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Advances in chemical physics

From Coherent to Incoherent Dynamical Control of Open Quantum Systems

Gershon Kurizki, Analía Zwick

Published Apr 1, 2016• 6 citations
Publisher

Abstract

Coherence control was originally conceived by Shapiro and Brumer for closed quantum systems. In open quantum systems, the environment hampers or destroys coherence. Nevertheless, the Kurizki-Shapiro-Brumer coherent photocurrent control showed partial resilience to decoherence. Still, decoherence control is an essential prerequisite to our ability to fully exploit quantum coherence for any operational task. Yet decoherence control need not employ coherent fields: it may be incoherent. In operational tasks such as the preparation, transformation, transmission, and detection of quantumstates, environmental (bath) effects can be suppressed by dynamical decoupling, or by the more general incoherent dynamical control by modulation developed by our group. The resulting control dynamics must be Zeno-like in order to yield suppressed coupling to the bath in unitary operational tasks. There are however tasks which cannot be implemented by closed-system (unitary) evolution, in particular those involving a change of the system's entropy. Such tasks necessitate efficient coupling to a bath for their implementation. Examples are the use of measurements to cool (purify) a system, to equilibrate it, or harvest (and convert) energy from the environment. If the underlying dynamics is anti-Zeno like, enhancement of this coupling to the bath will occur and thereby facilitate the task, as discovered by us. A general task may also require state and energy transfer between non-interacting parties via shared modes of the bath. For such tasks, a more subtle interplay of Zeno and anti-Zeno dynamics may be optimal. We have therefore constructed a general framework for optimizing the way a system interacts with its environment to achieve a desired task. This optimization consists in adjusting a given “score” that quantifies the success of the task, such as the targeted fidelity, purity, entropy, energy or state transfer probability by dynamical modification of the system-bath coupling spectrum on demand.

DOI
10.1002/9781119096276.ch4

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Universal Dynamical Control of Open Quantum Systems

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Due to increasing demands on speed and security of data processing, along with requirements on measurement precision in fundamental research, quantum phenomena are expected to play an increasing role in future technologies. Special attention must hence be paid to omnipresent decoherence effects, which hamper quantumness. Their consequence is always a deviation of the quantum state evolution (error) with respect to the expected unitary evolution if these effects are absent. In operational tasks such as the preparation, transformation, transmission, and detection of quantum states, these effects are detrimental and must be suppressed by strategies known as dynamical decoupling, or the more general dynamical control by modulation developed by us. The underlying dynamics must be Zeno-like, yielding suppressed coupling to the bath. There are, however, tasks which cannot be implemented by unitary evolution, in particular those involving a change of the system’s state entropy. Such tasks necessitate efficient coupling to a bath for their implementation. Examples include the use of measurements to cool (purify) a system, to equilibrate it, or to harvest and convert energy from the environment. If the underlying dynamics is anti-Zeno like, enhancement of this coupling to the bath will occur and thereby facilitate the task, as discovered by us. A general task may also require state and energy transfer, or entanglement of noninteracting parties via shared modes of the bath which call for maximizing the shared (two-partite) couplings with the bath, but suppressing the single-partite couplings. For such tasks, a more subtle interplay of Zeno and anti-Zeno dynamics may be optimal. We have therefore constructed a general framework for optimizing the way a system interacts with its environment to achieve a desired task. This optimization consists in adjusting a given “score” that quantifies the success of the task, such as the targeted fidelity, purity, entropy, entanglement, or energy by dynamical modification of the system-bath coupling spectrum on demand.

