Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1208.2911 · Physical Review A

Steady-state crystallization of Rydberg excitations in an optically driven lattice gas

Michael Höning, Dominik Muth, David Petrosyan, Michael Fleischhauer

Published Feb 4, 2013• 98 citations
arXivHTMLPDF

Abstract

We study the conditions for attaining crystalline order in the stationary state of a continuously driven, open many-body system. Specifically, we consider resonant optical excitations of atoms in a one-dimensional lattice to the Rydberg states interacting via the van der Waals potential. Strong blockade of excitations at neighboring lattice sites steers the system toward a crystalline state while competing with the fluctuations associated with relaxation. We analyze the stationary state of the many-body system and the dynamics of its buildup employing numerically exact time-dependent density-matrix renormalization-group simulations for two- and three-level excitation schemes. We also present an approximate rate equation model which provides qualitative conditions for attaining crystalline order.

DOI
10.1103/physreva.87.023401

Related papers

Spatial correlations of Rydberg excitations in optically driven atomic ensembles

David Petrosyan, Michael Höning, Michael Fleischhauer

We study many-body correlations in the stationary state of a continuously driven, strongly interacting dissipative system. Specifically, we examine resonant optical excitations of Rydberg states of atoms interacting via long-range dipole-dipole and van der Waals potentials employing numerical and analytical techniques. Collection of atoms within a blockade distance form a ``superatom'' that can accommodate at most one Rydberg excitation. The superatom excitation probability saturates to $\frac{1}{2}$ for coherently driven atoms but is significantly higher in the presence of dephasing, approaching unity as the number of atoms increases. Using the exact numerical solution of the density-matrix equations for a small system, we demonstrate that strong dephasing of the optically driven dipoles renders the many-body problem amenable to semiclassical Monte Carlo simulations. We employ the Monte Carlo algorithm for a large number of atoms and find that in the steady state of a uniformly driven, extended one-dimensional system, the saturation of superatoms leads to quasicrystallization of Rydberg excitations whose correlations exhibit damped spatial oscillations. We show that the behavior of the system under the van der Waals interaction potential can be approximated by a rate-equations model based on a ``hard-rod'' interatomic potential, and by solving it we obtain the period and correlation length for the density wave of Rydberg excitations.

arXiv:1212.2423•Physical Review A•May 28, 2013•76 citations

Two-dimensional crystals of Rydberg excitations in a resonantly driven lattice gas

David Petrosyan

The competition between resonant optical excitation of Rydberg states of atoms and their strong, long-range van der Waals interaction results in spatial ordering of Rydberg excitations in a two-dimensional lattice gas, as observed in a recent experiment of Schau\ss{} et al. [Nature (London) 491, 87 (2012)]. Here we use semiclassical Monte Carlo simulations to obtain stationary states for hundreds of atoms in finite-size lattices. We show the formation of regular spatial structures of Rydberg excitations in a system of increasing size, and find highly sub-Poissonian distribution of the number of Rydberg excitations characterized by a large negative value of the Mandel $Q$ parameter which is nearly independent of the system size.

arXiv:1306.0320•Physical Review A•Oct 28, 2013•26 citations

Driven-Dissipative Rydberg Blockade in Optical Lattices

Javad Kazemi, Hendrik Weimer

While dissipative Rydberg gases exhibit unique possibilities to tune dissipation and interaction properties, very little is known about the quantum many-body physics of such long-range interacting open quantum systems. We theoretically analyze the steady state of a van der Waals interacting Rydberg gas in an optical lattice based on a variational treatment that also includes long-range correlations necessary to describe the physics of the Rydberg blockade, i.e., the inhibition of neighboring Rydberg excitations by strong interactions. In contrast to the ground state phase diagram, we find that the steady state undergoes a single first order phase transition from a blockaded Rydberg gas to a facilitation phase where the blockade is lifted. The first order line terminates in a critical point when including sufficiently strong dephasing, enabling a highly promising route to study dissipative criticality in these systems. In some regimes, we also find good quantitative agreement of the phase boundaries with previously employed short-range models, however, with the actual steady states exhibiting strikingly different behavior.

