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arXiv:1004.0198 · Physical Review B

Separation-dependent localization in a two-impurity spin-boson model

Dara P. S. McCutcheon, Ahsan Nazir, Sougato Bose, Andrew J. Fisher

Published Jun 18, 2010• 37 citations
arXivHTMLPDF

Abstract

Using a variational approach we investigate the delocalized to localized crossover in the ground state of an Ohmic two-impurity spin-boson model, describing two otherwise noninteracting spins coupled to a common bosonic environment. We show that a competition between an environment-induced Ising spin interaction and externally applied fields leads to variations in the system-bath coupling strength, ${\ensuremath{\alpha}}_{c}$, at which the delocalized-localized crossover occurs. Specifically, the crossover regime lies between ${\ensuremath{\alpha}}_{c}=0.5$ and ${\ensuremath{\alpha}}_{c}=1$ depending upon the spin separation and the strength of the transverse tunneling field. This is in contrast to the analogous single-spin case, for which the crossover occurs (in the scaling limit) at fixed ${\ensuremath{\alpha}}_{c}\ensuremath{\approx}1$. We also discuss links between the two-impurity spin-boson model and a dissipative two-spin transverse Ising model, showing that the latter possesses the same qualitative features as the Ising strength is varied. Finally, we show that signatures of the crossover may be observed in single impurity observables, as well as in the behavior of the system-environment entanglement.

