It is generally believed that dispersive polarimetric detection of collective angular momentum in large atomic spin systems gives rise to: squeezing in the measured observable, anti-squeezing in a conjugate observable, and collective spin eigenstates in the long-time limit (provided that decoherence is suitably controlled). We show that such behavior only holds when the particles in the ensemble cannot be spatially distinguished-- even in principle-- regardless of whether the measurement is only sensitive to collective observables. While measuring a cloud of spatially-distinguishable spin-1/2 particles does reduce the uncertainty in the measured spin component, it generates neither squeezing nor anti-squeezing. The steady state of the measurement is highly mixed, albeit with a well-defined value of the measured collective angular momentum observable.
It is generally believed that dispersive polarimetric detection of collective angular momentum in large atomic spin systems gives rise to: squeezing in the measured observable, anti-squeezing in a conjugate observable, and collective spin eigenstates in the long-time limit (provided that decoherence is suitably controlled). We show that such behavior only holds when the particles in the ensemble cannot be spatially distinguished-- even in principle-- regardless of whether the measurement is only sensitive to collective observables. While measuring a cloud of spatially-distinguishable spin-1/2 particles does reduce the uncertainty in the measured spin component, it generates neither squeezing nor anti-squeezing. The steady state of the measurement is highly mixed, albeit with a well-defined value of the measured collective angular momentum observable.
It has become common practice to model large spin ensembles as an effective pseudospin with total angular momentum J=Nj, where j is the spin per particle. Such approaches (at least implicitly) restrict the quantum state of the ensemble to the so-called symmetric Hilbert space. Here, we argue that symmetric states are not generally well preserved under the type of decoherence typical of experiments involving large clouds of atoms or ions. In particular, symmetric states are rapidly degraded under models of decoherence that act identically but locally on the different members of the ensemble. Using an approach [Phys. Rev. A 78, 052101 (2008)] that is not limited to the symmetric Hilbert space, we explore potential pitfalls in the design and interpretation of experiments on spin-squeezing and collective atomic phenomena when the properties of the symmetric states are extended to systems where they do not apply.
We determine the complete set of generalized spin squeezing inequalities, given in terms of the collective angular momentum components, for particles with an arbitrary spin. They can be used for the experimental detection of entanglement in an ensemble in which the particles cannot be individually addressed. We also present a large set of criteria involving collective observables different from the angular momentum coordinates. We show that some of the inequalities can be used to detect k-particle entanglement and bound entanglement.
Squeezing of collective atomic spins has been shown to improve the sensitivity of atomic clocks and magnetometers to levels significantly below the standard quantum limit. In most cases the requisite atom-atom entanglement has been generated by dispersive interaction with a quantized probe field or by state-dependent collisions in a quantum gas. Such experiments typically use complex multilevel atoms like Rb or Cs, with the relevant interactions designed so that atoms behave like pseudospin-21 particles. We demonstrate the viability of spin squeezing for collective spins composed of the physical angular momenta of 106 Cs atoms, each in an internal spin-4 hyperfine state. A peak metrological squeezing of at least 5dB is generated by quantum backaction from a dispersive quantum nondemolition (QND) measurement, implemented using a two-color optical probe that minimizes tensor light shifts without sacrificing measurement strength. Other significant developments include the successful application of composite pulse techniques for accurate dynamical control of the collective spin, enabled by broadband suppression of background magnetic fields inside a state-of-the-art magnetic shield. The absence of classical noise allows us to compare the observed quantum projection noise and squeezing to a theoretical model that properly accounts for both the relevant atomic physics and the spatial mode of the collective spin, finding good quantitative agreement and thereby validating its use in other contexts. Our work sets the stage for experiments on quantum feedback, deterministic squeezing, and closed-loop magnetometry. The implementation of real-time feedback may also create an opportunity for new types of quantum simulation, wherein the evolution of a quantum system is conditioned on the outcome of a time-continuous QND measurement. Such a scheme has the potential to access new regimes near the quantum-classical boundary, with opportunities to study long-standing issues related to quantum-classical correspondence in chaotic systems.
