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arXiv:1007.1481 · Physical Review A

Measurement of the Landé g factor of the 5D5/2 state of Ba ii with a single trapped ion

Nathan Kurz, Matthew Dietrich, Gang Shu, T. Noel, B. B. Blinov

Published Sep 27, 2010• 6 citations
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Abstract

We present a terrestrial measurement of the Land\'e $g$ factor of the $5{D}_{5/2}$ state of singly ionized barium. Measurements were performed on single Doppler-cooled ${}^{138}{\mathrm{Ba}}^{+}$ ions in a linear Paul trap. A frequency-stabilized fiber laser with a nominal wavelength of $1.762$ $\ensuremath{\mu}$m was scanned across the $6{S}_{1/2}\ensuremath{\leftrightarrow}5{D}_{5/2}$ transition to spectroscopically resolve transitions between Zeeman sublevels of the ground and excited states. From the relative positions of the four narrow transitions observed at several different values for the applied magnetic field, we find a value of $1.2020\ifmmode\pm\else\textpm\fi{}0.0005$ for ${g}_{5{D}_{5/2}}$.

DOI
10.1103/physreva.82.030501

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We report an improved measurement of the Land\'e ${g}_{J}$ factor of the $5{D}_{5/2}$ state of singly ionized barium. Measurements were performed on single Doppler-cooled ${}^{138}$Ba${}^{+}$ ions in linear Paul traps using two similar, independent apparatuses. Transitions between Zeeman sublevels of the $6{S}_{1/2}$ and $5{D}_{5/2}$ states were driven with two independent, stabilized radio-frequency synthesizers using a dedicated electrode within each ion trap chamber. State detection within each Zeeman manifold was achieved with a frequency-stabilized fiber laser operating at 1.76 $\ensuremath{\mu}$m. By calculating the ratio of the two Zeeman splittings, and using the measured Land\'e ${g}_{J}$ factor of the $6{S}_{1/2}$ state, we find a value of 1.200 372$({4}_{\mathrm{stat}})({7}_{\mathrm{sys}})$ for ${g}_{{D}_{5/2}}$.

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Measurement of the $^{138}{\mathrm{Ba}}^{+}$ ${^{2}S}_{1/2}\ensuremath{-}{^{2}D}_{5/2}$ clock transition frequency and ${D}_{5/2}$ Land\'e ${g}_{J}$ factor are reported. The clock transition frequency ${\ensuremath{\nu}}_{{\mathrm{Ba}}^{+}}=170126432449333.31\ifmmode\pm\else\textpm\fi{}(0.39{)}_{\mathrm{stat}}\ifmmode\pm\else\textpm\fi{}(0.29{)}_{\mathrm{sys}}\text{ }\text{ }\mathrm{Hz}$, is obtained with accuracy limited by the frequency calibration of the maser used as a reference oscillator. The Land\'e ${g}_{J}$ factor for the ${^{2}D}_{5/2}$ level is determined to be ${g}_{D}=1.20036739(24)$, which is a 30-fold improvement on previous measurements. The $g$-factor measurements are corrected for an ac-magnetic field from trap-drive-induced currents in the electrodes, and data taken over a range of magnetic fields underscores the importance of accounting for this systematic.

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Coherent excitation of the 6S1/2 to 5D3/2 electric-quadrupole transition in 138 Ba +

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The electric dipole-forbidden, quadrupole $6{S}_{1/2}\ensuremath{\leftrightarrow}5{D}_{3/2}$ transition in Ba${}^{+}$ near 2051 nm, with a natural linewidth of 13 mHz, is attractive for potential observation of parity nonconservation, and also as a clock transition for a barium ion optical frequency standard. This transition also offers a direct means of populating the metastable $5{D}_{3/2}$ state to measure the nuclear magnetic octupole moment in the odd barium isotopes. Light from a diode-pumped, solid-state Tm,Ho:YLF laser operating at 2051 nm is used to coherently drive this transition between resolved Zeeman levels in a single trapped ${}^{138}$Ba${}^{+}$ ion. The frequency of the laser is stabilized to a high-finesse Fabry-P\'erot cavity at 1025 nm after being frequency doubled. Rabi oscillations on this transition indicate a laser-ion coherence time of 3 ms, most likely limited by ambient magnetic field fluctuations.

