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arXiv:0908.4303

Deterministic generation of non-classical states of light using photon blockade

Andrei Faraon, Arka Majumdar, Jelena Vuckovic A

Published Aug 28, 2009• 0 citations
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Abstract

The generation of non-classical states of light via photon blockade with time-modulated input is analyzed. We show that improved single photon statistics can be obtained by adequately choosing the parameters of the driving laser pulses. An alternative method, where the system is driven via a continuous wave laser and the frequency of the dipole is controlled (e.g. electrically) at very fast timescales is presented.

DOI
10.48550/arxiv.0908.4303

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The generation of non-classical states of light via photon blockade with time-modulated input is analyzed. We show that improved single photon statistics can be obtained by adequately choosing the parameters of the driving laser pulses. An alternative method, where the system is driven via a continuous wave laser and the frequency of the dipole is controlled (e.g. electrically) at very fast timescales is presented.
The single photon character of nonclassical states of light that can be generated using photon blockade is analyzed for time domain operation. We show that improved single photon statistics (single photon around 85% with a multi-photon of 8%) can be obtained by adequately choosing the parameters (mainly amplitude and pulseduration) of the driving laser pulses. An alternative method, where the system is driven via a continuous wave laser and the frequency of the dipole is controlled (e.g. electrically) at very fast timescales is presented. We also show that this non-classical state performs better than a weak coherent pulse, when applied to BB84 quantum cryptography protocol.
Non-Gaussian quantum states are essential resources for continuous-variable quantum information processing and for metrology. Among these, multi-photon added coherent states bridge classical and non-classical behaviors; however, their generation typically relies on small photon numbers and probabilistic heralding schemes. Here, we propose a protocol for the post-selection free generation of high fidelity multi-photon added coherent states using the photon blockade effect in a driven Kerr nonlinear resonator, where such states emerge naturally during the dynamics. We demonstrate that high-fidelity states can be prepared by optimizing the external drive power and the interaction time. Furthermore, we show that the protocol is robust under realistic experimental conditions, achieving fidelities of ≈99%\approx 99\%≈99% with current state-of-the-art parameters. Our results unlock a deterministic route to complex non-classical states using well-established quantum optical platforms.
We theoretically analyzed the photon quantum statistics properties of the output field from an optomechanical system driven by different pulsed lasers. Our results show that the probability of generating a single-photon state at the photon blockade region is greatly dependent on properties such as the shape, area, central frequency, length, and amplitude of the driving pulse. These results will give guidance to the design of the potential optimal optical pulse for generating a high-performance single-photon source.
The generation of non-classical states of light [1] is an important scientific challenge with many potential applications. For example, squeezed states of light [2] have generated much interest in the past decade, because measurements can be performed with noise levels that are lower than those available with classical light. A particularly novel non-classical source of light is a triggered single-photon source: a source that has the property to emit with a high degree of certainty one (and only one) photon at a user-specified time. Such a deterministic source of single photons can be important for quantum information processing [3], quantum cryptography [4] and certain quantum computation problems [5]. A single quantum emitter such as a molecule or an atom is a good potential source because it can emit only one photon at a time. The emitted light is antibunched [6, 7] and consists of single photons separated by random time intervals, which depend on the excited state lifetime and on the pumping rate. Thus triggered emission of single photons can be obtained with controlled excitation of a single emitter. The first demonstration of a single photons source [8] using a single molecule in a solid is based on a rapid adiabatic passage method [9] to excite the molecule. In the effective spin picture, the Bloch vector follows the driving magnetic field adiabatically if the laser-molecule frequency detuning is swept slowly through the resonance. Since the passage inverts the field, the system goes from the ground to the excited state. From this fluorescent state the molecule can emit only a single photon. The molecular resonance is swept by Stark effect at fixed laser frequency. This is done easily by applying a radio frequency electric field to the molecule. The results showed photon states with statistics that differ radically from those of coherent states. But this method requires cryogenic temperatures (2K) since narrow zero phonon lines are needed for the adiabatic following. At room temperature a source of triggered single photons based on the concept of pulsed optical excitation of a single highly fluorescent molecule has been demonstrated [10]. A short pulse of green laser light pumps the molecule from the ground state to a vibronically excited level of the first electronic excited state. After fast (ps) relaxation to the lowest electronic excited state, the molecule subsequently emits a single photon. A frequency-doubled mode-locked Nd-YAG laser is used to pump highly stable single terrylene molecules contained in a p-terphenyl molecular crystal where they are protected from exposure to diffusing quenchers (such as oxygen). The result shows that the photons are emitted after the laser pulses at times separated by the laser repetition time within the lifetime of terrylene in p-terphenyl. Since the pump pulse width is very short compared to the fluorescence lifetime, the probability of two (or more) photon emission per pulse is always zero. At the maximum laser power, 90% of the laser pulses lead to a single photon emission. The parameters of this source (repetition rate and single photon generation probability) were limited only by the laser system used; nevertheless, this performance already surpasses that of previous work. The high performance combined with the vanishing two photon emission probability and the simplicity of this source suggests that it can be considered for a variety of quantum optical experiments and for secure quantum cryptography [11]. Semiconductor quantum dots (QD) are other potential systems for single photon generation [12]. QDs are often referred to as “artificial atoms” because many of their optical properties, such as ultranarrow transitions, arise from discrete, atomic-like energy levels [13, 14]. To reinforce this analogy a study of the photon antibunching in this system was needed. QDs differ from atoms and molecules since the creation of multiple excitons is possible in QDs. Consequently, if two electron-hole pairs can radiatively recombine, the simultaneous emission of two photons from a QD is then possible. Thus different regimes of photon statistics were expected because the probability of multiple exciton creation depends on excitation intensity. The fluorescence intensity correlation function of a single CdSe quantum dot has been investigated [15] using a coincidence setup (start-stop experiment). A strong photon antibunching has been observed over a large range of intensities (0.1-100 kW/cm2). The lack of coincidence at zero time delay indicates a highly efficient Auger ionization process [16], which suppresses multi-photon emission in these colloidal quantum dots. This result shows that room temperature single photon sources can be achieved with colloidal nanoparticles.