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arXiv:1009.1403

Tunneling under Coherent Control by Sequences of Unitary Pulses

Saha, Rajdeep, Víctor S. Batista

Published Sep 7, 2010• 0 citations
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Abstract

A general coherent control scenario to suppress, or accelerate, tunneling of quantum states decaying into a continuum, is investigated. The method is based on deterministic, or stochastic, sequences of unitary pulses that affect the underlying interference phenomena responsible for quantum dynamics, without inducing decoherence, or collapsing the coherent evolution of the system. The influence of control sequences on the ensuing quantum dynamics is analyzed by using perturbation theory to first order in the control pulse fields and compared to dynamical decoupling (DD) protocols and sequences of pulses that collapse the coherent evolution and induce quantum Zeno (QZE) or quantum anti-Zeno effects (AZE). The analysis reveals a subtle interplay between coherent and incoherent phenomena and demonstrating that dynamics analogous to evolution due to QZE or AZE can be generated from stochastic sequences of unitary pulses when averaged over all possible realizations.

DOI
10.48550/arxiv.1009.1403

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A general coherent control scenario to suppress, or accelerate, tunneling of quantum states decaying into a continuum, is investigated. The method is based on deterministic, or stochastic, sequences of unitary pulses that affect the underlying interference phenomena responsible for quantum dynamics, without inducing decoherence, or collapsing the coherent evolution of the system. The influence of control sequences on the ensuing quantum dynamics is analyzed by using perturbation theory to first order in the control pulse fields and compared to dynamical decoupling (DD) protocols and sequences of pulses that collapse the coherent evolution and induce quantum Zeno (QZE) or quantum anti-Zeno effects (AZE). The analysis reveals a subtle interplay between coherent and incoherent phenomena and demonstrating that dynamics analogous to evolution due to QZE or AZE can be generated from stochastic sequences of unitary pulses when averaged over all possible realizations.
A general coherent control scenario to suppress or accelerate tunneling of quantum states decaying into a continuum is investigated. The method is based on deterministic, or stochastic, sequences of unitary pulses that affect the underlying interference phenomena responsible for quantum dynamics, without inducing decoherence, or collapsing the coherent evolution of the system. The influence of control sequences on the ensuing quantum dynamics is analyzed by using perturbation theory to first order in the control pulse fields and compared to dynamical decoupling protocols and to sequences of pulses that collapse the coherent evolution and induce quantum Zeno (QZE) or quantum anti-Zeno effects (AZE). The analysis reveals a subtle interplay between coherent and incoherent phenomena and demonstrates that dynamics analogous to the evolution due to QZE or AZE can be generated from stochastic sequences of unitary pulses when averaged over all possible realizations.
This paper investigates the feasibility of using sequences of unitary pulses for achieving coherent-control of quantum dynamical phenomena, including quantum control of electron tunnelling in archetype model systems and control of decoherence in a quantum dot system coupled to a thermal bath. The proposed dynamical decoupling scenario is based on the repetitive application of 2π pulses, affecting the interference phenomena between wave-packet components. The pulses affect the overall relaxation dynamics without collapsing the coherent-quantum evolution of the system. It is shown that both bound-to-bound state tunnelling and bound-to-continuum tunnelling processes can be inhibited and eventually halted by sufficiently frequent pulse fields that exchange energy with the system but do not affect the potential energy tunnelling barriers. Furthermore, the proposed quantum-control scenario is demonstrated as applied to manipulating the electronic quantum dynamics in a quantum dot coupled to a free standing quasi two-dimensional phonon cavity. The reported results are therefore particularly relevant to the understanding of coherent optical manipulation of electronic excitations in semiconductor devices where performance is limited by quantum tunnelling and decoherence.
The quantum-Zeno and anti-Zeno effects (QZE/AZE) are known for a long time, in a quantum system with coupled levels, the measurement of a particular level population can lead to either acceleration (i.e. AZE) or retardation (i.e. QZE) of its population transfer to other levels. Here we consider how one can control the population flow from a coupled quantum state by measurement at a particular time, and what system parameters are responsible for that. We propose a framework for analysis of quantum Zeno dynamics based on time-dependent density matrix perturbation theory. This framework allows us to clearly separate state populations from their coherences and to predict appearance of either QZE or AZE. We illustrate our analysis on two model systems: 1) two coupled levels and 2) a level coupled to a continuum. In both cases dynamics of quantum coherences play a crucial role, and perturbative considerations allow us to predict the effect of projective measurements. In addition, we have extended our consideration to a closely related coherent control scenario, a unitary transformation flipping a sign of a state in a coherent superposition describing the system wavefunction.
The feasibility of achieving coherent control of tunnelling dynamics, associated with electronic excitations in functionalized semiconductor nanostructures, is investigated. The coherent control scenario is based on the application of frequent stochastic unitary pulses, affecting the interference phenomena between electronic wave-packet components and consequently the overall electronic tunnelling dynamics without collapsing the coherent quantum evolution of the system. It is shown that tunnelling can be inhibited and eventually halted by sufficiently frequent pulse fields that exchange energy with the system but do not affect the potential energy tunnelling barriers. Further, the proposed stochastic quantum-control scenario is demonstrated more generally as applied to an archetype model, a particle tunnelling in a quartic double-well potential.
Coherent-optical-control schemes exploit the coherence of laser pulses to change the phases of interfering dynamical pathways and manipulate dynamical processes. These active control methods are closely related to dynamical decoupling techniques, popularized in the field of quantum information. Inspired by nuclear magnetic resonance spectroscopy, dynamical decoupling methods apply sequences of unitary operations to modify the interference phenomena responsible for the system dynamics thus also belonging to the general class of coherent-control techniques. This article reviews related developments in the fields of coherent optical control and dynamical decoupling, emphasizing the control of tunneling and decoherence in general model systems. Considering recent experimental breakthroughs in the demonstration of active control of a variety of systems, we anticipate that the reviewed coherent-control scenarios and dynamical-decoupling methods should raise significant experimental interest.
Coherence control was originally conceived by Shapiro and Brumer for closed quantum systems. In open quantum systems, the environment hampers or destroys coherence. Nevertheless, the Kurizki-Shapiro-Brumer coherent photocurrent control showed partial resilience to decoherence. Still, decoherence control is an essential prerequisite to our ability to fully exploit quantum coherence for any operational task. Yet decoherence control need not employ coherent fields: it may be incoherent. In operational tasks such as the preparation, transformation, transmission, and detection of quantumstates, environmental (bath) effects can be suppressed by dynamical decoupling, or by the more general incoherent dynamical control by modulation developed by our group. The resulting control dynamics must be Zeno-like in order to yield suppressed coupling to the bath in unitary operational tasks. There are however tasks which cannot be implemented by closed-system (unitary) evolution, in particular those involving a change of the system's entropy. Such tasks necessitate efficient coupling to a bath for their implementation. Examples are the use of measurements to cool (purify) a system, to equilibrate it, or harvest (and convert) energy from the environment. If the underlying dynamics is anti-Zeno like, enhancement of this coupling to the bath will occur and thereby facilitate the task, as discovered by us. A general task may also require state and energy transfer between non-interacting parties via shared modes of the bath. For such tasks, a more subtle interplay of Zeno and anti-Zeno dynamics may be optimal. We have therefore constructed a general framework for optimizing the way a system interacts with its environment to achieve a desired task. This optimization consists in adjusting a given “score” that quantifies the success of the task, such as the targeted fidelity, purity, entropy, energy or state transfer probability by dynamical modification of the system-bath coupling spectrum on demand.