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arXiv:1001.4952 · Physical Review A

Diagrammatic semiclassical laser theory

Oleg Zaitsev, Lev Deych

Published Feb 22, 2010• 13 citations
arXivHTMLPDF

Abstract

We derive semiclassical laser equations valid in all orders of nonlinearity. With the help of a diagrammatic representation, the perturbation series in powers of electric field can be resummed in terms of a certain class of diagrams. The resummation makes it possible to take into account a weak effect of population pulsations in a controlled way while treating the nonlinearity exactly. The proposed laser theory reproduces the all-order nonlinear equations in the approximation of constant population inversion and the third-order equations with population-pulsation terms as special cases. The theory can be applied to arbitrarily open and irregular lasers, such as random lasers.

DOI
10.1103/physreva.81.023822

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Physical Review A•Oct 1, 1976•15 citations
We derive semiclassical laser equations valid in all orders of nonlinearity. With the help of a diagrammatic representation, the perturbation series in powers of electric field can be resummed in terms of a certain class of diagrams. The resummation makes it possible to take into account a weak effect of population pulsations in a controlled way while treating the nonlinearity exactly. The proposed laser theory reproduces the all-order nonlinear equations in the approximation of constant population inversion and the third-order equations with population-pulsation terms as special cases. The theory can be applied to arbitrarily open and irregular lasers, such as random lasers.
A Lamb semiclassical theory is developed for multimode, mode-locked laser operation. The equality of frequency spacings between adjacent modes causes population pulsations generated in the nonlinear atomic response to be integer multiples of the adjacent-mode spacing. This allows the atomic response to be written in terms of Fourier series, thereby reducing coupled differential equations of motion to algebraic equations ultimately expressible in terms of a continued fraction. A unidirectional ring configuration is assumed so that the more complicated spatial dependence of standing waves is avoided. Reductions are made to the rateequation limit and to the special two-mode cases of bidirectional ring operation and single-mode, standing-wave, gas-laser operation. Numerical analysis of the equations is motivated. Specific results are given in the following (companion) paper.
This paper presents a semiclassical theory of a single-mode gas laser valid for essentially arbitrary values of field intensity. The theory is formulated in terms of an ensemble-averaged form of the density-matrix equations of motion involving a single set of coordinates. The polarization and the population-inversion density are expanded in spatial Fourier components. One obtains a set of coupled difference equations in the Fourier coefficients yn{y}_{n}yn​, which may be solved subject to appropriate boundary conditions on yn{y}_{n}yn​ for large nnn. The solutions may be expressed in terms of continued fractions in the general case, and in closed form in important special cases. Quantities of interest are evaluated by computer. The steady-state laser intensity and frequency are obtained from the coupled electromagnetic field equations as functions of the cavity parameters and the linear gain of the amplifying medium. At moderate values of field intensity, the velocity distribution of the space-averaged population inversion density exhibits a fine structure for low-velocity atoms superimposed on the usual broader depletion. This structure is a manifestation of the coherent ringing of the amplifying medium. The results are compared with those obtained in the rate-equation approximation, and with the recent work of Stenholm and Lamb. Discrepancies with the latter paper are explained.
Abstract This present paper is an attempt to describe the operation of a laser by a method patterned closely after the classical theory of dispersion. There, the electromagnetic field is treated as a classical system interacting with a collection of classical harmonic oscillators which are at rest. In the present case the radiation field is still treated classically, but, in accordance with the correspondence principle, the oscillators are now virtual oscillators associated with the up-and-down transitions in effective two-state atoms which are described quantum mechanically. The atoms carrying these virtual oscillators are not at rest but move with different velocities. We show how the Lorentz averaging can be performed for such systems, and derive a closed set of equations linking the average electric field E, with the average polarization density P„ and the average population inversion density Mp associated with atoms moving with the velocity v. Next, we investigate the conditions for the existence of a steady state if pumping is present, and if the electric field is represented by a standing wave, or a travelling wave of a single frequency (single-mode case). It turns out that, notwithstanding the nonlinear nature of the equations, the steady-state conditions give a simple complex dispersion relation; moreover, the real and imaginary part of this dispersion relation are equivalent to the usual heuristic expressions which specify the operating frequency in terms of the index of refraction and cavity length, and which balance the gain against the losses. The single-mode case is analysed in detail without any smallness assumptions for the resultant intensity. The small-intensity case gives the usual results exhibiting the tuning dip. For high intensities the relative depth of the dip tends to zero. At the end of the paper we discuss proposed extensions and additional applications.
Using semiclassical radiation theory, a formalism similar to that used by Lamb in his Theory of an Optical Maser is developed for studying the amplification of vector traveling waves in a laser-type medium. The effect of the medium on the waves is given in terms of space (or time) dependent field amplitudes and phases and a nonlinear index of refraction. With particular emphasis on typical gaseous media, the effects of Doppler broadening are treated in detail for arbitrary ratios of natural to Doppler linewidths. Polarization and propagation vectors in various directions are considered, and the nonlinear effects are found to make an isotropic medium effectively anisotropic. Lowest order nonlinear effects (due to a polarization cubic in the field amplitudes) are studied extensively, and the frequency dependence of several of these processes is presented in graphical form. In particular, the introduction of fields at new frequencies and polarization effects are considered. The characteristics of these nonlinear processes peculiar to Doppler broadened lines are discussed, and the processes are interpreted in terms of saturation and coherent modulation of the population inversion density. Strong nonlinear effects are considered in a more approximate way and are found to consist of saturation of the various linear and nonlinear processes previously considered. These strong nonlinear effects should occur at low enough intensities to be easily observed in practice on a CW basis. With the present formalism, the analytical results of Gordon, White and Rigden regarding gain saturation in laser amplifiers are obtained, and the extension is made to include frequencies away from line center and the effects of multiple spectral components. Again, the introduction of fields at new frequencies is considered in detail. These results are also discussed in terms of saturation and coherent modulation of the populations and hole burning.
The semiclassical interaction of a two-level system with a multimode electromagnetic field is discussed in detail. The equations of motion for the macroscopic density matrix are transformed into a single integral equation for the population density, with a complex kernel which can take into account both running- and standing-wave configurations. The iterative solution to this integral equation, which corresponds to an expansion in terms of powers of the electromagnetic field amplitudes, turns out to be divergent when the field amplitudes are greater than some critical value. In the case in which the kernel is a periodic or quasiperiodic function of time, a general solution to the integral equation is found, and this solution turns out to be unique and convergent for every value of the electromagnetic (e.m.) field amplitude. This solution is expressed through a continued-fraction expansion, whose terms are matrices, which can be readily obtained from the kernel. This solution is a generalization of the continued-fraction expansion usually met in the strong-signal semiclassical theory of lasers. Some particular cases are then treated in detail; among them, the solution to the multimode operation in laser devices is given in which the excited level lifetime is long compared with the period of the beating term between two adjacent modes. Although the theory presented is directed towards the steady-state regime in multimode lasers, it may also treat the transient regime of laser operations, or it may be extended to include phenomena where a strong e.m. field, made up of several modes equally spaced in frequency, interacts with a two-level system.