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Quantum control theory for coherence and information dynamics

Lorenza Viola, David J. Tannor

Precisely characterizing and controlling the dynamics of realistic open quantum systems has emerged in recent years as a key challenge across contemporary quantum sciences and technologies, with implications ranging from physics, chemistry and applied mathematics to quantum information processing (QIP) and quantum engineering. Quantum control theory aims to provide both a general dynamical-system framework and a constructive toolbox to meet this challenge. The purpose of this special issue of Journal of Physics B: Atomic, Molecular and Optical Physics is to present a state-of-the-art account of recent advances and current trends in the field, as reflected in two international meetings that were held on the subject over the last summer and which motivated in part the compilation of this volume—the Topical Group: Frontiers in Open Quantum Systems and Quantum Control Theory , held at the Institute for Theoretical Atomic, Molecular and Optical Physics (ITAMP) in Cambridge, Massachusetts (USA), from 1–14 August 2010, and the Safed Workshop on Quantum Decoherence and Thermodynamics Control , held in Safed (Israel), from 22–27 August 2010. Initial developments in quantum control theory date back to (at least) the early 1980s, and have been largely inspired by the well-established mathematical framework for classical dynamical systems. As the above-mentioned meetings made clear, and as the burgeoning body of literature on the subject testifies, quantum control has grown since then well beyond its original boundaries, and has by now evolved into a highly cross-disciplinary field which, while still fast-moving, is also entering a new phase of maturity, sophistication, and integration. Two trends deserve special attention: on the one hand, a growing emphasis on control tasks and methodologies that are specifically motivated by QIP, in addition and in parallel to applications in more traditional areas where quantum coherence is nevertheless vital (such as, for instance, quantum control of chemical reactions or high-resolution magnetic resonance spectroscopy); on the other hand, an unprecedented demand for close coupling between theory and experiment , with theoretical developments becoming more and more attuned to and driven by experimental advances as different quantum technologies continue to evolve at an impressive pace in the laboratory. Altogether, these two trends account for several of the recurrent themes in this volume, as well as in the current quantum control literature as a whole: namely, the quest for control strategies that can attain the highest degree of precision and robustness possible, while striving for efficiency and, ultimately, optimality in achieving the intended control task under realistic operational constraints. From a theory standpoint, this makes it imperative to take into account increasingly more realistic control settings; to assess the quantitative impact of limited control resources and/or system knowledge; and to provide a rigorous and general foundation for existing experimental approaches in order to further enhance applicability and performance. From an experimental standpoint, renewed emphasis is in turn placed on validating theoretical predictions and benchmarking performance, so that the limiting constraints can be singled out for additional theoretical analysis and guidance. This ongoing cross-talk is clearly reflected in this collection, which brings together theoreticians and experimentalists, with a significant fraction of the papers reporting on combined quantum control theory–experiment efforts. While a precise categorization would neither be possible nor desirable, contributions to this volume have been loosely grouped into five broad sections. This grouping has been made in the hope that connections between different problems and/or technical approaches will become more transparent, facilitating the transfer of concepts and methods. The special issue opens with a section devoted to open-loop control methods, with special emphasis on dynamical decoupling (DD), which is becoming an increasingly important tool for decoherence control at the physical 'quantum firmware' level. In addition to including original research results, the first two articles, by Brion et al and Biercuk et al , also serve to pedagogically review some background in their respective subjects. In particular, Brion et al revisit one of the conceptually simplest approaches to open-loop manipulation of both closed and open quantum systems, nonholonomic control , motivated by its broad applicability to QIP settings. A special instance of open-loop control based on sequences of (nearly) instantaneous `bang-bang' pulses is addressed by Biercuk et al , who reformulate the simplest DD scenario, suppression of phase decoherence in a single qubit, as a filter-design problem. Peng et al report on the implementation of 'concatenated' DD for arbitrary single-qubit decoherence in the context of nuclear magnetic resonance QIP. A dedicated analysis of the performance of different DD schemes in the presence of realistic pulse errors is given by Wang and Dobrovitski. DD is also one of the strategies used by Lucamarini et al to reduce polarization decoherence in a photon qubit. These authors additionally report on the use of active feedback to counter transmission noise, effectively setting the stage for the second section, which is centered on closed-loop control. Unlike in open-loop control, measurement is an essential ingredient in closed-loop schemes aimed at both reliably identifying features of the target quantum system and further modifying its dynamics. The importance of directly measuring the spectrum of the underlying system-environment coupling is stressed by Almog et al , who show how this knowledge is crucial, in particular, for predicting the performance of DD sequences in experiments and for optimizing performance. Riofrio et al address a weak-measurement protocol for implementing quantum state tomography , which is a necessary 'primitive' for inferring the target quantum state and thereby diagnosing the control performance. Next, the impact of realistic control and system imperfections in continuous-time Markovian feedback strategies for rapid state preparation is analyzed by Combes and Wiseman. A prominent role is played in the special issue by optimal control (OC) approaches, reflecting their central importance for quantum control and QIP. The OC contributions have been divided into two separate sections, depending on whether the target dynamics is modeled as Hamiltonian (section 3) or dissipative (section 4), respectively. The contribution by Beltrani et al deals with `control landscapes', which provide a foundation for analyzing the performance of numerical OC algorithms and their robustness against control errors. Specifically, this paper characterizes geometric properties of the control landscape, relevant to the optimal control of state-to-state transitions. 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Alternative approaches for optimized control of qubits exposed to various decoherence processes are developed by Esher et al and Xue et al , based on a perturbative 'bath-optimized' formalism and on numerical optimization via a genetic algorithm, respectively. Testifying to the richness of the field, the volume concludes with four contributions that address a diverse range of problems. The exploitation of properties of adiabatic quantum evolutions is common to the first two papers. In particular, Legthtas et al offer a rigorous explanation for the robustness of a control protocol, chirped pulsing , that is widely employed in 'adiabatic rapid passage' experiments, while Han et al present a theoretical framework for adiabatic Raman photo-association schemes relevant to ultracold atomic systems. In the context of cavity quantum electrodynamics, Montenegro and Orszag describe how to engineer a system of two atoms coupled to distant lossy cavities so that stable atomic entanglement is generated. Finally, still very little is known about the physical mechanisms that are responsible for and control the experimentally observed 'coherent' features of transport phenomena in biological systems. The last contribution by Alicki and Giraldi analyzes energy transport in dynamical systems that can be modeled as 'quantum networks', and points to this fascinating emerging frontier. It is our hope that the above papers may help readers to gain an overview of some of the main trends in current quantum control efforts, both theoretical and experimental. In closing, we take the opportunity to thank the organizations which sponsored the above-mentioned ITAMP Topical Group (the United States National Science Foundation and Harvard University) and the Safed Workshop (the Israeli Science Foundation, the Safed Scientific Workshop program, CECAM and ACAM). Last but not least our sincere gratitude goes to all of the contributors to the volume and the reviewers as well as the J. Phys. B staff, for their respective efforts in preparing the papers and ensuring the overall quality of this special issue.

