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arXiv:0807.1503

Theory for superfluidity in a Bose system

Zhidong Hao

Published Jul 9, 2008• 0 citations
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Abstract

We present a microscopic theory for superfluidity in an interacting many-particle Bose system (such as liquid $^4$He). We show that, similar to superconductivity in superconductors, superfluidity in a Bose system arises from pairing of particles of opposite momenta. We show the existence of an energy gap in single-particle excitation spectrum in the superfluid state and the existence of a specific heat jump at the superfluid transition. We derive an expression for superfluid particle density $n_s$ as a function of temperature $T$ and superfluid velocity ${\bf v}_s$. We show that superfluid-state free energy density $F$ is an increasing function of $v_s$ (i.e., $\partial F/\partial v_s > 0$), which indicates that a superfluid has a tendency to remain motionless (this result qualitatively explains the Hess-Fairbank effect, which is analogous to the Meissner effect in superconductors). We further speculate the existence of the equation ${\bf j}=-Λ\nabla\times \text{\boldmath $ω$}$, where ${\bf j} = n_s{\bf v}_s$ is the superfluid current density, $\text{\boldmath $ω$}=\nabla\times {\bf v}_s$ the superfluid vorticity, and $Λ$ a positive constant (with the help of this equation, the Hess-Fairbank effect can be quantitatively described).