arXiv:1203.1978•Physical Review A•Apr 20, 2012•14 citations
We present a terrestrial measurement of the Land'e ggg factor of the 5D5/25{D}_{5/2}5D5/2​ state of singly ionized barium. Measurements were performed on single Doppler-cooled 138Ba+{}^{138}{\mathrm{Ba}}^{+}138Ba+ ions in a linear Paul trap. A frequency-stabilized fiber laser with a nominal wavelength of 1.7621.7621.762 \ensuremathμ\ensuremath{\mu}\ensuremathμm was scanned across the 6S1/2\ensuremath↔5D5/26{S}_{1/2}\ensuremath{\leftrightarrow}5{D}_{5/2}6S1/2​\ensuremath↔5D5/2​ transition to spectroscopically resolve transitions between Zeeman sublevels of the ground and excited states. From the relative positions of the four narrow transitions observed at several different values for the applied magnetic field, we find a value of 1.2020\ifmmode±\else\textpm\fi0.00051.2020\ifmmode\pm\else\textpm\fi{}0.00051.2020\ifmmode±\else\textpm\fi0.0005 for g5D5/2{g}_{5{D}_{5/2}}g5D5/2​​.
We report an improved measurement of the Land\'e gJ{g}_{J}gJ​ factor of the 5D5/25{D}_{5/2}5D5/2​ state of singly ionized barium. Measurements were performed on single Doppler-cooled 138{}^{138}138Ba+{}^{+}+ ions in linear Paul traps using two similar, independent apparatuses. Transitions between Zeeman sublevels of the 6S1/26{S}_{1/2}6S1/2​ and 5D5/25{D}_{5/2}5D5/2​ states were driven with two independent, stabilized radio-frequency synthesizers using a dedicated electrode within each ion trap chamber. State detection within each Zeeman manifold was achieved with a frequency-stabilized fiber laser operating at 1.76 $\ensuremath{\mu}$m. By calculating the ratio of the two Zeeman splittings, and using the measured Land\'e gJ{g}_{J}gJ​ factor of the 6S1/26{S}_{1/2}6S1/2​ state, we find a value of 1.200 372(4stat)(7sys)({4}_{\mathrm{stat}})({7}_{\mathrm{sys}})(4stat​)(7sys​) for gD5/2{g}_{{D}_{5/2}}gD5/2​​.
Dual-Platform Precision Measurement of the 32D5/23^2D_{5/2}32D5/2​ to 42S1/24^2S_{1/2}42S1/2​ ggg-Factor Ratio in 40Ca+^{40}\text{Ca}^+40Ca+
We report precision measurements of the ratio of Landé ggg factors between the 32D5/23^2D_{5/2}32D5/2​ and 42S1/24^2S_{1/2}42S1/2​ states of a single trapped 40Ca+^{40}\text{Ca}^+40Ca+ ion. The measurements are performed in two distinct ion trap apparatus: a cryogenic surface electrode radiofrequency Paul trap and a room-temperature permanent magnet Penning trap. The Penning trap measurements rely on resonant microwave excitation of magnetic sublevels and yield a ratio of 0.599 488 813 3(2)0.599~488~813~3(2)0.599 488 813 3(2), which is a more than 40-fold uncertainty reduction compared to previous work. The radiofrequency trap measurements utilize optical electric quadrupole transitions and yield a concurring value of 0.599 488 813(6)0.599~488~813(6)0.599 488 813(6). We estimate that systematic shifts for each system are well below the respective statistical uncertainty.
Regarding microwave frequency standards based on trapped ions, we report on the determination of the hyperfine splittings and the Land\'e gJ{g}_{J}gJ​ factors of 111,113Cd+^{111,113}\mathrm{Cd}^{+}111,113Cd+. The hyperfine splittings and Land\'e gJ{g}_{J}gJ​ factors of the 5s2S1/25s{\phantom{\rule{0.16em}{0ex}}}^{2}{S}_{1/2}5s2S1/2​ and 5p2P1/2,3/25p{\phantom{\rule{0.16em}{0ex}}}^{2}{P}_{1/2,3/2}5p2P1/2,3/2​ states of 111,113Cd+^{111,113}\mathrm{Cd}^{+}111,113Cd+ are calculated using the multiconfiguration Dirac-Hartree-Fock scheme. Furthermore, the