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The ability to optimally control quantum systems in the presence of environmentally-induced decoherence is important for many physical and chemical problems.We discuss both theoretical and experimental aspects of optimal control of open quantum systems. The theoretical analysis is based on fundamental concepts of open-system controllability and control landscapes. These theoretical advances lay the groundwork for practical applications, including numerical simulations and experimental implementations of adaptive feedback control. In particular, the adaptive approach was utilized to implement coherent control of decoherence, which uses coherent (unitary) preparation and manipulation of an open quantum system to significantly alter its incoherent (non-unitary) dynamics caused by coupling to an environment. We also discuss other applications, including optimal dynamic discrimination of similar quantum systems and optimal control of high-fidelity quantum gates in the presence of decoherence.

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Conventional approaches for controlling open quantum systems use coherent control which affects the system's evolution through the Hamiltonian part of the dynamics. Such control, although being extremely efficient for a large variety of problems, has limited capabilities, e.g., if the initial and desired target states have density matrices with different spectra or if a control field needs to be designed to optimally transfer different initial states to the same target state. Recent research works suggest extending coherent control by including active manipulation of the non-unitary (i.e., incoherent) part of the evolution. This paper summarizes recent results specifically for incoherent control by the environment (e.g., incoherent radiation or a gaseous medium) with a kinematic description of controllability and landscape analysis.

