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arXiv:0910.3897 · Physical Review A

Collective uncertainty in partially polarized and partially decohered spin- 12 systems

Ben Q. Baragiola, Bradley A. Chase, J. M. Geremia

Published Mar 5, 2010• 44 citations
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Abstract

It has become common practice to model large spin ensembles as an effective pseudospin with total angular momentum $J=\mathit{Nj}$, where $j$ is the spin per particle. Such approaches (at least implicitly) restrict the quantum state of the ensemble to the so-called symmetric Hilbert space. Here, we argue that symmetric states are not generally well preserved under the type of decoherence typical of experiments involving large clouds of atoms or ions. In particular, symmetric states are rapidly degraded under models of decoherence that act identically but locally on the different members of the ensemble. Using an approach [Phys. Rev. A 78, 052101 (2008)] that is not limited to the symmetric Hilbert space, we explore potential pitfalls in the design and interpretation of experiments on spin-squeezing and collective atomic phenomena when the properties of the symmetric states are extended to systems where they do not apply.

DOI
10.1103/physreva.81.032104

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It has become common practice to model large spin ensembles as an effective pseudospin with total angular momentum J=NjJ=\mathit{Nj}J=Nj, where jjj is the spin per particle. Such approaches (at least implicitly) restrict the quantum state of the ensemble to the so-called symmetric Hilbert space. Here, we argue that symmetric states are not generally well preserved under the type of decoherence typical of experiments involving large clouds of atoms or ions. In particular, symmetric states are rapidly degraded under models of decoherence that act identically but locally on the different members of the ensemble. Using an approach [Phys. Rev. A 78, 052101 (2008)] that is not limited to the symmetric Hilbert space, we explore potential pitfalls in the design and interpretation of experiments on spin-squeezing and collective atomic phenomena when the properties of the symmetric states are extended to systems where they do not apply.
The symmetric collective states of an atomic spin ensemble (i.e., many-body states that are invariant under particle exchange) are not preserved by decoherence that acts identically but individually on members of the ensemble. We develop a class of collective states in an ensemble of N spin-1/2 particles that is invariant under symmetric local decoherence and find that the dimension of the Hilbert space spanned by these collective states scales only as N^2. We then investigate the open system dynamics of experimentally relevant non-classical collective atomic states, including Schroedinger cat and spin squeezed states, subject to various symmetric but local decoherence models.
When the dynamics of a spin ensemble are expressible solely in terms of symmetric processes and collective spin operators, the symmetric collective states of the ensemble are preserved. These many-body states, which are invariant under particle relabeling, can be efficiently simulated since they span a subspace whose dimension is linear in the number of spins. However, many open system dynamics break this symmetry, most notably when ensemble members undergo identical, but local, decoherence. In this paper, we extend the definition of symmetric collective states of an ensemble of spin-1∕21∕21∕2 particles in order to efficiently describe these more general collective processes. The corresponding collective states span a subspace that grows quadratically with the number of spins. We also derive explicit formulas for expressing arbitrary, identical, local decoherence in terms of these states. We then investigate the open system dynamics of experimentally relevant nonclassical collective atomic states, including superposition and spin squeezed states, subject to various symmetric but local decoherence models.
It is generally believed that dispersive polarimetric detection of collective angular momentum in large atomic spin systems gives rise to: squeezing in the measured observable, anti-squeezing in a conjugate observable, and collective spin eigenstates in the long-time limit (provided that decoherence is suitably controlled). We show that such behavior only holds when the particles in the ensemble cannot be spatially distinguished-- even in principle-- regardless of whether the measurement is only sensitive to collective observables. While measuring a cloud of spatially-distinguishable spin-1/2 particles does reduce the uncertainty in the measured spin component, it generates neither squeezing nor anti-squeezing. The steady state of the measurement is highly mixed, albeit with a well-defined value of the measured collective angular momentum observable.
In this thesis I explore the use of collective spin angular momentum as a platform for quantum information processing. Such systems have several nice features that make them excellent choices for such protocols, especially ones where information is also stored in photonic variables. The longer coherence times of atoms makes it possible to store information from light in atoms for future use, and it is generally easier to couple atomic variables than to create nonlinear interactions of light. Above and beyond the advantages of atomic systems, collective atomic systems have additional strengths. In the limit of a large number of atoms, the collective variables of atomic systems have a natural connection to the bosonic algebra of light (known as the Holstein-Primakoff or HP approximation) where components of the collective spin angular momentum effectively act as quadratures, making them natural systems for coupling to light. Also, collectively addressing the atoms allows one to access a large state space without individual addressing of the atoms. A natural first step towards control of these collective variables is generating large amounts of atomic spin squeezing. In the HP approximation going from rotations to squeezing corresponds to going from linear to quadratic interactions in the atomic quadratures; for extremely large squeezing one should see the breakdown of the HP approximation and the ability to generate arbitrary collective atomic states. I have sought to improve previous schemes for the spin