The field of quantum metrology concerns the physical measurement of sensors with a precision comparable to fundamental limits set by quantum mechanics. It is possible to outperform naive interpretations of these limits by using entangled states of the sensor system. One example is that of a spin-squeezed state, in which the uncertainty of one variable is decreased at the expense of another while still obeying Heisenberg's uncertainty principle, improving rotation sensitivity along a chosen axis. These states are potentially useful in devices including atomic clocks, inertial sensors, and magnetometers. Any model of a quantum metrology device must respect the fact that physical measurements are not passive, as imagined classically, but necessarily invasive. Far from being a negative feature, well-understood quantum measurement can conditionally drive a system into desirable entangled states, including spin-squeezed states. Furthermore, the fundamental randomness of this process can, in principle, be removed with real-time feedback control, motivating an adaptation of classical feedback concepts to the quantum realm. In this thesis, I describe these ideas in the context of one experimental example. A laser-cooled cloud of cesium spins is polarized along one axis via optical pumping and, subsequently, a linearly polarized far-off resonant probe beam traverses the sample. Due to the interaction Hamiltonian, the optical polarization rotates by an amount nominally proportional to one spin component of the collective spin state, enacting a weak, continuous, nondemolition measurement of that collective variable. This optical Faraday rotation is then measured with a polarimeter and the inherently noisy result used to condition the collective atomic state via a quantum filter, or stochastic master equation. Ideally, this process is capable of producing spin-squeezed states via the measurement itself. The details of this measurement are investigated in depth, including a derivation of the nonideal polarizability Hamiltonian, an analysis of the projection process with control, and a derivation of the magnetometry sensitivity. Experimentally, we demonstrate continuous measurement of the collective spin state with a large single-shot signal-to-noise ratio and verify many predictions of the model. Finally, we describe attempts to observe the atomic projection noise, which would infer the preparation of spin-squeezed states.
A complete set of generalized spin-squeezing inequalities is derived for an ensemble of particles with an arbitrary spin. Our conditions are formulated with the first and second moments of the collective angular momentum coordinates. A method for mapping the spin-squeezing inequalities for spin-21 particles to entanglement conditions for spin-j particles is also presented. We apply our mapping to obtain a generalization of the original spin-squeezing inequality to higher spins. We show that, for large particle numbers, a spin-squeezing parameter for entanglement detection based on one of our inequalities is strictly stronger than the original spin-squeezing parameter defined in S\o{}rensen et al. [Nature (London) 409, 63 (2001)]. We present a coordinate system independent form of our inequalities that contains, besides the correlation and covariance tensors of the collective angular momentum operators, the nematic tensor appearing in the theory of spin nematics. Finally, we discuss how to measure the quantities appearing in our inequalities in experiments.
We investigate the properties of angular-momentum states which yield high sensitivity to rotation. We discuss the application of these ``squeezed-spin'' or correlated-particle states to spectroscopy. Transitions in an ensemble of N two-level (or, equivalently, spin-1/2) particles are assumed to be detected by observing changes in the state populations of the particles (population spectroscopy). When the particles' states are detected with 100% efficiency, the fundamental limiting noise is projection noise, the noise associated with the quantum fluctuations in the measured populations. If the particles are first prepared in particular quantum-mechanically correlated states, we find that the signal-to-noise ratio can be improved over the case of initially uncorrelated particles. We have investigated spectroscopy for a particular case of Ramsey's separated oscillatory method where the radiation pulse lengths are short compared to the time between pulses. We introduce a squeezing parameter ${\ensuremath{\xi}}_{\mathit{R}}$ which is the ratio of the statistical uncertainty in the determination of the resonance frequency when using correlated states vs that when using uncorrelated states. More generally, this squeezing parameter quantifies the sensitivity of an angular-momentum state to rotation. Other squeezing parameters which are relevant for use in other contexts can be defined. We discuss certain states which exhibit squeezing parameters ${\ensuremath{\xi}}_{\mathit{R}}$\ensuremath{\simeq}${\mathit{N}}^{\mathrm{\ensuremath{-}}1/2}$. We investigate possible experimental schemes for generation of squeezed-spin states which might be applied to the spectroscopy of trapped atomic ions. We find that applying a Jaynes-Cummings--type coupling between the ensemble of two-level systems and a suitably prepared harmonic oscillator results in correlated states with ${\ensuremath{\xi}}_{\mathit{R}}$1.