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arXiv:0803.0239 · Physical Review Letters

Resonant Spin-Changing Collisions in Spinor Fermi Gases

N. Bornemann, P. Hyllus, Luis Santos

Published May 22, 2008• 5 citations
arXivHTMLPDF

Abstract

The compensation of quadratic Zeeman effect and trap energy in high-spin fermions is shown to lead to resonances in the spin-changing collisions that are typically absent in spinor condensates and spin-1/2 fermions. We study these resonances in lattice fermions, showing that they permit the targeting of a particular spin-changing channel while suppressing the rest and the creation of magnetically insensitive superpositions of many-body states with entangled spin and trap degrees of freedom. Finally, the intersite tunneling may lead to a quantum phase transition described by a quantum Ising model.

DOI
10.1103/physrevlett.100.205302

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The compensation of quadratic Zeeman effect and trap energy in high-spin fermions is shown to lead to resonances in the spin-changing collisions that are typically absent in spinor condensates and spin-1/2 fermions. We study these resonances in lattice fermions, showing that they permit the targeting of a particular spin-changing channel while suppressing the rest and the creation of magnetically insensitive superpositions of many-body states with entangled spin and trap degrees of freedom. Finally, the intersite tunneling may lead to a quantum phase transition described by a quantum Ising model.
The production of large-scale entangled states is one of the main goals of next-generation quantum technologies, with an immediate potential for applications in the context of entanglement-assisted quantum sensing. A very promising platform to achieve this goal is offered by ultracold spinor gases, made of atoms with a large internal spin sensitive to magnetic fields. Here we show that the native spin-changing collisions in a spinor Bose-Einstein condensate, combined with an arbitrary quadratic Zeeman shift, can generate scalable spin squeezing in the collective spin of the ensemble, following the universal paradigm of the celebrated one-axis-twisting model. Squeezing dynamics is driven by the quadratic Zeeman shift when this shift is small; and by the spin-changing collisions for large shifts, in the form of stroboscopic squeezing. Turning off the Zeeman shift freezes out the collective-spin dynamics, so that the ensuing collective spin dynamics can be uniquely governed by an external field to be sensed. Our theoretical results pave the way for the use of spinor Bose gases with a large spin in fundamental studies of entanglement, as well as in advanced metrological applications.
In this thesis we study various aspects of spinor Bose-Einstein condensates in optical superlattices using a Bose-Hubbard Hamiltonian that takes spin effects into account. We decouple the unit cells of the superlattice via a mean-field approach and take into account the dynamics within the unit cell exactly. In this way we derive the ground-state phase diagram of spinor bosons in superlattices. The system supports Mott-insulating as well as superfluid phases. The transitions between these phases are second-order for spinless bosons and second- or first-order for spin-1 bosons. Antiferromagnetic interactions energetically penalize high-spin configurations and elongate all Mott lobes, especially the ones corresponding to an even atom number on each lattice site. We find that the quadratic Zeeman effect lifts the degeneracy between different polar superfluid phases leading to additional metastable phases and first-order phase transitions. A change of magnetic fields can drive quantum phase transitions in the same way as a change in the tunneling amplitude does. Furthermore we study the physics of spin-1 atoms in superlattices deep in the Mott insulating phase when the superlattice decomposes into isolated double-well potentials. Assuming that a small number of spin-1 bosons is loaded in an optical double-well potential, we study single-particle tunneling that occurs when one lattice site is ramped up relative to a neighboring site. Spin-dependent effects modify the tunneling events in a qualitative and quantitative way. Depending on the asymmetry of the double well different types of magnetic order occur, making the system of spin-1 bosons in an optical superlattice a model for mesoscopic magnetism with an unprecedented control of the parameters. Homogeneous and inhomogeneous magnetic fields are applied and the effects of the linear and the quadratic Zeeman shifts are examined. We generalize the concept of bosonic staircases to connected double-well potentials. We show that an energy offset between the two sites of the unit cell in an extended superlattice induces a staircase of single-atom resonances in \nthe same way as in isolated double well. We also examine single-atom resonances in the superfluid regime and find clear fingerprints of them in the superfluid density. We also investigate the bipartite entanglement between the sites and construct states of maximal entanglement. The entanglement in our system is due to both orbital and spin degrees of freedom. We calculate the contribution of orbital and \nspin entanglement and show that the sum of these two terms gives a lower bound for the total entanglement.
We observe evidence of first-order superfluid-to-Mott-insulator quantum phase transitions in a lattice-confined antiferromagnetic spinor Bose-Einstein condensate. The observed signatures include the hysteresis effect, significant heatings across the phase transitions, and changes in spin populations due to the formation of spin singlets in the Mott-insulator phase. The nature of the phase transitions is found to strongly depend on the ratio of the quadratic Zeeman energy to the spin-dependent interaction. Our observations are qualitatively understood by the mean field theory and suggest tuning the quadratic Zeeman energy is a new approach to realize superfluid-to-Mott-insulator phase transitions.
I will discuss the spin dynamics of two magnetic atoms trapped in an external trap. Assuming that initially the atoms are in their orbital ground state I will discuss in details all possible elementary processes of spin flipping. Dipole-dipole interactions couple spin degrees of freedom of the two particles to their quantized orbital motion. Because of conservation of the total angular momentum if a magnetization of the system changes the system acquires an orbital angular momentum and atoms circulate around the center of the trap. I show that spin dynamics driven by dipolar interactions is possible only when the energies of the initial and the final sates are equal. In a case of weak magnetic moments of atoms this condition can be fulfilled utilizing a resonant external magnetic field, which tunes energies of involved states via the linear Zeeman effect. I will illustrate the resonant dynamics comparing the theoretical predictions to some results of experiments on Chromium atoms.
Bose-Einstein condensates of atoms with non-zero spin are known to constitute an ideal system to investigate fundamental properties of magnetic superfluids. More recently it was realized that they also provide the fascinating opportunity to investigate the macroscopic amplification of quantum and classical fluctuations. This is strikingly manifested in a sample initially prepared in the m F = 0 state, where spin-changing collisions triggered by quantum fluctuations may lead to the creation of correlated pairs in m F = ±1. We show that the pair creation efficiency is strongly influenced by the interplay between the external trapping potential and the Zeeman effect. It thus reflects the confinement-induced magnetic field dependence of elementary spin excitations of the condensate. Remarkably, pair production in our experiments is therefore characterized by a multi-resonant dependence on the magnetic field. Pair creation at these resonances acts as strong parametric matter-wave amplifier. Depending on the resonance condition, this amplification can be extremely sensitive or insensitive to the presence of seed atoms. We show that pair creation at a resonance which is insensitive to the presence of seed atoms is triggered purely by quantum fluctuations and thus the system acts as a matter-wave amplifier for the vacuum state.