DOI
10.1103/physrevb.81.235321

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Using a variational approach we investigate the delocalized to localized crossover in the ground state of an Ohmic two-impurity spin-boson model, describing two otherwise noninteracting spins coupled to a common bosonic environment. We show that a competition between an environment-induced Ising spin interaction and externally applied fields leads to variations in the system-bath coupling strength, \ensuremathαc{\ensuremath{\alpha}}_{c}\ensuremathαc​, at which the delocalized-localized crossover occurs. Specifically, the crossover regime lies between \ensuremathαc=0.5{\ensuremath{\alpha}}_{c}=0.5\ensuremathαc​=0.5 and \ensuremathαc=1{\ensuremath{\alpha}}_{c}=1\ensuremathαc​=1 depending upon the spin separation and the strength of the transverse tunneling field. This is in contrast to the analogous single-spin case, for which the crossover occurs (in the scaling limit) at fixed \ensuremathαc\ensuremath≈1{\ensuremath{\alpha}}_{c}\ensuremath{\approx}1\ensuremathαc​\ensuremath≈1. We also discuss links between the two-impurity spin-boson model and a dissipative two-spin transverse Ising model, showing that the latter possesses the same qualitative features as the Ising strength is varied. Finally, we show that signatures of the crossover may be observed in single impurity observables, as well as in the behavior of the system-environment entanglement.
We investigate quantum impurity problems, where a local magnetic moment is coupled to the spin density of a bosonic environment, leading to bosonic versions of the standard Kondo and Anderson impurity models. In a physical situation, these bosonic environments can correspond either to deconfined spinons in certain classes of Z2{Z}_{2}Z2​ frustrated antiferromagnets, or to particles in a multicomponent Bose gase (in which case the spin degree of freedom is attributed to hyperfine levels). Using renormalization group techniques, we establish that our impurity models, which feature an exchange interaction analogous to Kondo impurities in Fermi liquids, allow flow toward a stable strong-coupling state. Since the low-energy bosons exist around a single point in momentum space, and there is no Fermi surface, an impurity quantum phase transition occurs at intermediate coupling, separating screened and unscreened phases. This behavior is qualitatively different from previously studied spin-isotropic variants of the spin-boson model, which display stable intermediate-coupling fixed points and no screening.
We investigate the entanglement between a spin and its environment in impurity systems which exhibit a second-order quantum phase transition separating a delocalized and a localized phase for the spin. As an application, we employ the spin-boson model, describing a two-level system (spin) coupled to a sub-Ohmic bosonic bath with power-law spectral density, J(omega) proportional to omega(s) and 0 < s < 1. Combining Wilson's numerical renormalization group method and hyperscaling relations, we demonstrate that the entanglement between the spin and its environment is always enhanced at the quantum phase transition resulting in a visible cusp (maximum) in the entropy of entanglement. We formulate a correspondence between criticality and impurity entanglement entropy, and the relevance of these ideas to nanosystems is outlined.
We study the competition between Kondo physics and dissipation within an Anderson model of a magnetic impurity level that hybridizes with a metallic host and is also coupled, via the impurity charge, to the displacement of a bosonic bath having a spectral density proportional to ${\ensuremath{\omega}}^{s}$. As the impurity-bath coupling increases from zero, the effective Coulomb interaction between two electrons in the impurity level is progressively renormalized from its repulsive bare value until it eventually becomes attractive. For weak hybridization, this renormalization in turn produces a crossover from a conventional spin-sector Kondo effect to a charge Kondo effect. At particle-hole symmetry, and for sub-Ohmic bath exponents 0<s<10<s<10<s<1, further increase in the impurity-bath coupling results in a continuous zero-temperature transition to a broken-symmetry phase in which the ground-state impurity occupancy ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{n}}_{d}$ acquires an expectation value ${⟨{\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{n}}_{d}⟩}_{0}\ensuremath{\ne}1$. The response of the impurity occupancy to a locally applied electric potential features the hyperscaling of critical exponents and $\ensuremath{\omega}∕T$ scaling that are expected at an interacting critical point. The numerical values of the critical exponents suggest that the transition lies in the same universality class as that of the sub-Ohmic spin-boson model. For the Ohmic case s=1s=1s=1, the transition is instead of Kosterlitz-Thouless type. Away from particle-hole symmetry, the quantum phase transition is replaced by a smooth crossover but signatures of the symmetric quantum critical point remain in the physical properties at elevated temperatures and/or frequencies.
We propose a ground-state ansatz for the Ohmic spin-boson model that improves upon the variational treatment of Silbey and Harris for biased systems in the scaling limit. In particular, it correctly captures the smooth crossover behavior expected for the ground-state magnetization when moving between the delocalized and localized regimes of the model, a feature that the variational treatment is unable to properly reproduce, while it also provides a lower ground-state energy estimate in the crossover region. We further demonstrate the validity of our intuitive ground-state by showing that it leads to predictions in excellent agreement with those derived from a nonperturbative Bethe-ansatz technique. Finally, recasting our ansatz in the form of a generalized polaron transformation, we are able to explore the dissipative two-state dynamics beyond weak system-environment coupling within an efficient time-local master equation formalism.
Abstract We investigate the ground state properties and the nonequilibrium dynamics of a lattice trapped bosonic mixture consisting of an impurity species and a finite-sized medium. For the case of one as well as two impurities we observe that, depending on the lattice depth and the interspecies interaction strength, a transition from a strongly delocalized to a localized impurity distribution occurs. In the latter regime the two species phase separate, thereby forming a particle–hole pair. For two impurities we find that below a critical lattice depth they are delocalized among two neighboring outer lattice wells and are two-body correlated. This transition is characterized by a crossover from strong to a suppressed interspecies entanglement for increasing impurity-medium repulsion. Turning to the dynamical response of the mixture, upon quenching the interspecies repulsion to smaller values, we reveal that the predominant tunneling process for a single impurity corresponds to that of a particle–hole pair, whose dynamical stability depends strongly on the quench amplitude. During the time-evolution a significant increase of the interspecies entanglement is observed, caused by the build-up of a superposition of states and thus possesses a many-body nature. In the case of two bosonic impurities the particle–hole pair process becomes unstable in the course of the dynamics with the impurities aggregating in adjacent lattice sites while being strongly correlated.
The ground state and the spectral structure of lower-lying excited states of a dissipative two-level system coupled to a sub-Ohmic bath (s = 1/2) with nonzero bias have been studied using the unitary transformation method. By calculating the ground-state entanglement entropy, the ground-state average of σ(z)(G), and the static susceptibility of the two-level system, we explore the nature of the transition (crossover) between the delocalized and localized state of the two-level system. Furthermore, we calculate the time-dependent expectation (σ(z)(t)) and the time evolution of the entanglement entropy to show that, when the system undergoes a transition (crossover) from the delocalized to the localized state, the time evolution of the two-level system changes from coherent to decoherent dynamics.