative) Hamiltonian for the ground-state manifold and show that it correctly describes the full multi-state dynamics. We discuss excitation transport in detail for a chain of five atoms. In the presented scheme, the actual population in the Rydberg state is kept small. Dressing offers many advantages over the direct use of Rydberg levels: it reduces ionization probabilities and provides an additional tuning parameter for lifetimes and interaction strengths.
In any physical platform, two ingredients are essential for quantum information processing: single-qubit control, and entangling interactions between qubits. Neutral atoms can be individually controlled with high fidelity and are resilient to environmental noise, making them attractive candidates for implementing quantum information protocols. However, achieving strong interactions remains a major obstacle. One way to increase the interaction strength between neutral atoms is to excite them into high-lying Rydberg states, which exhibit large electric dipole moments (and by extension, strong electric dipole-dipole interactions). By slowly ramping up the Rydberg level coupling in a system, one can "dress'' the atomic ground states with some Rydberg character; this maps the Rydberg dipole interaction to an effective interaction between ground states. Such Rydberg-dressed interaction is the focus of this dissertation. After describing the physics of the Rydberg-dressed interaction, we propose three protocols that demonstrate its versatility and provide a framework for considering some of the details of realistic implementation. In all three cases, Rydberg dressing --- along with some form of single-atom control --- is used to generate highly entangled states of interest. Our first proposal relates to the adiabatic model of quantum computing, in which solutions to problems are encoded in the ground states of carefully engineered Hamiltonians. The Rydberg-dressed interaction can provide nonlinear Hamiltonian terms, allowing us to encode NP-hard and other interesting problems. We model this protocol in the presence of decoherence, and find that computational fidelities of ~0.98 for four atoms should be possible with currently realistic experimental parameters. Our second proposal is also related to quantum computing, this time in the circuit model. The Rydberg-dressed interaction can be used to generate a controlled-NOT logic gate which, when interwoven with single-qubit gates, can perform universal quantum computation. Experimentally, noise due to atomic thermal motion has been a primary limitation on the fidelities of these gates. We show that a Doppler-free setup, with counterpropagating lasers, effectively suppresses this type of noise, allowing simulated fidelities of up to ~0.998 per gate. Such strong suppression is only possible because the Doppler-free configuration can harness the natural robustness of adiabatic dressing; other gate schemes using, e.g., resonant pulses, do not exhibit the same degree of improvement. Finally, we consider exploiting the many-body character of the Rydberg-dressed interaction to generate collective entanglement in mesoscopic ensembles of neutral atoms. An atomic ensemble uniformly illuminated by a single Rydberg-exciting laser is isomorphic to the well-known Jaynes-Cummings model. In addition to adapting generic Jaynes-Cummings entanglement protocols developed in other platforms, one can apply microwaves to drive entanglement in a way that is unique to the atomic platform. We prove that by allowing the microwave phase to vary in time, one can generate arbitrary symmetric states of the ensemble. While this method compares favorably with other entanglement protocols in many ways, the required frequency of phase switching presents a fundamental limitation on its effectiveness. To mitigate this, we propose a variant scheme in which parameters are chosen to only allow excitations within the system's dressed-ground subspace; this effectively cuts phase switching demands in half. All three protocols serve to illustrate the power of the Rydberg-dressed interaction and suggest directions for future study.
We discuss techniques to generate long-range interactions in a gas of ground state alkali atoms, by weakly admixing excited Rydberg states with laser light. This provides a tool to engineer strongly correlated phases with reduced decoherence from inelastic collisions and spontaneous emission. As an illustration, we discuss the quantum phases of dressed atoms with dipole-dipole interactions confined in a harmonic potential, as relevant to experiments. We show that residual spontaneous emission from the Rydberg state acts as a heating mechanism, leading to a quantum-classical crossover.
Quantum state transport is an important way to study the energy or information flow. By combining the unconventional Rydberg pumping mechanism and the diagonal form of van der Waals interactions, we construct a theoretical model via second-order perturbation theory to realize a long-range coherent transport inside the ground-state manifold of neutral atoms systems. With the adjustment of the Rabi frequencies and the interatomic distance, this model can be used to simulate various single-body physics phenomena such as a Heisenberg XX spin chain restricted in the single-excitation manifold, coherently perfect quantum state transfer, the parameter-adjustable Su-Schrieffer-Heeger model, and chiral motion of atomic excitation in a triangle by varying the geometrical arrangement of the three atoms, which effectively avoids the influence of atomic spontaneous emission at the same time. Moreover, the influence of atomic position fluctuation on the fidelity of quantum state transmission is discussed in detail, and the corresponding numerical results show that our work provides a robust and easily implemented scheme for quantum state transport with neutral atoms.
