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arXiv:0705.0957 · Physical Review Letters

Entanglement and Criticality in Quantum Impurity Systems

Karyn Le Hur, Philippe Doucet-Beaupré, Walter Hofstetter

Published Sep 17, 2007• 101 citations
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Abstract

We investigate the entanglement between a spin and its environment in impurity systems which exhibit a second-order quantum phase transition separating a delocalized and a localized phase for the spin. As an application, we employ the spin-boson model, describing a two-level system (spin) coupled to a sub-Ohmic bosonic bath with power-law spectral density, J(omega) proportional to omega(s) and 0 < s < 1. Combining Wilson's numerical renormalization group method and hyperscaling relations, we demonstrate that the entanglement between the spin and its environment is always enhanced at the quantum phase transition resulting in a visible cusp (maximum) in the entropy of entanglement. We formulate a correspondence between criticality and impurity entanglement entropy, and the relevance of these ideas to nanosystems is outlined.

DOI
10.1103/physrevlett.99.126801

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We investigate the entanglement between a spin and its environment in impurity systems which exhibit a second-order quantum phase transition separating a delocalized and a localized phase for the spin. As an application, we employ the spin-boson model, describing a two-level system (spin) coupled to a sub-Ohmic bosonic bath with power-law spectral density, J(omega) proportional to omega(s) and 0 < s < 1. Combining Wilson's numerical renormalization group method and hyperscaling relations, we demonstrate that the entanglement between the spin and its environment is always enhanced at the quantum phase transition resulting in a visible cusp (maximum) in the entropy of entanglement. We formulate a correspondence between criticality and impurity entanglement entropy, and the relevance of these ideas to nanosystems is outlined.
We describe the generalization of Wilson's numerical renormalization group method to quantum impurity models with a bosonic bath, providing a general nonperturbative approach to bosonic impurity models which can access exponentially small energies and temperatures. As an application, we consider the spin-boson model, describing a two-level system coupled to a bosonic bath with power-law spectral density, J(omega) proportional to omega(s). We find clear evidence for a line of continuous quantum phase transitions for sub-Ohmic bath exponents 0<s<1; the line terminates in the well-known Kosterlitz-Thouless transition at s=1. Contact is made with results from perturbative renormalization group, and various other applications are outlined.
The concept of entanglement entropy appears in multiple contexts, from black hole physics to quantum information theory, where it measures the entanglement of quantum states. We investigate the entanglement entropy in a simple model, the spin-boson model, which describes a qubit (two-level system) interacting with a collection of harmonic oscillators that models the environment responsible for decoherence and dissipation. The entanglement entropy allows to make a precise unification between entanglement of the spin with its environment, decoherence, and quantum phase transitions. We derive exact analytical results which are confirmed by Numerical Renormalization Group arguments both for an ohmic and a subohmic bosonic bath. Those demonstrate that the entanglement entropy obeys universal scalings. We make comparisons with entanglement properties in the quantum Ising model and in the Dicke model. We also emphasize the possibility of measuring this entanglement entropy using charge qubits subject to electromagnetic noise; such measurements would provide an empirical proof of the existence of entanglement entropy.
We study the impurity entanglement entropy SeS_eSe​ in quantum impurity models that feature a Kondo-destruction quantum critical point (QCP) arising from a pseudogap in the conduction-band density of states or from coupling to a bosonic bath. On the local-moment (Kondo-destroyed) side of the QCP, the entanglement entropy contains a critical component that can be related to the order parameter characterizing the quantum phase transition. In Kondo models describing a spin-$\Simp$, SeS_eSe​ assumes its maximal value of $\ln(2\Simp+1)$ at the QCP and throughout the Kondo phase, independent of features such as particle-hole symmetry and under- or over-screening. In Anderson models, SeS_eSe​ is nonuniversal at the QCP, and at particle-hole symmetry, rises monotonically on passage from the local-moment phase to the Kondo phase; breaking this symmetry can lead to a cusp peak in SeS_eSe​ due to a divergent charge susceptibility at the QCP. Implications of these results for quantum critical systems and quantum dots are discussed.
The ground state and the spectral structure of lower-lying excited states of a dissipative two-level system coupled to a sub-Ohmic bath (s = 1/2) with nonzero bias have been studied using the unitary transformation method. By calculating the ground-state entanglement entropy, the ground-state average of σ(z)(G), and the static susceptibility of the two-level system, we explore the nature of the transition (crossover) between the delocalized and localized state of the two-level system. Furthermore, we calculate the time-dependent expectation (σ(z)(t)) and the time evolution of the entanglement entropy to show that, when the system undergoes a transition (crossover) from the delocalized to the localized state, the time evolution of the two-level system changes from coherent to decoherent dynamics.
Recent work is reviewed on continuous quantum phase transitions in impurity models, both with fermionic and bosonic baths – these transitions are interesting realizations of boundary critical phenomena at zero temperature. The models with fermion bath are generalizations of the standard Kondo model, with the common feature that Kondo screening of the localized spin can be suppressed due to competing processes. The models with boson bath are related to the spin–boson model of dissipative two-level systems, where the interplay between tunneling and friction results in multiple phases. The competition inherent to all models can generate unstable fixed points associated with quantum phase transitions, where the impurity properties undergo qualitative changes. Interestingly, certain impurity transitions feature both lower-critical and upper-critical “dimensions” and allow for epsilon-type expansions. Results are presented for a number of observables, obtained by both analytical and numerical renormalization group techniques, and connections made to experiments.
We investigate quantum impurity problems, where a local magnetic moment is coupled to the spin density of a bosonic environment, leading to bosonic versions of the standard Kondo and Anderson impurity models. In a physical situation, these bosonic environments can correspond either to deconfined spinons in certain classes of Z2{Z}_{2}Z2​ frustrated antiferromagnets, or to particles in a multicomponent Bose gase (in which case the spin degree of freedom is attributed to hyperfine levels). Using renormalization group techniques, we establish that our impurity models, which feature an exchange interaction analogous to Kondo impurities in Fermi liquids, allow flow toward a stable strong-coupling state. Since the low-energy bosons exist around a single point in momentum space, and there is no Fermi surface, an impurity quantum phase transition occurs at intermediate coupling, separating screened and unscreened phases. This behavior is qualitatively different from previously studied spin-isotropic variants of the spin-boson model, which display stable intermediate-coupling fixed points and no screening.