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arXiv:1511.07550 · Journal of the Optical Society of America B

Effect of atomic diffusion on the Raman–Ramsey coherent population trapping resonances

Elena Kuchina, Eugeniy E. Mikhailov, Irina V. Novikova

Published Mar 10, 2016• 9 citations
arXivHTMLPDF

Abstract

We experimentally investigated the characteristics of two-photon transmission resonances in Rb vapor cells with different amounts of buffer gas under the conditions of steady-state coherent population trapping (CPT) and a pulsed Raman–Ramsey (RR) CPT interrogation scheme. We particularly focused on the influence of the Rb atoms diffusing in and out of the laser beam. We showed that this effect modifies the shape of both CPT and RR resonances as well as their projected performance for CPT clock applications. In particular we found that at moderate buffer gas pressures RR-CPT did not improve the projected atomic clock stability compared to the regular steady-state CPT resonance.

DOI
10.1364/josab.33.000610

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A gas cell atomic frequency standard based on coherent population trapping (CPT) with Ramsey interrogation pulses is developed. The clock resonance is detected in a Cs cell with buffer gas using two phase-locked diode lasers tuned to the D1 line. A preliminary short-term stability of3.5×10−12t−1/23.5 \times 10^{-12}t^{-1/2}3.5×10−12t−1/2is reported. The CPT specificity allows a new interrogation–detection sequence, i.e., the continuous pulse train, which, with phase modulation, could lead to better short-term stability compared to usual continuous CPT clocks. The parameters optimizing the stability include a high Rabi frequency, a very short measurement time, and an interrogation time equal to the lifetime of the hyperfine coherence.
We report the results of experimental investigation of the Raman – Ramsey method of pulsed excitation of coherent population trapping (CPT) resonances in a rubidium vapour cell filled with a mixture of Ar and Ne buffer gases. For the development of compact quantum microwave frequency standards, this method is an alternative to the pulsed optical pumping method recently implemented using the same rubidium cell. Both methods have advantages over the traditional double radio-optical resonance technique, the main of which is the substantial suppression of the light shift of the clock transition frequency, since the evolution of the coherence of atomic states forming the clock transition occurs in the absence of laser radiation in the cell. The narrow (110 – 240 Hz) Raman – Ramsey resonances are obtained using the scheme of pulsed excitation of CPT resonances on the D 1 lines of the 87 Rb atom with the same linear (lin||lin) polarisations of the bichromatic laser radiation components. The process of optimising the central fringe linewidth, its contrast, and the linewidth-to-contrast ratio is described. The magnetic dependence of the Raman – Ramsey line central fringe linewidth is experimentally investigated.
We propose a two-step pulse observation method to enhance the frequency stability of coherent population trapping (CPT) atomic clocks. The proposed method is a Raman–Ramsey scheme with low light intensity at resonance observation and provides a Ramsey-CPT resonance with both reduced frequency sensitivity to the light intensity and a high signal-to-noise ratio by reducing the repumping into a steady dark state. The resonance characteristics were calculated using density matrix analysis of a Λ-type three-level system that was modeled on the 133 Cs D 1 line, and the characteristics were also measured using a vertical-cavity surface-emitting laser and a Cs vapor cell.
The phenomenon of all-optical Ramsey interference using pulsed coherent population trapping (CPT) beams provides a new avenue for developing frequency standards using atomic vapor. In this study, we show that frequency narrowed Ramsey fringes can be produced in rubidium vapor without the effect of power broadening. We observed fringes of width as narrow as 1 kHz using a buffer-gas filled rubidium cell. A compact injection-locked laser (ILL) system was used to generate CPT beams. Studies also show that ac Stark effect on Ramsey fringes can be reduced, and higher frequency stability can be achieved in a clock application. The results are encouraging to propose an architecture for development of a pulsed CPT Ramsey clock. In this paper, we also provide related discussions on clock frequency stability, and our plans for future experiments.
Vapor cell atomic clocks exhibit reduced frequency stability for averaging time between about one hundred and a few thousand seconds. Here we report a study on the impact of the main parameters on the mid-to-long term instability of a buffer-gas vapor cell Cs clock, based on coherent population trapping (CPT). The CPT signal is observed on the Cs D1 line transmission, using a double Λ scheme and a Ramsey interrogation technique. The effects on the clock frequency of the magnetic field, the cell temperature, and the laser intensities are reported. We show in particular that the laser intensity shift is temperature dependent. Along with the laser intensity ratio and laser polarization properties, this is one of the most important parameters.
SummaryWe investigated the Ramsey–coherent population trapping (CPT) characteristics of a new observation method that employs different laser sideband combinations as the two interrogation pulses during Ramsey–CPT resonance observation. In an experimental setup using a gas cell containing Cs atoms, Ramsey–CPT resonance was observed using the 1st-1stsideband combination for the common preparation pulse and the 1st-1stand C-2nd sideband combinations for the detection pulse. The Ramsey–CPT spectral shapes were inverted to each other. The light shift characteristic was 2.7 times different to its light sensitivity. This difference in the light shift characteristics is expected to allow the estimation of the light frequency shift in the Ramsey–CPT atomic clock during operation.