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Physical Review Letters

Magnetoroton Softening in Rb Spinor Condensates with Dipolar Interactions

R. W. Cherng, Eugene Demler

Published Oct 27, 2009• 31 citations
Publisher

Abstract

Superfluids with a tendency towards periodic order have both phonon- and rotonlike spectra. We show that magnetoroton softening occurs in 87Rb spinor condensates. A rich variety of dynamical instabilities emerges as a function of the magnetic field orientation and strength of the quadratic Zeeman shift. These instabilities are driven by an effective dipolar interaction modified dramatically by quasi-two-dimensionality and rapid Larmor precession.

DOI
10.1103/physrevlett.103.185301

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Superfluids with a tendency towards periodic order have both phonon- and rotonlike spectra. We show that magnetoroton softening occurs in 87Rb spinor condensates. A rich variety of dynamical instabilities emerges as a function of the magnetic field orientation and strength of the quadratic Zeeman shift. These instabilities are driven by an effective dipolar interaction modified dramatically by quasi-two-dimensionality and rapid Larmor precession.
Superfluids with a tendency towards periodic crystalline order have both a phonon and roton like spectrum of collective modes. The softening of the roton spectrum provides one route to a supersolid. We show that roton softening occurs in 87Rb spinor condensates once dipolar interactions and spin dynamics are taken into account. By including the effects of a quasi-two-dimensional geometry and rapid Larmor precession, we show a dynamical instability develops in the collective mode spectrum at finite wavevectors. We construct phase diagrams showing a variety of instabilities as a function of the direction of the magnetic field and strength of the quadratic Zeeman shift. Our results provide a possible explanation of current experiments in the Berkeley group Phys. Rev. Lett. 100:170403 (2008).
Roton-type excitations usually emerge from strong correlations or long-range interactions, as in superfluid helium or dipolar ultracold atoms. However, in a weakly short-range interacting quantum gas, the recently synthesized spin-orbit (SO) coupling can lead to various unconventional phases of superfluidity and give rise to an excitation spectrum of roton-maxon character. Using Bragg spectroscopy, we study a SO-coupled Bose-Einstein condensate of ^{87}Rb atoms and show that the excitation spectrum in a "magnetized" phase clearly possesses a two-branch and roton-maxon structure. As Raman coupling strength Ω is decreased, a roton-mode softening is observed, as a precursor of the phase transition to a stripe phase that spontaneously breaks spatially translational symmetry. The measured roton gaps agree well with theoretical calculations. Furthermore, we determine sound velocities both in the magnetized and in the nonmagnetized phases, and a phonon-mode softening is observed around the phase transition in between. The validity of the f-sum rule is examined.
We study the effects of quasiparticle interactions in a quasi-two-dimensional (quasi-2D), zero-temperature Bose-Einstein condensate of dipolar atoms, which can exhibit a roton-maxon feature in its quasiparticle spectrum. Our focus is the Beliaev damping process, in which a quasiparticle collides with the condensate and resonantly decays into a pair of quasiparticles. Remarkably, the rate for this process exhibits a highly nontrivial dependence on the quasiparticle momentum and the dipolar interaction strength. For weak interactions, low-energy phonons experience no damping, and higher-energy quasiparticles undergo anomalously weak damping. In contrast, the Beliaev damping rates become anomalously large for stronger dipolar interactions, as rotons become energetically accessible as final states. When the dipoles are tilted off the axis of symmetry, the damping rates acquire an anisotropic character. Surprisingly, this anisotropy does not simply track the anisotropy of the dipolar interactions, rather, the mechanisms for damping are qualitatively modified in the anisotropic case. Our study reveals the unconventional nature of Beliaev damping in dipolar condensates, and has important implications for ongoing studies of equilibrium and nonequilibrium dynamics in these systems. Further, our results are relevant for other 2D superfluids with roton excitations, including spin-orbit-coupled Bose gases, magnon condensates, and 4He^{4}\mathrm{He}4He films.
Selected topics on spinor-dipolar aspects of Bose-Einstein condensation are overviewed. Spinor aspects include spin correlations, fragmentation, dynamical symmetries, and quantum mass acquisition. Dipolar aspects include magnetostriction, d-wave collapse, roton-maxon spectrum, supersolidity, and ferrofluidity. Finally, spinor-dipolar aspects concern the Einstein–de Haas effect and spontaneous mass and spin currents in the ground state. Introduction Bose-Einstein condensation is a phenomenon in which a macroscopic number of particles occupy the same single-particle state as a consequence of symmetrization of a many-body wave function and thereby quantum effects are amplified to the macroscopic level. The amplified single-particle state serves as a complex order parameter whose phase behaves as an emergent thermodynamic quantity, with its temporal and spatial variations giving the chemical potential and the superfluid velocity, respectively. If the interparticle interaction is repulsive, a Bose-Einstein condensate (BEC) acquires stability against excitations out of the condensate because they would cost the Fock exchange energy. This rigidity of the order parameter or the condensate wave function endows a BEC with several remarkable transport properties which are collectively known as superfluidity. In particular, the superfluid fraction can be 100% at zero temperature even though the condensate fraction is depleted due to interparticle interactions. Interparticle interactions also make excited particles phase-locked to the condensate, leading to Bogoliubov quasiparticles, which are the manifestation of phase-coherent particle– hole excitations. When constituent particles have spin degrees of freedom, a BEC features magnetism and spin nematicity which conspire with superfluidity to produce a rich phase diagram. In the absence of an external magnetic field, the mean-field groundstate phase diagram includes two [1, 2], five [3, 4, 5], and eleven phases [6, 7] for spin-1, 2, and 3 BECs, respectively. BECs with spin degrees of freedom are called spinor condensates. Moreover, the magnetic dipole–dipole interaction (MDDI) between atoms lends distinct twists to spinor condensates because it is long-ranged and anisotropic in sharp contrast with other interactions, which are short-ranged and isotropic. In this chapter, we will present a brief overview on the spinordipolar aspects of BEC. An early experimental work of spinor BECs is reviewed in Ref. [8]. Later developments with an emphasis on theoretical aspects are described in Ref. [9]. Many-body physics of polarized dipolar gases is reviewed in Ref. [10].
We show that metastable phases of an antiferromagnetic spin-1 condensate in a simple model with pure contact interactions can exhibit a rotonlike minimum in the excitation spectrum. The introduction of a magnetic field gives rise to the instability of roton modes, which can lead to spontaneous emergence of regular periodic, polygonal, polyhedral, or crystalline patterns, as shown in numerical simulations within the truncated Wigner approximation. An explanation of the occurrence of rotonlike instability is given based on the energy and spin conservation laws.