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Tunneling under Coherent Control by Sequences of Unitary Pulses

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A general coherent control scenario to suppress, or accelerate, tunneling of quantum states decaying into a continuum, is investigated. The method is based on deterministic, or stochastic, sequences of unitary pulses that affect the underlying interference phenomena responsible for quantum dynamics, without inducing decoherence, or collapsing the coherent evolution of the system. The influence of control sequences on the ensuing quantum dynamics is analyzed by using perturbation theory to first order in the control pulse fields and compared to dynamical decoupling (DD) protocols and sequences of pulses that collapse the coherent evolution and induce quantum Zeno (QZE) or quantum anti-Zeno effects (AZE). The analysis reveals a subtle interplay between coherent and incoherent phenomena and demonstrating that dynamics analogous to evolution due to QZE or AZE can be generated from stochastic sequences of unitary pulses when averaged over all possible realizations.

arXiv:1009.1403•Sep 7, 2010•0 citations

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Known as decoherence, the unavoidable interaction of a quantum system with its surrounding environment is usually considered to be detrimental for quantum information processing. In this thesis the coherent, open loop control of such open systems is studied. Concepts from quantum control theory and the theory of open quantum system are adopted in order to fight decoherence and implement quantum gates in a noiseless manner. In particular, Lie algebraic methods and numerical optimization tools are used to investigate the control properties of a single spin interacting with a spin environment. We show that, independent of the size of the environment, every unitary transformation can be implemented on the system spin through a single control field. We proceed by investigating dynamical decoupling, a method to suppress the interactions with the environment, for finite- and for in- finite dimensional systems. We prove that every finite dimensional system can be protected from decoherence, even if the environment is infinite dimensional, whereas for noise described by a Lindblad master equation dynamical decoupling will never succeed. This will lead to a new method to distinguish decoherence from intrinsic noise terms. We further prove that not every infinite dimensional system can be protected from decoherence through dynamical decoupling. Afterwards we investigate dynamical decoupling of systems that are described by quadratic Hamiltonians, showing that such interactions can always be suppressed with two simple operations. In the last part we investigate the coherent control of a Lindblad master equation. We show that a strong noise process exhibiting a decoherence free subspace can substantially increase the number of unitary operations that can be implemented, allowing us to fully control parts of the system. Afterwards we develop a scheme to make Hamiltonians and Lindbladians commutative by adding an auxiliary system. The old, possibly non-commutative dynamics, is recovered through a non-selective measurement.