DOI
10.48550/arxiv.0807.1503

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Physical Review•Dec 13, 1965•284 citations
We present a microscopic theory for superfluidity in an interacting many-particle Bose system (such as liquid 4^44He). We show that, similar to superconductivity in superconductors, superfluidity in a Bose system arises from pairing of particles of opposite momenta. We show the existence of an energy gap in single-particle excitation spectrum in the superfluid state and the existence of a specific heat jump at the superfluid transition. We derive an expression for superfluid particle density nsn_sns​ as a function of temperature TTT and superfluid velocity vs{\bf v}_svs​. We show that superfluid-state free energy density FFF is an increasing function of vsv_svs​ (i.e., ∂F/∂vs>0\partial F/\partial v_s > 0∂F/∂vs​>0), which indicates that a superfluid has a tendency to remain motionless (this result qualitatively explains the Hess-Fairbank effect, which is analogous to the Meissner effect in superconductors). We further speculate the existence of the equation {\bf j}=-Λ\nabla\times \text{\boldmath ω}, where j=nsvs{\bf j} = n_s{\bf v}_sj=ns​vs​ is the superfluid current density, \text{\boldmath ω}=\nabla\times {\bf v}_s the superfluid vorticity, and ΛΛΛ a positive constant (with the help of this equation, the Hess-Fairbank effect can be quantitatively described).
A original microscopic theory of superfluidity and superconductivity driven by the single particle (SPC) and pair condensation (PC) of attracting bosons both in Fermi and in Bose systems is developed. This theory (as distinct from the existing theories) for Fermi systems contains two order parameters Δ F and Δ B characterizing the attracting fermion pairs and boson pairs, respectively. In such systems superconducting (SC) phase transition is accompanied, as a rule, by the formation of k-space composite bosons (e.g. Cooper pairs and bipolarons) with their subsequent transition to the superfluid (SF) state by attractive SPC and PC. A novel Fermi-liquid and SF Bose-liquid theories are elaborated for description this two-stage Fermi–Bose-liquid (FBL) scenario of SC (or SF) transition. The crossover from k- to real (r)-space pairing regime for BCS-like coupling constants γ F ≃ 0.7-0.9 and the irrelevance of r-space pairs to the superconductivity are shown. The developed SF Bose-liquid theory predicts the first-order phase transition SPC ↔ PC of attracting 3d-bosons with the kink-like behaviors of all SC (SF) parameters near [Formula: see text] in accordance with the observations in 4 He , 3 He and superconductors. It is argued that the coexistence of the order parameters Δ F and Δ B leads to the superconductivity by two FBL scenarios. One of these scenarios is realized in the so-called fermion (type I, II and III) superconductors (FSC) (where formation of k-space composite bosons and their condensation occur at the same temperature) and the other in the boson (type II and III) superconductors (BSC) (where BCS-like pairing take place in the normal state with manifesting of the second-order phase transition and opening of the pseudogap at T=T F > T c ). There the gapless superfluidity (superconductivity) is caused by the gapless excitation spectrum of bosons at [Formula: see text] and not by the presence of point or line nodes of the BCS-like gap Δ F assumed in some s-, p- and d-pairing models. The 3D- and 2D-insulator–metal–superconductor phase diagrams are presented. The necessary and sufficient microscopic criterions for superfluidity is formulated. The theory proposed are in close agreement with the observations in 4 He , 3 He , superconductors, nuclear and neutron star matter, cosmology, etc.
One considers the superfluid (SF) state of a Bose liquid with a strong repulsion between bosons, in which at T=0, along with a weak single-particle Bose-Einstein condensate (BEC), there exists an intensive pair coherent condensate (PCC), analogous to the Cooper condensate in a Fermi liquid with an attraction between the fermions. Such a PCC emerges in a system of bosons due to an oscillating sign-changing momentum dependence of the Fourier component of the pair interaction potential, which is characteristic of a certain family of repulsion potentials. In such cases, the Fourier component is negative in some domain of nonzero momentum transfer, which corresponds to an effective attraction. The collective effects of renormalization (``screening'') of the initial interaction lead to a suppression of the repulsion and an enhancement of the effective attraction. It is the ratio of the BEC density to the full density of the liquid n0/n≪1n_0/n\ll 1n0​/n≪1 that is used as a small parameter---unlike in the Bogolyubov theory for a quasi-ideal Bose gas, in which the small parameter is the ratio of the number of supracondensate excitations to the number of particles in an intensive BEC, (n−n0)/n0≪1(n-n_0)/n_0\ll 1(n−n0​)/n0​≪1. A closed system of nonlinear integral equations for the normal and anomalous self-energy parts is obtained, in the framework of a renormalized perturbation theory built on combined hydrodynamic and field variables. In the framework of the hard-spheres model, a spectrum of quasiparticles is obtained, which is in good accordance with the experimental spectrum of elementary excitations in superfluid 4^44He. The question of applicability of the Landau criterion in the absence of quantum vortices is discussed.
We conclude our study of superfluidity in Bose liquids with a brief summary of the strengths, and of the inadequacies, of the theory. The cornerstone of our fundamental understanding of superfluidity has been the recognition of the central importance of the condensate, a single quantum state which is macroscopically occupied. For the Bose liquid one has a particle condensate, characterized by a non-vanishing expectation value of ψ (r). The existence of the condensate explains all major aspects of superfluid behavior; in particular, we now possess: A clear understanding of the static and the long wavelength dynamic properties of an equilibrium Bose liquid, including a microscopic basis for the two-fluid model. A precise microscopic theory at T = 0 for a specific model, the dilute Bose gas. Variational calculations of the excitation spectrum of liquid He II (and of the ground state properties as well), which are in good quantitative agreement with experiment. A satisfactory phenomenological treatment of the interactions between elementary excitations which give rise to various irreversible phenomena. A qualitative understanding of the role which is played by quantized vortices in both equilibrium and non-equilibrium phenomena.