hyperfine splittings of the 5p2P3/25p{\phantom{\rule{0.16em}{0ex}}}^{2}{P}_{3/2}5p2P3/2​ state of 111,113Cd+^{111,113}\mathrm{Cd}^{+}111,113Cd+ are derived based on the laser-induced fluorescence spectroscopy. The Cd+{\mathrm{Cd}}^{+}Cd+ ions are confined in a linear Paul trap and sympathetically cooled by laser-cooled Ca+{\mathrm{Ca}}^{+}Ca+ ions. The calculated values and the derived values are cross-checked, thereby guaranteeing the reliability of our results. The results provided in this paper can improve the signal-to-noise ratio of the clock transition and the accuracy of the second-order Zeeman shift correction, thus further improving the stability and accuracy of the microwave frequency standards based on trapped 111,113Cd+^{111,113}\mathrm{Cd}^{+}111,113Cd+ ions.
Measurement of the 138Ba+^{138}{\mathrm{Ba}}^{+}138Ba+ ${^{2}S}_{1/2}\ensuremath{-}{^{2}D}_{5/2}$ clock transition frequency and D5/2{D}_{5/2}D5/2​ Land\'e gJ{g}_{J}gJ​ factor are reported. The clock transition frequency ${\ensuremath{\nu}}_{{\mathrm{Ba}}^{+}}=170126432449333.31\ifmmode\pm\else\textpm\fi{}(0.39{)}_{\mathrm{stat}}\ifmmode\pm\else\textpm\fi{}(0.29{)}_{\mathrm{sys}}\text{ }\text{ }\mathrm{Hz}$, is obtained with accuracy limited by the frequency calibration of the maser used as a reference oscillator. The Land\'e gJ{g}_{J}gJ​ factor for the 2D5/2{^{2}D}_{5/2}2D5/2​ level is determined to be gD=1.20036739(24){g}_{D}=1.20036739(24)gD​=1.20036739(24), which is a 30-fold improvement on previous measurements. The ggg-factor measurements are corrected for an ac-magnetic field from trap-drive-induced currents in the electrodes, and data taken over a range of magnetic fields underscores the importance of accounting for this systematic.
The Zeeman splitting of the metastable 5D3/2{\mathit{D}}_{3/2}D3/2​ level of 138Ba+^{138}\mathrm{Ba}^{+}138Ba+ in a magnetic field of 6 T has been measured in a laser-microwave double resonance experiment in a Penning ion trap. The magnetic field at the ion's position is determined by the cyclotron frequency of electrons stored in the same trap. From the ratio of both transition frequencies we obtain a gJ{\mathit{g}}_{\mathit{J}}gJ​ value of 0.799 327 8(3). As a by-product, we confirmed earlier measurements on the 6S1/2{\mathit{S}}_{1/2}S1/2​ ground-state gJ{\mathit{g}}_{\mathit{J}}gJ​ factor to 2.002 492 2(10). The precision in both experiments is sufficient to test relativistic many-body calculations. \textcopyright{} 1996 The American Physical Society.
The electric dipole-forbidden, quadrupole $6{S}_{1/2}\ensuremath{\leftrightarrow}5{D}_{3/2}$ transition in Ba+{}^{+}+ near 2051 nm, with a natural linewidth of 13 mHz, is attractive for potential observation of parity nonconservation, and also as a clock transition for a barium ion optical frequency standard. This transition also offers a direct means of populating the metastable 5D3/25{D}_{3/2}5D3/2​ state to measure the nuclear magnetic octupole moment in the odd barium isotopes. Light from a diode-pumped, solid-state Tm,Ho:YLF laser operating at 2051 nm is used to coherently drive this transition between resolved Zeeman levels in a single trapped 138{}^{138}138Ba+{}^{+}+ ion. The frequency of the laser is stabilized to a high-finesse Fabry-P\'erot cavity at 1025 nm after being frequency doubled. Rabi oscillations on this transition indicate a laser-ion coherence time of 3 ms, most likely limited by ambient magnetic field fluctuations.