We consider two clouds of ground-state alkali atoms in two distinct hyperfine ground states. Each level is far off-resonantly coupled to a Rydberg state, which leads to dressed ground states with a weak admixture of the Rydberg state properties. Due to this admixture, for a proper choice of the Rydberg states, the atoms experience resonant dipole–dipole interactions that induce mechanical forces acting on all atoms within both clouds. This behaviour is in contrast to the dynamics predicted for bare dipole–dipole interactions between Rydberg superatoms, where only a single atom per cloud is subject to dipole–dipole induced motion (Möbius et al 2013 Phys. Rev. A 88 012716).
Rydberg-dressed ground state atoms are atoms with an electron off-resonantly excited to a very high energy state, i.e., a state of high principal quantum number n ≫ 1. This thesis investigates the quantum dynamics of interacting Rydberg-dressed ground state atoms trapped in several multi-well potential traps. Rydberg atoms are atoms with exaggerated properties. One of their most interesting properties is that they exhibit a strong and long-ranged interaction that can be tuned leading to a variety of different quantum behaviours. My work focuses on studying the effects of these interacting atoms when loaded in multi-well potential traps. Generally, multi-well systems are considered as the simplest example of a finite optical lattice structure. For this reason, this thesis covers three research topics that examine the effects of long-range interaction on Rydberg-dressed atoms trapped in several potential confinements. I begin, in the introduction, by discussing the theoretical background of relevance to this work. It starts with presenting the physics of Bose-Einstein condensate. Then, the fundamentals of the interaction between two-level atom and light are analytically studied. This study has the purpose of understanding both; the dressed interacting atoms and optical lattices. The definition, characteristics, and the nature of the interaction between Rydberg atoms are analysed afterwards. The second chapter examines the dynamics of an ensemble of interacting Rydberg- dressed atoms trapped in static, i.e., time-independent, multi-well potentials using a mean-field theoretical approach. I choose one-dimensional double- and triple-well in addition to a two-dimensional quadruple-well potentials. The time-dependent non-linear Gross-Pitaevskii equation is used to numerically explore the ensemble’s quantum dynamics. Solving the dynamical differential equations along with tuning the strength of the applied long-range interaction shows that the behaviour of non-interacting Rydberg-dressed atoms does not differ conceptually according to the geometry of the trapping potential. However, this changes when the interactions are switched on where the shape of the confinement leads to interesting outcomes especially in the non-linear interacting limit, such as macroscopic quantum self-trapping. After investigating an ensemble of interacting Rydberg-dressed atoms in static multi-well potential traps, the second research topic examines the dynamical evolution of these atoms when loaded in a finite optical lattice using the extended Bose-Hubbard model. In this chapter, the atoms ensemble is assumed to be in a superfluid state where I investigate both, the order parameter when the Rydberg excitation laser is applied and the interference pattern of the condensates in different dimensions. The study shows the emerging long-range interactions lead to a rapid collapse of the superfluid order parameter and in general allow only for partial revivals. In addition, the interference experiments can directly reveal the interaction between Rydberg-dressed atoms. In the fourth chapter, the dynamics of Rydberg-dressed atoms trapped in a dynamical, i.e., time-dependent, potential confinement is presented. The dynamical trap is constructed such that it begins as a harmonic oscillator and ends as a double- well potential. The analysis investigates an ensemble of contact-interacting atoms via the time-dependent non-linear GP equation.
We present a scheme for engineering quantum transport dynamics of spin excitations in a chain of laser-dressed Rydberg atoms, mediated by synthetic spin exchange arising from diagonal van der Waals interaction. The dynamic tunability and long-range interaction feature of our scheme allows for the exploration of transport physics unattainable in conventional spin systems. As two concrete examples, we first demonstrate a topological exciton pumping protocol that facilitates quantized entanglement transfer, and second we discuss a highly nonlocal correlated transport phenomenon which persists even in the presence of dephasing. Unlike previous schemes, our proposal requires neither resonant dipole-dipole interaction nor off-diagonal van der Waals interaction. It can be readily implemented in existing experimental systems.