The paradoxes and disparities in the contemporary microscopic theory of superfluid helium (He–II) are discussed along with possible ways of resolving them by taking pair correlations of He4 atoms into consideration. It is shown that most paradoxes are associated with the commonly accepted initial assumption concerning the dominating role of single-particle Bose condensate (SPBC) in the quantum microstructure of the superfluid component ρs. The existence of intensive SPBC leads to a strong hybridization of the elementary excitation branches and to a common dispersion law for all boson branches, which is identified with the quasiparticle spectrum E(p) observed experimentally from slow neutron scattering in liquid helium. However, the stability of this spectrum during a transition through the λ-point and the large value of the gap in the vicinity of the “rotonic” minimum contradict both the Landau theoretical criterion of superfluidity and the small value of experimentally measured critical velocity. At the same time, a strong interaction between particles in the Bose liquid He4 strongly suppresses the SPBC which amounts to less than 1% of all He4 atoms and hence cannot be the main constituent of the superfluid component, unlike the case of a weakly nonideal Bose gas. Moreover, for a quite strong attraction between particles in a certain region of the momentum space, bound pairs of bosons can be formed in the superfluid Bose liquid, and a coherent pair condensate (CPC) analogous to the Cooper pair condensate in superconductors may appear. Such a strong CPC may completely suppress the weak SPBC. In this case, the one-particle spectrum ε(p) of elementary excitations does not hybridize with the collective (two-particle) spectrum and does not appear in the structure of the dynamic form factor S(p,ε), i.e., does not coincide with the spectrum measured from neutron scattering. The dispersion of one-particle spectrum is defined by the momentum dependence of the pair order parameter Ψ̃(p) and may have a minimum or a point of inflection at p≠0. This peculiarity in the one-particle spectrum of a Bose liquid with CPC but without SPBC vanishes together with Ψ̃(p) at the temperature Tc=Tλ of the phase transition from the superfluid to the normal state (unlike the rotonic minimum in the collective spectrum), while the corresponding critical velocity vc=min[ε(p)/p] vanishes at the λ-point in accordance with the Landau criterion and the experimental data. The assumption that the strong “Cooper-like” CPC is responsible for the quantum structure of the superfluid component ρs is confirmed indirectly by the successful application of the Justrow approximation (based on strong pair correlations) for describing the properties of liquid He4 and quantum liquid mixtures He3–4He on one hand, and by an anomalously large effective mass of He3 impurity atoms in He4, which is approximately equal to total mass of He3 and He4 atoms, thus pointing to the existence of helium atoms in superfluid liquid He–II. The value of the superfluid velocity circulation quantum in the Onsager–Feynman vortices in a Bose liquid with CPC but without SPBC is discussed as well as the critical velocities of superfluid He4 in ultrathin films and channels in which the creation and motion of quantum vortices are ruled out, and the quasiparticle spectrum undergoes dimensional quantization.
A self-consistent model of the superfluid (SF) state of a Bose liquid with strong interaction between bosons is considered, in which at T=0, along with a weak single-particle Bose-Einstein condensate (BEC), there exists an intensive pair coherent condensate (PCC) of bosons, analogous to the Cooper pair condensate of fermions. Such a PCC emerges due to an effective attraction between bosons in some regions of momentum space, which results from an oscillating sign-changing momentum dependence of the Fourier component V(p) of the interaction potential. The collective many-body effects of renormalization ("screening") of the initial interaction, which are described by the bosonic polarization operator Π(p,ω), lead to a suppression of the repulsion [V(p)>0] and an enhancement of the effective attraction [V(p)<0] in the respective domains of nonzero momentum transfer. The ratio of the BEC density n_0 to the total particle density n of the Bose liquid is used as a small parameter of the model. A closed system of nonlinear integral equations for the normal and anomalous self-energy parts is obtained with account for the terms of first order in the BEC density. In the framework of the ``soft spheres'' model with the single fitting parameter--the value of the repulsion potential at r=0, a theoretical quasiparticle spectrum E(p) is obtained, which is in good accordance with the experimental spectrum E_{exp}(p) of elementary excitations in superfluid 4^44He.
The microscopic theory of a superfluid Fermi liquid at finite temperature is developed for the case of a pure system with SSS-wave pairing, and applied to the calculation of the static properties. As a function of $\ensuremath{\theta}\ensuremath{\equiv}\frac{T}{{T}_{c}}$ these properties are determined entirely by the Landau parameters F0{F}_{0}F0​, F1{F}_{1}F1​, Z0{Z}_{0}Z0​, etc., characterizing quasiparticle interactions in the normal phase. In particular the spin susceptibility $\ensuremath{\chi}$ and the density of the normal component ${\ensuremath{\rho}}_{n}$ are given by $\frac{\ensuremath{\chi}(\ensuremath{\theta})}{\ensuremath{\chi}(1)}=(1+\frac{1}{4}{Z}_{0})\frac{f(\ensuremath{\theta})}{[1+\frac{1}{4}{Z}_{0}f(\ensuremath{\theta})]},$ $\frac{{\ensuremath{\rho}}_{n}}{\ensuremath{\rho}}=(1+\frac{1}{3}{F}_{1})\frac{f(\ensuremath{\theta})}{[1+\frac{1}{3}{F}_{1}f(\ensuremath{\theta})]},$ where the universal function $f(\ensuremath{\theta})\ensuremath{\equiv}\ensuremath{-}{[\ensuremath{\nu}(0)]}^{\ensuremath{-}1}{\ensuremath{\Sigma}}_{\mathrm{p}}(\frac{\mathrm{dn}}{d{E}_{\mathrm{p}}})$ is the "effective density of states near the Fermi surface" relative to its value $\ensuremath{\nu}(0)$ in the normal phase. Thus the often-quoted expression ${\ensuremath{\rho}}_{n}=\frac{1}{3}{\ensuremath{\Sigma}}_{\mathrm{p}}{\mathrm{p}}^{2}(\frac{\mathrm{dn}}{d{E}_{\mathrm{p}}})$ is valid for an interacting system only in the limit $T\ensuremath{\rightarrow}0$. In the latter part of the paper a simple phenomenological theory of "Fermi-liquid" effects on $\ensuremath{\chi}$ and ${\ensuremath{\rho}}_{n}$ is developed for arbitrary conditions (including the presence of impurities and pairing with $l\ensuremath{\ne}0$); it is found that under most circumstances explicit expressions for $\ensuremath{\chi}$ and ${\ensuremath{\rho}}_{n}$ may be obtained which involve only the Landau parameters and a suitably generalized effective density of states. The theory should apply to the possible superfluid phase of He3{\mathrm{He}}^{3}He3 and to most superconductors. It is suggested that the Knight shift in nontransition-metal superconductors should display some "Fermi-liquid" effects. The weak-field dc penetration depth $\ensuremath{\lambda}(T)$ is shown to be insensitive to such effects both in the Pippard limit and near Tc{T}_{c}Tc​; however, in a London superconductor at lower temperatures the correction to $\ensuremath{\lambda}(T)$ should be observable and yield a direct estimate of F1{F}_{1}F1​.