We compute the dynamics of excitation and two-body correlation for two-level 'pseudoatoms' in a one-dimensional (1D) lattice. We adopt a simplified model where pair excitation within a finite range is perfectly blocked. Each superatom is initially in the ground state, and then subjected to an external driving laser with Rabi frequency satisfying a Poissonian distribution, mimicking the scenario in Rydberg gases. We find that two-body quantum correlation drops very fast with the distance between pseudoatoms. However, the total correlation decays slowly even at large distance. Our results may be useful to the understanding of Rydberg gases in the strong blockade regime.
We compute the dynamics of excitation and two-body correlation for two-level 'pseudoatoms' in a one-dimensional (1D) lattice. We adopt a simplified model where pair excitation within a finite range is perfectly blocked. Each superatom is initially in the ground state, and then subjected to an external driving laser with Rabi frequency satisfying a Poissonian distribution, mimicking the scenario in Rydberg gases. We find that two-body quantum correlation drops very fast with the distance between pseudoatoms. However, the total correlation decays slowly even at large distance. Our results may be useful to the understanding of Rydberg gases in the strong blockade regime.
We study the excitation dynamics of Rydberg atoms in a one-dimensional lattice with periodic boundary conditions where the atomic Rydberg states are resonantly excited from the electronic ground state. Our description of the corresponding dynamics is numerically exact within the perfect blockade regime, i.e., no two atoms in a given range can be excited. The time evolution of the mean Rydberg density, density-density correlations, as well as entanglement properties is analyzed in detail. We demonstrate that the short-time dynamics is universal and dominated by quantum phenomena, while for larger time the characteristics of the lattice become important and the classical features determine the dynamics. The results of the perfect blockade approach are compared to the predictions of an effective Hamiltonian which includes the interaction of two neighboring Rydberg atoms up to the second-order perturbation theory.
In this thesis I present several theoretical methods to explore the excitation dynamics of Ultracold Rydberg systems in various regimes. For some applications the details of interactions between Rydberg atoms have to be carefully examined, while for others, the many-body aspect of Rydberg excitation may be crucial. In both cases, the basic prerequisite is to know the interactions sufficiently well. I will review the basic concepts how to evaluate molecular potentials in various Hund's cases and approximations. Long-range Rydberg-Rydberg interactions between Rydberg atoms induce ℓ-mixing which in certain situations gives rise to molecular resonances. For these resonances, we calculate long-range potentials in Hund's case (c) by diagonalization of an interaction matrix. The excitation dynamics of the resonances is always modeled as pair excitation. At high principal quantum number n, the interactions between Rydberg atoms can blockade the excitation of many surrounding atoms in the range of few μm. The atoms within this range are strongly correlated so that many-body treatments are, in general, needed. To describe this blockading effect and other manifestations of the collective behavior of Rydberg excitation, such as the many-body Rabi oscillations, spatial correlations between atoms and the fluctuations of the number of excited atoms, I have used three different approaches. In the mean-field approach the interactions between different atoms is modeled by a distribution of mean-field shifts for which a distribution of probabilities is calculated, A good agreement between the theoretical model and experimental measurements is found. To study the correlations between atoms the many-body wavefunction is numerically computed. The possibility of observing the many-body Rabi oscillations of Rydberg excitation and other aspects of many-body dynamics is analyzed. Although strong interactions cannot be treated perturbatively other expansions may be feasible. I will show that the expansion in powers of the single atom Rabi frequency can be evaluated in the interaction and Heisenberg picture. The expansion is expected to behave well for arbitrary strong interactions. ^
Owing to the unique physical characteristics of Rydberg atoms, which play an important role in quantum information and quantum computation, the theoretical and applied research of Rydberg atoms have become the hot spots of scientific research in recent years. With the large polarizability of Rydberg atoms, even a small electric field could cause a considerable electric dipole moment, resulting in a strong dipole-dipole interaction between Rydberg atoms. The multiple excitations of the Rydberg states are strongly inhibited because of the strong dipole interaction between atoms within a mesoscopic interaction (blockade) region. We call this phenomenon the dipole blockade effect. The dipole blockade effect makes it possible to build single-photon quantum devices, implement quantum gates, generate quantum entanglement, and simulate many-body quantum problems, etc. A Rydberg atomic ensemble in the same blockade region can be regarded as a superatom. In the same way, if these atoms trapped in two optical dipole traps, each sub-ensemble can be considered as a sub-superatom which is closely related to the superatom. According to the fact that two Rydberg sub-superatoms can be strongly correlated due to sharing no more than one excited Rydberg atom, we study correlated collective excitation and quantum entanglement between two Rydberg sub-superatoms in a steady state. With the superatom model, the problem of exponentially increasing system size with the number of atoms can be circumvented to a certain extent in studying many-body physics. By solving the two-body Lindblad’s master equation accurately, we obtain the analytical expressions for the collective excitation probabilities of the two sub-superatoms, and the concurrence measuring the bipartite entanglement between them. Our results show that they are all sensitive to the number of atoms in each Rydberg superatom: the bigger (including more atoms) the Rydberg superatom, the higher the collective Rydberg excitation probability is. And that the maximally entangled state can only be obtained with two equal-sized Rydberg superatoms. When this condition is fulfilled, the mesoscopic entanglement can be generated by adding the number of atoms in each Rydberg superatom. This may provide an attractive platform for studying the quantum-classical correspondence and have potential promising applications in quantum information processing.
