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arXiv:0904.2515 · Physical Review Letters

Collisional Losses, Decoherence, and Frequency Shifts in Optical Lattice Clocks with Bosons

Christian Lisdat, J. S. Raaj Vellore Winfred, Thomas Middelmann, F. Riehle, Uwe Sterr

Published Aug 28, 2009• 87 citations
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Abstract

We have quantified collisional losses, decoherence and the collision shift in a one-dimensional optical lattice clock on the highly forbidden transition (1)S(0)-(3)P(0) at 698 nm with bosonic (88)Sr. We were able to distinguish two loss channels: inelastic collisions between atoms in the upper and lower clock state and atoms in the upper clock state only. Based on the measured coefficients, we determine the operation parameters at which a 1D-lattice clock with (88)Sr shows no degradation due to collisions on the fractional uncertainty level of 10(-16).

DOI
10.1103/physrevlett.103.090801

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We have quantified collisional losses, decoherence and the collision shift in a one-dimensional optical lattice clock on the highly forbidden transition (1)S(0)-(3)P(0) at 698 nm with bosonic (88)Sr. We were able to distinguish two loss channels: inelastic collisions between atoms in the upper and lower clock state and atoms in the upper clock state only. Based on the measured coefficients, we determine the operation parameters at which a 1D-lattice clock with (88)Sr shows no degradation due to collisions on the fractional uncertainty level of 10(-16).
We present detailed analyses of our recent experiment on the three-dimensional (3D) optical lattice clock with bosonic 88Sr^{88}\mathrm{Sr}88Sr atoms in which the collisional frequency shift was suppressed by applying a single-occupancy lattice. Frequency shifts in magnetically induced spectroscopy on the 1S0−−3P0{}^{1}{S}_{0}--{}^{3}{P}_{0}1S0​−−3P0​ clock transition ($\ensuremath{\lambda}=698$ nm) of 88Sr^{88}\mathrm{Sr}88Sr were experimentally investigated by referencing a one-dimensional (1D) lattice clock based on spin-polarized 87Sr^{87}\mathrm{Sr}87Sr atoms. We discuss that the clock stability is limited by the current laser stability as well as the experimental sequence of the clock operation, which may be improved to ${\ensuremath{\sigma}}_{y}(\ensuremath{\tau})=2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}16}/\sqrt{\ensuremath{\tau}}$ by optimizing the cycle time of the clock operation.
We discuss two possible configurations for optical lattice clocks; a one-dimensional (1D) lattice loaded with spinpolarized fermions, and a three-dimensional (3D) lattice loaded with bosons. In the former scheme, collisional frequency shifts are suppressed by the quantum statistical property of identical fermions. This Pauli blocking of collisions is critically dependent on the degree of spin polarization of the fermionic atoms, which we carefully investigated in the Rabi excitation process of the clock transition. In the latter scheme, a single occupancy lattice suppresses bunching of bosons and collisional frequency shifts. We demonstrate a frequency comparison of these two optical lattice clocks based on fermionic 87Sr and bosonic 88Sr. Operating these clocks parallely has yielded a stability approaching 10−17. Such measurements are an important step to ascertain the lattice clocks' uncertainty at the 10−17 level and beyond.
We describe our experiment which evaluates frequency shifts due to collisions in a 1-D optical lattice clock with88Sr. The atoms in the lattice are probed on the1S0-3P0transition which is highly forbidden but becomes weakly allowed by applying a static homogeneous magnetic field which mixes3P1to the3P0state. Using the method of interleaved stabilization, we have quantified the density dependent shift of the88Sr clock transition. By knowing the coefficient of the shift we can determine optimum conditions under which a 1-D lattice clock with88Sr can be operated with a fractional accuracy of 10-16.
We study the influence of ultracold collisions induced by the inhomogeneous excitation on the clock-transition frequency in one- and two-dimensional shallow blue-detuned (BD) 87{}^{87}87Sr optical lattice clocks with a magic wavelength of ${\ensuremath{\lambda}}_{b}=389.889$ nm. The minimal lattice potential required to tightly confine atoms in each single lattice site is much larger than that required for a red-detuned (RD) lattice operating at ${\ensuremath{\lambda}}_{r}=813.4$ nm because of the relatively smaller magic wavelength. For a deep optical lattice, the two-body interactions of atoms in a single lattice site mainly contribute to the clock-transition frequency shift, while the intersite collisions primarily affect the collisional shift in a shallow optical lattice. For an effective misalignment angle $\ensuremath{\Delta}\ensuremath{\theta}\ensuremath{\sim}10$ mrad of the probe beam with respect to the lattice axis, the fractional collisional shifts in both one- and two-dimensional BD lattices are at the ${10}^{\ensuremath{-}16}$ level.
We demonstrate a one-dimensional optical lattice clock with a spin-polarized fermionic isotope designed to realize a collision-shift-free atomic clock with neutral atom ensembles. To reduce systematic uncertainties, we developed both Zeeman shift and vector light-shift cancellation techniques. By introducing both an H-maser and a Global Positioning System (GPS) carrier phase link, the absolute frequency of the 1S0(F=9/2)−3P0(F=9/2)^1S_0(F=9/2) - {}^3P_0(F=9/2)1S0​(F=9/2)−3P0​(F=9/2) clock transition of the 87^{87}87Sr optical lattice clock is determined as 429,228,004,229,875(4) Hz, where the uncertainty is mainly limited by that of the frequency link. The result indicates that the Sr lattice clock will play an important role in the scope of the redefinition of the ``second'' by optical frequency standards.
We observe two-body loss of 3P0{}^{3}\phantom{\rule{-0.16em}{0ex}}{P}_{0}3P0​ 87{}^{87}87Sr atoms trapped in a one-dimensional optical lattice. We measure loss rate coefficients for atomic samples between 1 and 6 $\ensuremath{\mu}$K that are prepared either in a single nuclear-spin sublevel or with equal populations in two sublevels. The measured temperature and nuclear-spin preparation dependence of rate coefficients agree well with calculations and reveal that rate coefficients for distinguishable atoms are only slightly enhanced over those of indistinguishable atoms. We further observe a suppression of excitation and losses during interrogation of the 1S0{}^{1}\phantom{\rule{-0.16em}{0ex}}{S}_{0}1S0​--3P0{}^{3}\phantom{\rule{-0.16em}{0ex}}{P}_{0}3P0​ transition as density increases and Rabi frequency decreases, which suggests the presence of strong interactions in our dynamically driven many-body system.