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arXiv:0802.0243 · Physics Letters A

Phonon-induced decoherence of the two-level quantum subsystem due to relaxation and dephasing processes

L. А. Openov

Published Feb 12, 2008• 5 citations
arXivHTMLPDF
DOI
10.1016/j.physleta.2008.01.064

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Spin-phonon interactions are known to drive magnetic relaxation in solid-state systems but are generally overlooked as a contribution to spin decoherence through dephasing. Here, we extend quantum master equations to account for coherence terms and describe the full effect of up to two-phonon processes on spin dynamics. We implement this method fully ab initio for a molecule with large magnetization blocking temperature and show that, although strong axial magnetic anisotropy ensures slow magnetic relaxation approaching seconds at 77 kelvins, the superposition of Kramers doublets is coherent for less than 10 nanoseconds due to a two-phonon pure dephasing mechanism. This process, in principle, applies to any quantum system interacting with a thermal bath of phonons, advancing our understanding of quantum decoherence in solid-state systems.
We present a detailed theory for the Andreev level qubit, a system consisting of a highly transmissive quantum point contact embedded in a superconducting loop. The two-level Hamiltonian for Andreev levels interacting with quantum phase fluctuations is derived by using a path integral method. We also derive a kinetic equation describing qubit decoherence due to interaction of the Andreev levels with acoustic phonons. The collision terms are nonlinear due to the fermionic nature of the Andreev states, leading to slow nonexponential relaxation and dephasing of the qubit at temperatures smaller than the qubit level spacing.