Recent achievements in ultra-cold experiments have made quantum simulation of interacting many-body systems possible in a well controllable environment. Of many candidates as quantum simulators, Rydberg atoms have been extensively utilised due to its exaggerated and fascinating atomic properties. Example includes high susceptibility to electric fields and relatively long life time in comparison to atoms in low-lying states. The tunable interaction between Rydberg atoms have made them even more versatile in simulating quantum many-body systems, e.g. interacting spin-1/2 particles. We will start the thesis by reviewing these properties of Rydberg atoms and explain how they lead to the Rydberg lattice gases that of interest. Following the review of the essential knowledge of Rydberg atoms, we first study the ground states of interacting Rydberg lattice gases in both one-dimension and two-dimensions. The many-body system we are interested in is initially prepared in a Mott-insulator state, with each lattice site containing one atom that is laser coupled to its highly excited Rydberg state. The extremely huge van der Waals interactions between Rydberg atoms at close distance leads to an interesting Rydberg blockade effect. As we shall show, these strong interactions lead to rich phases and critical behaviours in the ground states of the many-body Hamiltonians that describes the systems. The aim of the first three chapters is to analyse these ground states in detail. Having investigated the static properties, we then move on to study the dynamical behaviour of a class of generic spin models which can in principal be realised by Rydberg lattice gases with tunable blockade radius. By deriving an effective master equation, and comparing it to the exact calculation, we will demonstrate how different pure initial states eventually evolve to the same equilibrium state and analysed in detail the time evolution and the steady state.
We investigate the excitation of a collection of cold atoms to Rydberg states. By a direct numerical solution of Schrödinger's equation, we are able to compute various interesting properties of the many-body wavefunction. The high polarizability of Rydberg atoms allows them to support large dipole moments which in turn can interact with each other over long ranges. If the interaction energy between excited atoms is large enough, the resultant energy shift will move the two excitation states out of resonance, thus effectively blocking a two excitation state from occurring. One particular topic investigated is the quantum phase gate, where both groups of atoms are within a blockade radius R b and subjected to a π − 2π − π sequence of pulses. We examine the regime where the groups are neither totally within nor totally outside the blockade radius. Our results explore the tolerance in variation of intergroup lattice distances for a series of quantum gates.
We study many-body correlations in the stationary state of a continuously driven, strongly interacting dissipative system. Specifically, we examine resonant optical excitations of Rydberg states of atoms interacting via long-range dipole-dipole and van der Waals potentials employing numerical and analytical techniques. Collection of atoms within a blockade distance form a ``superatom'' that can accommodate at most one Rydberg excitation. The superatom excitation probability saturates to 21 for coherently driven atoms but is significantly higher in the presence of dephasing, approaching unity as the number of atoms increases. Using the exact numerical solution of the density-matrix equations for a small system, we demonstrate that strong dephasing of the optically driven dipoles renders the many-body problem amenable to semiclassical Monte Carlo simulations. We employ the Monte Carlo algorithm for a large number of atoms and find that in the steady state of a uniformly driven, extended one-dimensional system, the saturation of superatoms leads to quasicrystallization of Rydberg excitations whose correlations exhibit damped spatial oscillations. We show that the behavior of the system under the van der Waals interaction potential can be approximated by a rate-equations model based on a ``hard-rod'' interatomic potential, and by solving it we obtain the period and correlation length for the density wave of Rydberg excitations.