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Coherence control was originally conceived by Shapiro and Brumer for closed quantum systems. In open quantum systems, the environment hampers or destroys coherence. Nevertheless, the Kurizki-Shapiro-Brumer coherent photocurrent control showed partial resilience to decoherence. Still, decoherence control is an essential prerequisite to our ability to fully exploit quantum coherence for any operational task. Yet decoherence control need not employ coherent fields: it may be incoherent. In operational tasks such as the preparation, transformation, transmission, and detection of quantumstates, environmental (bath) effects can be suppressed by dynamical decoupling, or by the more general incoherent dynamical control by modulation developed by our group. The resulting control dynamics must be Zeno-like in order to yield suppressed coupling to the bath in unitary operational tasks. There are however tasks which cannot be implemented by closed-system (unitary) evolution, in particular those involving a change of the system's entropy. Such tasks necessitate efficient coupling to a bath for their implementation. Examples are the use of measurements to cool (purify) a system, to equilibrate it, or harvest (and convert) energy from the environment. If the underlying dynamics is anti-Zeno like, enhancement of this coupling to the bath will occur and thereby facilitate the task, as discovered by us. A general task may also require state and energy transfer between non-interacting parties via shared modes of the bath. For such tasks, a more subtle interplay of Zeno and anti-Zeno dynamics may be optimal. We have therefore constructed a general framework for optimizing the way a system interacts with its environment to achieve a desired task. This optimization consists in adjusting a given “score” that quantifies the success of the task, such as the targeted fidelity, purity, entropy, energy or state transfer probability by dynamical modification of the system-bath coupling spectrum on demand.
Due to increasing demands on speed and security of data processing, along with requirements on measurement precision in fundamental research, quantum phenomena are expected to play an increasing role in future technologies. Special attention must hence be paid to omnipresent decoherence effects, which hamper quantumness. Their consequence is always a deviation of the quantum state evolution (error) with respect to the expected unitary evolution if these effects are absent. In operational tasks such as the preparation, transformation, transmission, and detection of quantum states, these effects are detrimental and must be suppressed by strategies known as dynamical decoupling, or the more general dynamical control by modulation developed by us. The underlying dynamics must be Zeno-like, yielding suppressed coupling to the bath. There are, however, tasks which cannot be implemented by unitary evolution, in particular those involving a change of the system’s state entropy. Such tasks necessitate efficient coupling to a bath for their implementation. Examples include the use of measurements to cool (purify) a system, to equilibrate it, or to harvest and convert energy from the environment. If the underlying dynamics is anti-Zeno like, enhancement of this coupling to the bath will occur and thereby facilitate the task, as discovered by us. A general task may also require state and energy transfer, or entanglement of noninteracting parties via shared modes of the bath which call for maximizing the shared (two-partite) couplings with the bath, but suppressing the single-partite couplings. For such tasks, a more subtle interplay of Zeno and anti-Zeno dynamics may be optimal. We have therefore constructed a general framework for optimizing the way a system interacts with its environment to achieve a desired task. This optimization consists in adjusting a given “score” that quantifies the success of the task, such as the targeted fidelity, purity, entropy, entanglement, or energy by dynamical modification of the system-bath coupling spectrum on demand.
Precisely characterizing and controlling the dynamics of realistic open quantum systems has emerged in recent years as a key challenge across contemporary quantum sciences and technologies, with implications ranging from physics, chemistry and applied mathematics to quantum information processing (QIP) and quantum engineering. Quantum control theory aims to provide both a general dynamical-system framework and a constructive toolbox to meet this challenge. The purpose of this special issue of Journal of Physics B: Atomic, Molecular and Optical Physics is to present a state-of-the-art account of recent advances and current trends in the field, as reflected in two international meetings that were held on the subject over the last summer and which motivated in part the compilation of this volume—the Topical Group: Frontiers in Open Quantum Systems and Quantum Control Theory , held at the Institute for Theoretical Atomic, Molecular and Optical Physics (ITAMP) in Cambridge, Massachusetts (USA), from 1–14 August 2010, and the Safed Workshop on Quantum Decoherence and Thermodynamics Control , held in Safed (Israel), from 22–27 August 2010. Initial developments in quantum control theory date back to (at least) the early 1980s, and have been largely inspired by the well-established mathematical framework for classical dynamical systems. As the above-mentioned meetings made clear, and as the burgeoning body of literature on the subject testifies, quantum control has grown since then well beyond its original boundaries, and has by now evolved into a highly cross-disciplinary field which, while still fast-moving, is also entering a new phase of maturity, sophistication, and integration. Two trends deserve special attention: on the one hand, a growing emphasis on control tasks and methodologies that are specifically motivated by QIP, in addition and in parallel to applications in more traditional areas where quantum coherence is nevertheless vital (such as, for instance, quantum control of chemical reactions or high-resolution magnetic resonance spectroscopy); on the other hand, an unprecedented demand for close coupling between theory and experiment , with theoretical developments becoming more and more attuned to and driven by experimental advances as different quantum technologies continue to evolve at an impressive pace in the laboratory. Altogether, these two trends account for several of the recurrent themes in this volume, as well as in the current quantum control literature as a whole: namely, the quest for control strategies that can attain the highest degree of precision and robustness possible, while striving for efficiency and, ultimately, optimality in achieving the intended control task under realistic operational constraints. From a theory standpoint, this makes it imperative to take into account increasingly more realistic control settings; to assess the quantitative impact of limited control resources and/or system knowledge; and to provide a rigorous and general foundation for existing experimental approaches in order to further enhance applicability and performance. From an experimental standpoint, renewed emphasis is in turn placed on validating theoretical predictions and benchmarking performance, so that the limiting constraints can be singled out for additional theoretical analysis and guidance. This ongoing cross-talk is clearly reflected in this collection, which brings together theoreticians and experimentalists, with a significant fraction of the papers reporting on combined quantum control theory–experiment efforts. While a precise categorization would neither be possible nor desirable, contributions to this volume have been loosely grouped into five broad sections. This grouping has been made in the hope that connections between different problems and/or technical approaches will become more transparent, facilitating the transfer of concepts and methods. The special issue opens with a section devoted to open-loop control methods, with special emphasis on dynamical decoupling (DD), which is becoming an increasingly important tool for decoherence control at the physical 'quantum firmware' level. In addition to including original research results, the first two articles, by Brion et al and Biercuk et al , also serve to pedagogically review some background in their respective subjects. In particular, Brion et al revisit one of the conceptually simplest approaches to open-loop manipulation of both closed and open quantum systems, nonholonomic control , motivated by its broad applicability to QIP settings. A special instance of open-loop control based on sequences of (nearly) instantaneous `bang-bang' pulses is addressed by Biercuk et al , who reformulate the simplest DD scenario, suppression of phase decoherence in a single qubit, as a filter-design problem. Peng et al report on the implementation of 'concatenated' DD for arbitrary single-qubit decoherence in the context of nuclear magnetic resonance QIP. A dedicated analysis of the performance of different DD schemes in the presence of realistic pulse errors is given by Wang and Dobrovitski. DD is also one of the strategies used by Lucamarini et al to reduce polarization decoherence in a photon qubit. These authors additionally report on the use of active feedback to counter transmission noise, effectively setting the stage for the second section, which is centered on closed-loop control. Unlike in open-loop control, measurement is an essential ingredient in closed-loop schemes aimed at both reliably identifying features of the target quantum system and further modifying its dynamics. The importance of directly measuring the spectrum of the underlying system-environment coupling is stressed by Almog et al , who show how this knowledge is crucial, in particular, for predicting the performance of DD sequences in experiments and for optimizing performance. Riofrio et al address a weak-measurement protocol for implementing quantum state tomography , which is a necessary 'primitive' for inferring the target quantum state and thereby diagnosing the control performance. Next, the impact of realistic control and system imperfections in continuous-time Markovian feedback strategies for rapid state preparation is analyzed by Combes and Wiseman. A prominent role is played in the special issue by optimal control (OC) approaches, reflecting their central importance for quantum control and QIP. The OC contributions have been divided into two separate sections, depending on whether the target dynamics is modeled as Hamiltonian (section 3) or dissipative (section 4), respectively. The contribution by Beltrani et al deals with `control landscapes', which provide a foundation for analyzing the performance of numerical OC algorithms and their robustness against control errors. Specifically, this paper characterizes geometric properties of the control landscape, relevant to the optimal control of state-to-state transitions. Application of OC theory to the problem of population transfer and coherence enhancement in Λ-systems is studied by Kumar et al , whereas Goerz et al report on the OC-design of a high-fidelity controlled phase-gate in atomic qubits. The robustness of an OC solution is specifically addressed by Negretti et al , along with an approach for identifying easily implementable while still 'close-to-optimal' control pulses. Powerful relaxation-optimized OC schemes (based on so-called opengrape algorithms) for generating unitary target gates in the presence of known dissipation parameters are discussed by Schulte-Herbrüggen et al . Next, Lapert et al report on the problem of time-optimal control of spin-1/2 systems undergoing Bloch relaxation dynamics, highlighting the crucial role played by singular extremals in the control synthesis. Alternative approaches for optimized control of qubits exposed to various decoherence processes are developed by Esher et al and Xue et al , based on a perturbative 'bath-optimized' formalism and on numerical optimization via a genetic algorithm, respectively. Testifying to the richness of the field, the volume concludes with four contributions that address a diverse range of problems. The exploitation of properties of adiabatic quantum evolutions is common to the first two papers. In particular, Legthtas et al offer a rigorous explanation for the robustness of a control protocol, chirped pulsing , that is widely employed in 'adiabatic rapid