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arXiv:0812.4894 · Physical Review A

Collective Rydberg excitations of an atomic gas confined in a ring lattice

Beatriz Olmos, Rosario González‐Férez, Igor Lesanovsky

Published Apr 24, 2009• 39 citations
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Abstract

We study the excitation dynamics of Rydberg atoms in a one-dimensional lattice with periodic boundary conditions where the atomic Rydberg states are resonantly excited from the electronic ground state. Our description of the corresponding dynamics is numerically exact within the perfect blockade regime, i.e., no two atoms in a given range can be excited. The time evolution of the mean Rydberg density, density-density correlations, as well as entanglement properties is analyzed in detail. We demonstrate that the short-time dynamics is universal and dominated by quantum phenomena, while for larger time the characteristics of the lattice become important and the classical features determine the dynamics. The results of the perfect blockade approach are compared to the predictions of an effective Hamiltonian which includes the interaction of two neighboring Rydberg atoms up to the second-order perturbation theory.

DOI
10.1103/physreva.79.043419

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We study the excitation dynamics of Rydberg atoms in a one-dimensional lattice with periodic boundary conditions where the atomic Rydberg states are resonantly excited from the electronic ground state. Our description of the corresponding dynamics is numerically exact within the perfect blockade regime, i.e., no two atoms in a given range can be excited. The time evolution of the mean Rydberg density, density-density correlations, as well as entanglement properties is analyzed in detail. We demonstrate that the short-time dynamics is universal and dominated by quantum phenomena, while for larger time the characteristics of the lattice become important and the classical features determine the dynamics. The results of the perfect blockade approach are compared to the predictions of an effective Hamiltonian which includes the interaction of two neighboring Rydberg atoms up to the second-order perturbation theory.
When Rydberg states are excited in a dense atomic gas, the mean number of excited atoms reaches a stationary value after an initial transient period. We shed light on the origin of this steady state that emerges from a purely coherent evolution of a closed system. To this end, we consider a one-dimensional ring lattice and employ the perfect blockade model, i.e. the simultaneous excitation of Rydberg atoms occupying neighboring sites is forbidden. We derive an equation of motion that governs the system's evolution in excitation number space. This equation possesses a steady state that is strongly localized. Our findings show that this state is, to good accuracy, given by the density matrix of the microcanonical ensemble where the corresponding microstates are the zero-energy eigenstates of the interaction Hamiltonian. We analyze the statistics of the Rydberg atom number count, providing expressions for the number of excited Rydberg atoms and the Mandel Q -parameter in equilibrium.
We investigate the dynamics of a strongly interacting spin system that is motivated by current experimental realizations of strongly interacting Rydberg gases in lattices. In particular, we are interested in the temporal evolution of quantities such as the density of Rydberg atoms and density–density correlations when the system is initialized in a fully polarized state without Rydberg excitations. We show that in the thermodynamic limit the expectation values of these observables converge at least logarithmically to universal functions and outline a method to obtain these functions. We prove that a finite one-dimensional system follows this universal behavior up to a given time. The length of this universal time period depends on the actual system size. This shows that the study of small systems allows us to make precise predictions about the thermodynamic limit provided that the observation time is sufficiently short. We discuss this for various observables and for systems with different dimensions, interaction ranges and boundary conditions.
When Rydberg states are excited in a dense atomic gas the mean number of excited atoms reaches a stationary value after an initial transient period. We shed light on the origin of this steady state that emerges from a purely coherent evolution of a closed system. To this end we consider a one-dimensional ring lattice, and employ the perfect blockade model, i.e. the simultaneous excitation of Rydberg atoms occupying neighboring sites is forbidden. We derive an equation of motion which governs the system's evolution in excitation number space. This equation possesses a steady state which is strongly localized. Our findings show that this state is to a good accuracy given by the density matrix of the microcanonical ensemble where the corresponding microstates are the zero energy eigenstates of the interaction Hamiltonian. We analyze the statistics of the Rydberg atom number count providing expressions for the number of excited Rydberg atoms and the Mandel Q-parameter in equilibrium.
We study the conditions for attaining crystalline order in the stationary state of a continuously driven, open many-body system. Specifically, we consider resonant optical excitations of atoms in a one-dimensional lattice to the Rydberg states interacting via the van der Waals potential. Strong blockade of excitations at neighboring lattice sites steers the system toward a crystalline state while competing with the fluctuations associated with relaxation. We analyze the stationary state of the many-body system and the dynamics of its buildup employing numerically exact time-dependent density-matrix renormalization-group simulations for two- and three-level excitation schemes. We also present an approximate rate equation model which provides qualitative conditions for attaining crystalline order.
Recent achievements in ultra-cold experiments have made quantum simulation of interacting many-body systems possible in a well controllable environment. Of many candidates as quantum simulators, Rydberg atoms have been extensively utilised due to its exaggerated and fascinating atomic properties. Example includes high susceptibility to electric fields and relatively long life time in comparison to atoms in low-lying states. The tunable interaction between Rydberg atoms have made them even more versatile in simulating quantum many-body systems, e.g. interacting spin-1/2 particles. We will start the thesis by reviewing these properties of Rydberg atoms and explain how they lead to the Rydberg lattice gases that of interest. Following the review of the essential knowledge of Rydberg atoms, we first study the ground states of interacting Rydberg lattice gases in both one-dimension and two-dimensions. The many-body system we are interested in is initially prepared in a Mott-insulator state, with each lattice site containing one atom that is laser coupled to its highly excited Rydberg state. The extremely huge van der Waals interactions between Rydberg atoms at close distance leads to an interesting Rydberg blockade effect. As we shall show, these strong interactions lead to rich phases and critical behaviours in the ground states of the many-body Hamiltonians that describes the systems. The aim of the first three chapters is to analyse these ground states in detail. Having investigated the static properties, we then move on to study the dynamical behaviour of a class of generic spin models which can in principal be realised by Rydberg lattice gases with tunable blockade radius. By deriving an effective master equation, and comparing it to the exact calculation, we will demonstrate how different pure initial states eventually evolve to the same equilibrium state and analysed in detail the time evolution and the steady state.
We study the dynamics of a one-dimensional Rydberg lattice gas under facilitation (anti-blockade) conditions which implements a so-called kinetically constrained spin system. Here an atom can only be excited to a Rydberg state when one of its neighbors is already excited. Once two or more atoms are simultaneously excited mechanical forces emerge, which couple the internal electronic dynamics of this many-body system to external vibrational degrees of freedom in the lattice. This electron-phonon coupling results in a so-called phonon dressing of many-body states which in turn impacts on the facilitation dynamics. In our theoretical study we focus on a scenario in which all energy scales are sufficiently separated such that a perturbative treatment of the coupling between electronic and vibrational states is possible. This allows to analytically derive an effective Hamiltonian for the evolution of clusters of consecutive Rydberg excitations in the presence of phonon dressing. We analyze the spectrum of this Hamiltonian and show --- by employing Fano resonance theory --- that the interaction between Rydberg excitations and lattice vibrations leads to the emergence of slowly decaying bound states that inhibit fast relaxation of certain initial states.