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arXiv:0806.1991 · Bulletin of the American Physical Society

Roton softening and supersolidity in Rb spinor condensates

R. W. Cherng, Eugene Demler

Published Jun 12, 2008• 3 citations
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Abstract

Superfluids with a tendency towards periodic crystalline order have both a phonon and roton like spectrum of collective modes. The softening of the roton spectrum provides one route to a supersolid. We show that roton softening occurs in 87Rb spinor condensates once dipolar interactions and spin dynamics are taken into account. By including the effects of a quasi-two-dimensional geometry and rapid Larmor precession, we show a dynamical instability develops in the collective mode spectrum at finite wavevectors. We construct phase diagrams showing a variety of instabilities as a function of the direction of the magnetic field and strength of the quadratic Zeeman shift. Our results provide a possible explanation of current experiments in the Berkeley group Phys. Rev. Lett. 100:170403 (2008).

DOI
10.48550/arxiv.0806.1991

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Superfluids with a tendency towards periodic crystalline order have both a phonon and roton like spectrum of collective modes. The softening of the roton spectrum provides one route to a supersolid. We show that roton softening occurs in 87Rb spinor condensates once dipolar interactions and spin dynamics are taken into account. By including the effects of a quasi-two-dimensional geometry and rapid Larmor precession, we show a dynamical instability develops in the collective mode spectrum at finite wavevectors. We construct phase diagrams showing a variety of instabilities as a function of the direction of the magnetic field and strength of the quadratic Zeeman shift. Our results provide a possible explanation of current experiments in the Berkeley group Phys. Rev. Lett. 100:170403 (2008).
Roton-type excitations usually emerge from strong correlations or long-range interactions, as in superfluid helium or dipolar ultracold atoms. However, in a weakly short-range interacting quantum gas, the recently synthesized spin-orbit (SO) coupling can lead to various unconventional phases of superfluidity and give rise to an excitation spectrum of roton-maxon character. Using Bragg spectroscopy, we study a SO-coupled Bose-Einstein condensate of ^{87}Rb atoms and show that the excitation spectrum in a "magnetized" phase clearly possesses a two-branch and roton-maxon structure. As Raman coupling strength Ω is decreased, a roton-mode softening is observed, as a precursor of the phase transition to a stripe phase that spontaneously breaks spatially translational symmetry. The measured roton gaps agree well with theoretical calculations. Furthermore, we determine sound velocities both in the magnetized and in the nonmagnetized phases, and a phonon-mode softening is observed around the phase transition in between. The validity of the f-sum rule is examined.
In a recent experiment, it has been found that by tuning the interaction strength of a dipolar Bose-Einstein Condensate confined in a quasi-1D geometry orthogonal to the polarization direction, the roton gap vanishes, while density modulations are induced in the trapped gas. This suggests the possibility of realizing a supersolid in dipolar quantum gases. Inspired by this experiment, we simulate a dipolar BEC in a ring geometry by confining the dipoles in a ”tube” orthogonal to the polarization direction and enforcing periodic boundary conditions. Our calculations are based on a Density Functional approach where the total energy density functional includes the beyond-mean-field correction of Lee-Huang-Yang, which partially accounts for quantum fluctuations. We study the ground state properties of the system by evolving in imaginary time the EulerLagrange equation derived from the variational principle. We also study the excitation spectrum of the system by solving the corresponding Bogoliubov-de Gennes equations. We find that the calculated excitation spectrum shows indeed a roton minimum, and the roton gap can become vanishingly small by reducing the effective scattering length. As the roton gap disappears, we find that the system spontaneously develops in its ground-state a periodic structure formed by denser clusters of atomic dipoles immersed in a dilute superfluid background. We find that this structure shows the hallmarks of a supersolid system, i.e. (i) a finite non-classical translational inertia and (ii) the appearance, besides the phonon mode, of the Nambu-Goldstone gapless mode corresponding to fluctuations in the phase, and related to the spontaneous breaking of the gauge symmetry.
We investigate the collective excitation spectrum and dynamics of a quasi two-dimensional spin-1 Bose-Einstein condensate with Rashba type spin-orbit (SO) coupling. Employing Bogoliubov-de-Gennes analysis, we analytically compute the excitation spectra across a wide range of interaction strengths and coupling parameters. By systematically varying the SO and Rabi couplings, we uncover distinct dynamical signatures of quantum phase transitions, including mode softening, the appearance of roton-like minima, and miscibility-driven instabilities in both ferromagnetic and antiferromagnetic interaction regimes. In the antiferromagnetic case, these instabilities lead to a dynamically unstable supersolid phase characterized by the coexistence of density modulation and global phase coherence. To corroborate the analytical predictions, we numerically solve the coupled Gross-Pitaevskii equations and analyze the dynamical stability of the condensate. Our results provide experimentally accessible signatures for spinor condensates with tunable spin-orbit coupling and demonstrate the rich interplay between spin-dependent interactions and synthetic couplings in nonequilibrium quantum fluids.
Dipolar condensates have recently been coaxed to form the long-sought supersolid phase. While one-dimensional supersolids may be prepared by triggering a roton instability, we find that such a procedure in two dimensions (2D) leads to a loss of both global phase coherence and crystalline order. Unlike in 1D, the 2D roton modes have little in common with the supersolid configuration. We develop a finite-temperature stochastic Gross-Pitaevskii theory that includes beyond-mean-field effects to explore the formation process in 2D and find that evaporative cooling directly into the supersolid phase-hence bypassing the first-order roton instability-can produce a robust supersolid in a circular trap. Importantly, the resulting supersolid is stable at the final nonzero temperature. We then experimentally produce a 2D supersolid in a near-circular trap through such an evaporative procedure. Our work provides insight into the process of supersolid formation in 2D and defines a realistic path to the formation of large two-dimensional supersolid arrays.
We characterize the role of roton instability in the formation of a supersolid state of an elongated dipolar condensate, following a quench of the contact interactions across the superfluid-supersolid transition, as observed in recent experiments. We perform dynamical simulations by means of the extended Gross-Pitaevskii equation including quantum corrections, for different final values of the $s\text{\ensuremath{-}}\mathrm{wave}$ scattering length. The corresponding excitation spectrum is computed using an effective one-dimensional description, which provides a reasonably accurate prediction for the growth rate of the most unstable mode observed in the simulations. To analyze the behavior of the system, we employ the inverse participation ratio, which conveniently characterizes the different degree of localization in the superfluid and supersolid phases. By means of a suitable effective ansatz for the density, we derive a simple yet effective expression for the formation time of the supersolid. This expression provides valuable insights regarding its scaling behavior with respect to the sss-wave scattering length.