passage' experiments, while Han et al present a theoretical framework for adiabatic Raman photo-association schemes relevant to ultracold atomic systems. In the context of cavity quantum electrodynamics, Montenegro and Orszag describe how to engineer a system of two atoms coupled to distant lossy cavities so that stable atomic entanglement is generated. Finally, still very little is known about the physical mechanisms that are responsible for and control the experimentally observed 'coherent' features of transport phenomena in biological systems. The last contribution by Alicki and Giraldi analyzes energy transport in dynamical systems that can be modeled as 'quantum networks', and points to this fascinating emerging frontier. It is our hope that the above papers may help readers to gain an overview of some of the main trends in current quantum control efforts, both theoretical and experimental. In closing, we take the opportunity to thank the organizations which sponsored the above-mentioned ITAMP Topical Group (the United States National Science Foundation and Harvard University) and the Safed Workshop (the Israeli Science Foundation, the Safed Scientific Workshop program, CECAM and ACAM). Last but not least our sincere gratitude goes to all of the contributors to the volume and the reviewers as well as the J. Phys. B staff, for their respective efforts in preparing the papers and ensuring the overall quality of this special issue.
The ability to optimally control quantum systems in the presence of environmentally-induced decoherence is important for many physical and chemical problems.We discuss both theoretical and experimental aspects of optimal control of open quantum systems. The theoretical analysis is based on fundamental concepts of open-system controllability and control landscapes. These theoretical advances lay the groundwork for practical applications, including numerical simulations and experimental implementations of adaptive feedback control. In particular, the adaptive approach was utilized to implement coherent control of decoherence, which uses coherent (unitary) preparation and manipulation of an open quantum system to significantly alter its incoherent (non-unitary) dynamics caused by coupling to an environment. We also discuss other applications, including optimal dynamic discrimination of similar quantum systems and optimal control of high-fidelity quantum gates in the presence of decoherence.
Conventional approaches for controlling open quantum systems use coherent control which affects the system's evolution through the Hamiltonian part of the dynamics. Such control, although being extremely efficient for a large variety of problems, has limited capabilities, e.g., if the initial and desired target states have density matrices with different spectra or if a control field needs to be designed to optimally transfer different initial states to the same target state. Recent research works suggest extending coherent control by including active manipulation of the non-unitary (i.e., incoherent) part of the evolution. This paper summarizes recent results specifically for incoherent control by the environment (e.g., incoherent radiation or a gaseous medium) with a kinematic description of controllability and landscape analysis.
A general coherent control scenario to suppress, or accelerate, tunneling of quantum states decaying into a continuum, is investigated. The method is based on deterministic, or stochastic, sequences of unitary pulses that affect the underlying interference phenomena responsible for quantum dynamics, without inducing decoherence, or collapsing the coherent evolution of the system. The influence of control sequences on the ensuing quantum dynamics is analyzed by using perturbation theory to first order in the control pulse fields and compared to dynamical decoupling (DD) protocols and sequences of pulses that collapse the coherent evolution and induce quantum Zeno (QZE) or quantum anti-Zeno effects (AZE). The analysis reveals a subtle interplay between coherent and incoherent phenomena and demonstrating that dynamics analogous to evolution due to QZE or AZE can be generated from stochastic sequences of unitary pulses when averaged over all possible realizations.
Known as decoherence, the unavoidable interaction of a quantum system with its surrounding environment is usually considered to be detrimental for quantum information processing. In this thesis the coherent, open loop control of such open systems is studied. Concepts from quantum control theory and the theory of open quantum system are adopted in order to fight decoherence and implement quantum gates in a noiseless manner. In particular, Lie algebraic methods and numerical optimization tools are used to investigate the control properties of a single spin interacting with a spin environment. We show that, independent of the size of the environment, every unitary transformation can be implemented on the system spin through a single control field. We proceed by investigating dynamical decoupling, a method to suppress the interactions with the environment, for finite- and for in- finite dimensional systems. We prove that every finite dimensional system can be protected from decoherence, even if the environment is infinite dimensional, whereas for noise described by a Lindblad master equation dynamical decoupling will never succeed. This will lead to a new method to distinguish decoherence from intrinsic noise terms. We further prove that not every infinite dimensional system can be protected from decoherence through dynamical decoupling. Afterwards we investigate dynamical decoupling of systems that are described by quadratic Hamiltonians, showing that such interactions can always be suppressed with two simple operations. In the last part we investigate the coherent control of a Lindblad master equation. We show that a strong noise process exhibiting a decoherence free subspace can substantially increase the number of unitary operations that can be implemented, allowing us to fully control parts of the system. Afterwards we develop a scheme to make Hamiltonians and Lindbladians commutative by adding an auxiliary system. The old, possibly non-commutative dynamics, is recovered through a non-selective measurement.