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arXiv:0811.2183 · Applied Physics Letters

Laser frequency stabilization to excited state transitions using electromagnetically induced transparency in a cascade system

R. P. Abel, Ashok Kumar Mohapatra, Mark G. Bason, Jonathan D. Pritchard, Kevin J. Weatherill, U. Raitzsch, Charles S. Adams

Published Feb 16, 2009• 118 citations
arXivHTMLPDF

Abstract

We demonstrate laser frequency stabilization to excited state transitions using cascade electromagnetically induced transparency. Using a room temperature Rb vapor cell as a reference, we stabilize a first diode laser to the D2 transition and a second laser to a transition from the intermediate 5P3/2 state to a highly excited state with principal quantum number n=19–70. A combined laser linewidth of 280±50 kHz over a 100 μs time period is achieved. This method may be applied generally to any cascade system and allows laser stabilization to an atomic reference in the absence of a direct absorption signal.

DOI
10.1063/1.3086305

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We demonstrate laser frequency stabilization to excited state transitions using cascade electromagnetically induced transparency. Using a room temperature Rb vapor cell as a reference, we stabilize a first diode laser to the D2 transition and a second laser to a transition from the intermediate 5P3/2 state to a highly excited state with principal quantum number n=19–70. A combined laser linewidth of 280±50 kHz over a 100 μs time period is achieved. This method may be applied generally to any cascade system and allows laser stabilization to an atomic reference in the absence of a direct absorption signal.
We present a laser frequency locking to Rydberg transition with electromagnetically induced transparency (EIT) spectra in a room-temperature cesium vapor cell. Cesium levels 6S 1/2 , 6P 3/2 , and the n D 5/2 state, compose a cascade three-level system, where a coupling laser drives Rydberg transition, and probe laser detects the EIT signal. The error signal, obtained by demodulating the EIT signal, is used to lock the coupling laser frequency to Rydberg transition. The laser frequency fluctuation, ∼0.7 MHz, is obtained after locking on, with the minimum Allan variance to be 8.9 × 10 −11 . This kind of locking method can be used to stabilize the laser frequency to the excited transition.
We propose a method to continuously frequency shift a target laser that is frequency stabilized by a reference laser, which is several hundreds of nanometers detuned. We demonstrate the technique using the 5S1/2→ 5P3/2→ 29D5/2Rydberg transition in87Rb vapor and lock the 482 nm target laser to the 780 nm reference laser using the cascaded electromagnetically induced transparency signal. The stabilized frequency of the target laser can be shifted by about 1.6 GHz by phase modulating the reference laser using a waveguide-type electro-optical modulator. This simple method for stable frequency shifting can be used in atomic or molecular physics experiments that require a laser frequency scanning range on the order of several GHz.
Electromagnetically induced transparency is observed in a mismatched-wavelength cascade system with a room-temperature rubidium vapor cell. A cw probe laser beam monitors the 5S(1/2) ? 5P(3/2) transition while another cw laser couples the 5P(3/2) state to a higher excited state. The ratio of the observed Rabi frequencies for coupling to the 5P(3/2) ? 8D(3/2), (5/2) transitions agrees well with that predicted by use of the transition oscillator strengths. Optical switching is demonstrated with an 80-mW coupling laser beam modulated up to 1 MHz.
An electromagnetically induced transparency (EIT) signal is observed in a V-type energy level scheme in a cesium vapor cell at room temperature. The effects of frequency detuning and the intensity of the pump laser on the EIT signal have been investigated. The performance of the probe-diode laser system, which is frequency stabilized on the EIT signal by using electrical feedback, is explored. The first derivative of the EIT signal offers a steeper slope and better S/N ratio for laser frequency stabilization than that of the Doppler-free hyperfine and crossover resonances. A comparative study of the frequency stability of an external-cavity diode laser stabilized at EIT and at the crossover resonance is presented. The square root of the Allan variance (σ) vs. integration time (τ) plot shows about a tenfold improvement in the frequency stability of the EIT-locked laser (σ ∼ 2.043 × 10 −13 τ −1/2 ) over that of the crossover-locked laser under a short integration time (1–10 ms), whereas a twofold improvement is found under a long integration time (∼1 s).
We herein develop and demonstrate a stable frequency-locking scheme for Rydberg atomic experiments. We use the Zeeman effect to modulate the three-level ladder-type Rydberg electromagnetically induced transparency (EIT) signal to lock the laser frequency of the coupling light for transition from its intermediate state to a Rydberg state. The effects of polarization of the probe and coupling lights, and the amplitude of the AC modulated magnetic field B 0 on the EIT and the corresponding dispersive error signal, are both analyzed. The results show that both the EIT signal and dispersive error signal are the strongest when the polarizations of coupling and probe fields are circular and equal. The signal-to-noise ratio of the dispersive error signal increases with B 0 . The slope of the dispersive error signal increases first and then decreases with B 0 , which is related to the increase of the EIT linewidth caused by the higher B 0 . The linewidth of the laser is significantly less than 500 kHz after frequency locking, which satisfies the requirements of most experiments involving Rydberg atoms. The method proposed herein can generally be applied to any cascade system of Rydberg atoms.
Electromagnetically induced transparency (EIT) was observed in a mismatched-wavelength cascade system using a room temperature vapor cell and laser-cooled atoms. A cw probe laser beam monitored the cesium ${6S}_{1/2}\ensuremath{\rightarrow}{6P}_{3/2}$ transition while another cw laser coupled the 6P3/2{6P}_{3/2}6P3/2​ state to a higher excited state. The ratio of the observed Rabi frequencies for coupling to the ${6P}_{3/2}\ensuremath{\rightarrow}(11--{13)D}_{3/2,5/2}$ transitions agreed closely with that predicted using the transition oscillator strengths. A comparison of the EIT signals obtained using cold atoms and the vapor cell is made.