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arXiv:1007.4425

Influence of diffusion of atoms on the dark resonance lineshape in spatially bounded laser fields

V. I. Romanenko, Alexander Romanenko, Леонід Петрович Яценко

Published Jul 26, 2010• 0 citations
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Abstract

We propose a diffusion model for the recently discovered diffusion-induced Ramsey narrowing arising when atoms diffuse in a buffer-gas cell in the laser radiation field. The diffusion equation for the coherence of metastable states coupled with an excited state by laser radiation of different frequencies in a three-level scheme of the atom-field interaction is obtained in the strong-collision approximation. The dependence of the shape of an absorption line near the transmission maximum of one of the frequencies on the two-photon resonance detuning for various geometries of the cell is investigated.

DOI
10.48550/arxiv.1007.4425

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We propose a diffusion model for the recently discovered diffusion-induced Ramsey narrowing arising when atoms diffuse in a buffer-gas cell in the laser radiation field. The diffusion equation for the coherence of metastable states coupled with an excited state by laser radiation of different frequencies in a three-level scheme of the atom-field interaction is obtained in the strong-collision approximation. The dependence of the shape of an absorption line near the transmission maximum of one of the frequencies on the two-photon resonance detuning for various geometries of the cell is investigated.
In a recent paper [Y. Xiao et al., Phys. Rev. Lett. 96, 043601 (2006)] we characterized diffusion-induced Ramsey narrowing as a general phenomenon, in which diffusion of coherence in-and-out of an interaction region such as a laser beam induces spectral narrowing of the associated resonance lineshape. Here we provide a detailed presentation of the repeated interaction model of diffusion-induced Ramsey narrowing, with particular focus on its application to Electromagnetically Induced Transparency (EIT) of atomic vapor in a buffer gas cell. We compare this model both to experimental data and numerical calculations.
Abstract We report on a theoretical model of the effect of coherent population trapping in alkali atoms in an optically thin gas cell with a buffer gas at a nonzero temperature in a pulsed laser field. The shape of the Ramsey resonance is analysed for two different temperature ranges, i. e. for a ‘cold’ atomic ensemble and for an ensemble of ‘hot’ atoms in a cell with a buffer gas. The influence of the hyperfine structure of the excited level on the shift of the central Ramsey resonance is investigated.
We experimentally investigated the characteristics of two-photon transmission resonances in Rb vapor cells with different amounts of buffer gas under the conditions of steady-state coherent population trapping (CPT) and a pulsed Raman–Ramsey (RR) CPT interrogation scheme. We particularly focused on the influence of the Rb atoms diffusing in and out of the laser beam. We showed that this effect modifies the shape of both CPT and RR resonances as well as their projected performance for CPT clock applications. In particular we found that at moderate buffer gas pressures RR-CPT did not improve the projected atomic clock stability compared to the regular steady-state CPT resonance.
An analysis of near-resonant collisions between dissimilar atoms in the presence of a radiation field reveals their effect on the far wings of the absorption profile. Extending a model due to Cavalieri, Arimondo, and Matera, we take into account the collisional shifts of atomic levels, as well as the collisional coupling between atoms and the coupling with the radiation field. A general formula for the absorption profile is derived and expressed in terms of the universal line-shape function of the unified Franck-Condon treatment of pressure broadening. We show that in some cases collision-induced coherence can give rise to a strongly depressed red wing that exhibits transparency for some values of the laser detuning. \textcopyright{} 1996 The American Physical Society.
We study laser-induced transparency and dark-line effects in a two-level atomic system where the upper transition level is coupled by a laser field to a dressed system consisting of two lower-energy metastable states mixed by a second laser field (\ensuremath{\Pi} configuration). We show that the emission (absorption) spectrum of the two-level system develops two dynamic dark lines (transparency holes) with tunable central frequencies equal to the Rabi frequency of the second field with positive and negative signs, and widths proportional to that of the first field. The detailed evolution of these effects at low- and high-field intensities and the role of quantum interferences are discussed by presenting a model based on laser-induced continuum structure and adopting a dressed-state picture. We discuss various nonlinear processes in this system and show how the dynamics of emission and absorption spectra are determined by one- and two-photon coupling processes.