arXiv:2209.00039•Physical Review Letters•Apr 19, 2023•10 citations

Spontaneous formation of one-dimensional Rydberg crystals in an ultracold gas

T.H.P. van der Weerden, S. J. J. M. F. Kokkelmans, Edgar J. D. Vredenbregt

Rydberg atoms have experimentally interestingproperties such as strong long-range Van der Waals interactions and the dipole blockade effect. In optical lattices the blockade effect ensures that only one Rydberg excitation per site is allowed, effectively creating a Rydberg crystal. We theoretically show that it is also possible for a one-dimensional Rydberg crystal to spontaneously form in a random ensemble of atoms, e.g. a magneto-optical trap. This is done using an existing Monte Carlo model [1] to simulate the excitation dynamics inside the intersection of two lasers for a two-step excitation scheme. With a blue-detuned laser for the upper transition, the first Rydberg excitation will occur after a relatively long time. That first Rydberg atom will then seed further Rydberg excitations, as the blockade effect shifts atoms at a certain distance into resonance. If two dimensions of the laser intersection are smaller than the blockade radius, a one-dimensional Rydberg crystal will form.

•Jan 1, 2016•0 citations

Thermalization of a strongly interacting 1D Rydberg lattice gas

Beatriz Olmos, Markus Müller, Igor Lesanovsky

When Rydberg states are excited in a dense atomic gas, the mean number of excited atoms reaches a stationary value after an initial transient period. We shed light on the origin of this steady state that emerges from a purely coherent evolution of a closed system. To this end, we consider a one-dimensional ring lattice and employ the perfect blockade model, i.e. the simultaneous excitation of Rydberg atoms occupying neighboring sites is forbidden. We derive an equation of motion that governs the system's evolution in excitation number space. This equation possesses a steady state that is strongly localized. Our findings show that this state is, to good accuracy, given by the density matrix of the microcanonical ensemble where the corresponding microstates are the zero-energy eigenstates of the interaction Hamiltonian. We analyze the statistics of the Rydberg atom number count, providing expressions for the number of excited Rydberg atoms and the Mandel Q -parameter in equilibrium.

arXiv:0907.4420•New Journal of Physics•Jan 28, 2010•38 citations

Collective Rydberg excitations of an atomic gas confined in a ring lattice

Beatriz Olmos, Rosario González‐Férez, Igor Lesanovsky

We study the excitation dynamics of Rydberg atoms in a one-dimensional lattice with periodic boundary conditions where the atomic Rydberg states are resonantly excited from the electronic ground state. Our description of the corresponding dynamics is numerically exact within the perfect blockade regime, i.e., no two atoms in a given range can be excited. The time evolution of the mean Rydberg density, density-density correlations, as well as entanglement properties is analyzed in detail. We demonstrate that the short-time dynamics is universal and dominated by quantum phenomena, while for larger time the characteristics of the lattice become important and the classical features determine the dynamics. The results of the perfect blockade approach are compared to the predictions of an effective Hamiltonian which includes the interaction of two neighboring Rydberg atoms up to the second-order perturbation theory.

