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arXiv:0901.4110 · New Journal of Physics

Generation of macroscopic singlet states in atomic ensembles

Géza Tóth, Morgan W Mitchell

Published May 6, 2010• 67 citations
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Abstract

We study squeezing of the spin uncertainties by quantum non-demolition (QND) measurement in non-polarized spin ensembles. Unlike the case of polarized ensembles, the QND measurements can be performed with negligible back-action, which allows, in principle, perfect spin squeezing as quantified by Tóth et al (2007 Phys. Rev. Lett. 99 250405). The generated spin states approach many-body singlet states and contain a macroscopic number of entangled particles even when individual spin is large. We introduce the Gaussian treatment of unpolarized spin states and use it to estimate the achievable spin squeezing for realistic experimental parameters. Our proposal might have applications for magnetometry with a high spatial resolution or quantum memories storing information in decoherence free subspaces.

DOI
10.1088/1367-2630/12/5/053007

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We study squeezing of the spin uncertainties by quantum non-demolition (QND) measurement in non-polarized spin ensembles. Unlike the case of polarized ensembles, the QND measurements can be performed with negligible back-action, which allows, in principle, perfect spin squeezing as quantified by Tóth et al (2007 Phys. Rev. Lett. 99 250405). The generated spin states approach many-body singlet states and contain a macroscopic number of entangled particles even when individual spin is large. We introduce the Gaussian treatment of unpolarized spin states and use it to estimate the achievable spin squeezing for realistic experimental parameters. Our proposal might have applications for magnetometry with a high spatial resolution or quantum memories storing information in decoherence free subspaces.
We demonstrate spin squeezing and entanglement in a large-spin system via quantum non-demolition measurement. We make non-destructive, projection-noise-limited collective spin measurements on an ensemble of up to in 8.4 × 105 laser-cooled 87Rb atoms in the f = 1 hyperfine ground state. A dynamically-decoupled probing scheme [Phys. Rev. Lett. 105, 093602 (2010)] prevents probe-induced decoherence. Repeated measurements show correlations beyond the standard quantum limit, indicating generation of a spin-squeezed state with up to −3.6 dB of noise reduction and −2.6 dB of metrologically-relevant squeezing.
Planar squeezed states, i.e. quantum states which are squeezed in two orthogonal spin components, have recently attracted attention due to their applications in atomic interferometry and quantum information (He et al 2012 New J. Phys. 14 093012). While canonical variables such as quadratures of the radiation field can be squeezed in at most one component, simultaneous squeezing in two orthogonal spin components can be achieved due to the angular momentum commutation relations. We present a novel scheme for planar squeezing via quantum non-demolition (QND) measurements in spin-1 systems. The QND measurement is achieved via near-resonant paramagnetic Faraday rotation probing, and the planar squeezing is obtained by sequential QND measurement of two orthogonal spin components. We compute the achievable squeezing for a variety of optical depths, initial conditions and probing strategies. The planar squeezed states generated in this way contain entanglement detectable by spin-squeezing inequalities and give an advantage relative to non-squeezed states for any precession phase angle, a benefit for single-shot and high-bandwidth magnetometry.
The work is organized in two main topics. At first we will outline the relation between spin squeezing, quantum metrology and entanglement detection, with a particular focus on the last. We will derive spin squeezing criteria for the detection of entanglement and its depth that outperform past approaches, especially for unpolarized states, recently produced in experiments and object of increasing interest in the community. Furthermore, we will extend the original definition of spin squeezed states by providing a new parameter that is thought to embrace different classes of states in a unified framework. Afterwards we consider a test of quantum principles in macroscopic objects originally designed by Leggett and Garg. In this case the scenario consists of a single party that is probed at different time instants and the quantum effect detected is the violation of Macrorealism (MR), due to strong correlations in time, rather than in space, between non-compatible observables. We will look at the problems of inconclusiveness of the LG tests arising from possible explanations of the results in terms of ``clumsy'' measurements, what has been termed ``clumsiness loophole''. We propose first a scheme to test and possibly falsify (MR) in macroscopic ensembles of cold atoms based on alternating Quantum Non-Demolition measurements and coherent, magnetically-driven collective spin rotations. Then we also propose a way to address the clumsiness loophole by introducing and computing an invasivity quantifier to add to the original LG expression. We provide numerical evidence that such a clumsiness-free test is feasible under state-of-the-art realistic experimental parameters and imperfections.
Spin squeezing of 101110^{11}1011 atoms
Atomic ensemble with large number of quantum correlated particles is a desirable resource for precision measurement and quantum simulation. Being a type of quantum correlated state particularly useful for quantum metrology, spin squeezed state (SSS) has been pursued in both cold atom and vapor cell systems, and the largest ensemble so far contains 10810^{8}108 atoms. We report experimental preparation of a SSS in a paraffin-coated macroscopic vapor cell in free space, containing 101110^{11}1011 87Rb^{87}\text{Rb}87Rb atoms, by means of stroboscopic quantum non-demolition measurement. We observed 2.38±0.23 dB2.38\pm0.23~\text{dB}2.38±0.23 dB noise reduction, and 1.31±0.23 dB1.31\pm0.23~\text{dB}1.31±0.23 dB spin squeezing \emph{below coherent spin state} by the Wineland criterion. Our result present the highest angular resolution on the Bloch sphere in all SSS up to date, and will open possibilities to implement quantum control, metrology and quantum simulations using such large entangled atomic ensembles. The universal off-resonance interaction utilized here can also be straightforwardly expanded to other systems, such as trapped ions and mechanical oscillators, in the application of entanglement generation and open-system quantum simulations.