squeezing of atomic ensembles, such as the proposal of Takeuchi et. al. based on coherent quantum feedback. In this scheme a beam of linearly polarized light passes through the atomic ensemble (prepared in a coherent state), coupling to the atoms through a state-dependent index of refraction (the Faraday effect). The light is then passed through a wave-plate and reflected back through the atoms for a second pass. This double-pass scheme leads to an effective nonlinearity as the atomic fluctuations are mapped onto the light on the first pass and then back on to the atoms in the second pass. The light acts as a bus coupling each atom to each of the others. This nonlinear interaction forms a shearing of the atomic coherent state that results in squeezing. The light is entangled to the atoms through these interactions, and remains entangled as it escapes the system. This leads to decoherence of the atoms as the light is lost to the environment, reducing the amount of spin squeezing achieved. The first step towards improving the double-pass scheme was to add a quantum eraser step in which the light is disentangled from the squeezed atoms. By first measuring one quadrature of the light, and then performing a measurement-dependent rotation on the atomic ensemble, it is possible to decouple the atoms and light so that the loss of the light does not reduce the atomic squeezing. This results in an improvement of the rate of atomic spin squeezing. The nonlinear shearing interaction that remains still falls short of the exponential squeezing seen in optical parametric amplification. The reason for this can be seen by decomposing the shearing interaction into squeezing along a given quadrature followed by a rotation. The rotation leads to a constantly changing axis along which the squeezing occurs, and thus the squeezing builds up more slowly. This can be corrected for by breaking up the light pulse into a sequence of small pulses, and performing a small phase matching rotation after each pulse. The squeezing then adds up along a constant direction, rather than along a constantly varying direction. This results in still further improvement of the rate of atomic spin squeezing. A complete model includes the effects of photon-atom scattering and other noise and loss effects on the overall rate of squeezing. Previous derivations of noise due to photon-atom scattering have started with the unjustified assumptions that the atomic and photonic decoherence channels were both Gaussian and independent of correlations between the two subsystems. They then proceed with very general statistical arguments that rely upon these simplifications. My work begins with the more fundamental master equation picture in which I find the Linblad jump operators. I find that in general the photonic and atomic loss channels are not independent, with the intensity of the light dictating the details of this dependence, and find the conditions under which the Gaussian approximation holds. Squeezing and loss is initially treated assuming ensembles of spin-1/2 atoms, but this work is further extended to higher dimensional subsystems. For a higher spin case, preparing the atoms in spin coherent states is not optimal. One can engineer a stronger interaction by preparing the atoms in an atomic "cat state", i.e., a superposition of the two stretch states along the direction of propagation of the light beam. The fluctuations of such a state are more strongly coupled to the light, resulting in a stronger nonlinearity. This leads to strong correlations between the atoms, but they are not immediately useful for squeezing; the cat state must be coherently mapped to a coherent state to achieve atomic spin squeezing. The state created in this manner is ultimately more squeezed than that achieved with the same interaction but prepared initially in a coherent state.
Squeezing of collective atomic spins has been shown to improve the sensitivity of atomic clocks and magnetometers to levels significantly below the standard quantum limit. In most cases the requisite atom-atom entanglement has been generated by dispersive interaction with a quantized probe field or by state-dependent collisions in a quantum gas. Such experiments typically use complex multilevel atoms like Rb or Cs, with the relevant interactions designed so that atoms behave like pseudospin-12\frac{1}{2}21​ particles. We demonstrate the viability of spin squeezing for collective spins composed of the physical angular momenta of 106{10}^{6}106 Cs atoms, each in an internal spin-4 hyperfine state. A peak metrological squeezing of at least 5dB is generated by quantum backaction from a dispersive quantum nondemolition (QND) measurement, implemented using a two-color optical probe that minimizes tensor light shifts without sacrificing measurement strength. Other significant developments include the successful application of composite pulse techniques for accurate dynamical control of the collective spin, enabled by broadband suppression of background magnetic fields inside a state-of-the-art magnetic shield. The absence of classical noise allows us to compare the observed quantum projection noise and squeezing to a theoretical model that properly accounts for both the relevant atomic physics and the spatial mode of the collective spin, finding good quantitative agreement and thereby validating its use in other contexts. Our work sets the stage for experiments on quantum feedback, deterministic squeezing, and closed-loop magnetometry. The implementation of real-time feedback may also create an opportunity for new types of quantum simulation, wherein the evolution of a quantum system is conditioned on the outcome of a time-continuous QND measurement. Such a scheme has the potential to access new regimes near the quantum-classical boundary, with opportunities to study long-standing issues related to quantum-classical correspondence in chaotic systems.
We determine the complete set of generalized spin squeezing inequalities, given in terms of the collective angular momentum components, for particles with an arbitrary spin. They can be used for the experimental detection of entanglement in an ensemble in which the particles cannot be individually addressed. We also present a large set of criteria involving collective observables different from the angular momentum coordinates. We show that some of the inequalities can be used to detect k-particle entanglement and bound entanglement.