arXiv:0812.4894•Physical Review A•Apr 24, 2009•39 citations
We study the conditions for attaining crystalline order in the stationary state of a continuously driven, open many-body system. Specifically, we consider resonant optical excitations of atoms in a one-dimensional lattice to the Rydberg states interacting via the van der Waals potential. Strong blockade of excitations at neighboring lattice sites steers the system toward a crystalline state while competing with the fluctuations associated with relaxation. We analyze the stationary state of the many-body system and the dynamics of its buildup employing numerically exact time-dependent density-matrix renormalization-group simulations for two- and three-level excitation schemes. We also present an approximate rate equation model which provides qualitative conditions for attaining crystalline order.
We study many-body correlations in the stationary state of a continuously driven, strongly interacting dissipative system. Specifically, we examine resonant optical excitations of Rydberg states of atoms interacting via long-range dipole-dipole and van der Waals potentials employing numerical and analytical techniques. Collection of atoms within a blockade distance form a ``superatom'' that can accommodate at most one Rydberg excitation. The superatom excitation probability saturates to 12\frac{1}{2}21​ for coherently driven atoms but is significantly higher in the presence of dephasing, approaching unity as the number of atoms increases. Using the exact numerical solution of the density-matrix equations for a small system, we demonstrate that strong dephasing of the optically driven dipoles renders the many-body problem amenable to semiclassical Monte Carlo simulations. We employ the Monte Carlo algorithm for a large number of atoms and find that in the steady state of a uniformly driven, extended one-dimensional system, the saturation of superatoms leads to quasicrystallization of Rydberg excitations whose correlations exhibit damped spatial oscillations. We show that the behavior of the system under the van der Waals interaction potential can be approximated by a rate-equations model based on a ``hard-rod'' interatomic potential, and by solving it we obtain the period and correlation length for the density wave of Rydberg excitations.
The competition between resonant optical excitation of Rydberg states of atoms and their strong, long-range van der Waals interaction results in spatial ordering of Rydberg excitations in a two-dimensional lattice gas, as observed in a recent experiment of Schau\ss{} et al. [Nature (London) 491, 87 (2012)]. Here we use semiclassical Monte Carlo simulations to obtain stationary states for hundreds of atoms in finite-size lattices. We show the formation of regular spatial structures of Rydberg excitations in a system of increasing size, and find highly sub-Poissonian distribution of the number of Rydberg excitations characterized by a large negative value of the Mandel QQQ parameter which is nearly independent of the system size.
While dissipative Rydberg gases exhibit unique possibilities to tune dissipation and interaction properties, very little is known about the quantum many-body physics of such long-range interacting open quantum systems. We theoretically analyze the steady state of a van der Waals interacting Rydberg gas in an optical lattice based on a variational treatment that also includes long-range correlations necessary to describe the physics of the Rydberg blockade, i.e., the inhibition of neighboring Rydberg excitations by strong interactions. In contrast to the ground state phase diagram, we find that the steady state undergoes a single first order phase transition from a blockaded Rydberg gas to a facilitation phase where the blockade is lifted. The first order line terminates in a critical point when including sufficiently strong dephasing, enabling a highly promising route to study dissipative criticality in these systems. In some regimes, we also find good quantitative agreement of the phase boundaries with previously employed short-range models, however, with the actual steady states exhibiting strikingly different behavior.
Rydberg atoms have experimentally interestingproperties such as strong long-range Van der Waals interactions and the dipole blockade effect. In optical lattices the blockade effect ensures that only one Rydberg excitation per site is allowed, effectively creating a Rydberg crystal. We theoretically show that it is also possible for a one-dimensional Rydberg crystal to spontaneously form in a random ensemble of atoms, e.g. a magneto-optical trap. This is done using an existing Monte Carlo model [1] to simulate the excitation dynamics inside the intersection of two lasers for a two-step excitation scheme. With a blue-detuned laser for the upper transition, the first Rydberg excitation will occur after a relatively long time. That first Rydberg atom will then seed further Rydberg excitations, as the blockade effect shifts atoms at a certain distance into resonance. If two dimensions of the laser intersection are smaller than the blockade radius, a one-dimensional Rydberg crystal will form.
When Rydberg states are excited in a dense atomic gas, the mean number of excited atoms reaches a stationary value after an initial transient period. We shed light on the origin of this steady state that emerges from a purely coherent evolution of a closed system. To this end, we consider a one-dimensional ring lattice and employ the perfect blockade model, i.e. the simultaneous excitation of Rydberg atoms occupying neighboring sites is forbidden. We derive an equation of motion that governs the system's evolution in excitation number space. This equation possesses a steady state that is strongly localized. Our findings show that this state is, to good accuracy, given by the density matrix of the microcanonical ensemble where the corresponding microstates are the zero-energy eigenstates of the interaction Hamiltonian. We analyze the statistics of the Rydberg atom number count, providing expressions for the number of excited Rydberg atoms and the Mandel Q -parameter in equilibrium.
We study the excitation dynamics of Rydberg atoms in a one-dimensional lattice with periodic boundary conditions where the atomic Rydberg states are resonantly excited from the electronic ground state. Our description of the corresponding dynamics is numerically exact within the perfect blockade regime, i.e., no two atoms in a given range can be excited. The time evolution of the mean Rydberg density, density-density correlations, as well as entanglement properties is analyzed in detail. We demonstrate that the short-time dynamics is universal and dominated by quantum phenomena, while for larger time the characteristics of the lattice become important and the classical features determine the dynamics. The results of the perfect blockade approach are compared to the predictions of an effective Hamiltonian which includes the interaction of two neighboring Rydberg atoms up to the second-order perturbation theory.