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arXiv:0801.3577 · Physical Review B

Strongly correlated superconductivity arising in a pseudogap metal

Marco Schirò, Massimo Capone, Michele Fabrizio, Claudio Castellani

Published Mar 19, 2008• 11 citations
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Abstract

We solve by dynamical mean field theory a toy model that has a phase diagram strikingly similar to that of high-${T}_{c}$ superconductors: a bell-shaped superconducting region adjacent to the Mott insulator and a normal phase that evolves from a conventional Fermi liquid to a pseudogapped semimetal as the Mott transition is approached. Guided by the physics of the impurity model that is self-consistently solved within dynamical mean field theory, we introduce an analytical ansatz to model the dynamical behavior across the various phases which fits the numerical data very accurately. The ansatz is based on the assumption that the wave-function renormalization, which is very severe, especially in the pseudogap phase close to the Mott transition, is perfectly canceled by the vertex corrections in the Cooper pairing channel. A remarkable outcome is that a superconducting state can develop even from a pseudogapped normal state in which there are no low-energy quasiparticles. The overall physical scenario that emerges, although unraveled in a specific model and in an infinite-coordination Bethe lattice, can be interpreted in terms of arguments general enough to suggest that it can be realized in other correlated systems.

DOI
10.1103/physrevb.77.104522

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We solve by dynamical mean field theory a toy model that has a phase diagram strikingly similar to that of high-Tc{T}_{c}Tc​ superconductors: a bell-shaped superconducting region adjacent to the Mott insulator and a normal phase that evolves from a conventional Fermi liquid to a pseudogapped semimetal as the Mott transition is approached. Guided by the physics of the impurity model that is self-consistently solved within dynamical mean field theory, we introduce an analytical ansatz to model the dynamical behavior across the various phases which fits the numerical data very accurately. The ansatz is based on the assumption that the wave-function renormalization, which is very severe, especially in the pseudogap phase close to the Mott transition, is perfectly canceled by the vertex corrections in the Cooper pairing channel. A remarkable outcome is that a superconducting state can develop even from a pseudogapped normal state in which there are no low-energy quasiparticles. The overall physical scenario that emerges, although unraveled in a specific model and in an infinite-coordination Bethe lattice, can be interpreted in terms of arguments general enough to suggest that it can be realized in other correlated systems.
Near a Mott transition, strong electron correlations may enhance Cooper pairing. This is demonstrated in the dynamical mean field theory solution of a twofold-orbital degenerate Hubbard model with an inverted on-site Hund rule exchange, favoring local spin-singlet configurations. Close to the Mott insulator (which here is a local version of a valence bond insulator) a pseudogap non-Fermi-liquid metal, a superconductor, and a normal metal appear, in striking similarity with the physics of cuprates. The strongly correlated s-wave superconducting state has a larger Drude weight than the corresponding normal state. The role of the impurity Kondo problem is underscored.
We study the dynamics of the Cooper pairing across the T = 0 phase diagram of the two-dimensional Hubbard model, relevant for high-temperature superconductors, using a cluster extension of dynamical mean-field theory. We find that the superconducting pairing function evolves from an unconventional form in the overdoped region into a more conventional boson-mediated retarded form in the underdoped region of the phase diagram. The boson, however, promotes the rise of a pseudogap in the electron density of states rather than a superconducting gap as in the standard theory of superconductivity. We discuss our results in terms of Mott-related phenomena, and we show that they can be observed in tunneling experiments.
We generalize the dynamical-mean field (DMFT) approximation by including into the DMFT equations some length scale $\ensuremath{\xi}$ via a momentum dependent external self-energy ${\ensuremath{\Sigma}}_{\mathbf{k}}$. This external self-energy describes nonlocal dynamical correlations induced by the short-ranged collective spin density wave--like antiferromagnetic spin (or the charge density wave--like charge) fluctuations. At high enough temperatures these fluctuations can be viewed as a quenched Gaussian random field with a finite correlation length. This generalized $\mathrm{DMFT}+{\ensuremath{\Sigma}}_{\mathbf{k}}$ approach is used for the numerical solution of the weakly doped one-band Hubbard model with repulsive Coulomb interaction on a square lattice with the nearest and the next nearest neighbor hopping. The effective single impurity problem in this generalized $\mathrm{DMFT}+{\ensuremath{\Sigma}}_{\mathbf{k}}$ is solved by the numerical renormalization group. Both types of the strongly correlated metals, namely: (i) The doped Mott insulator and (ii) the case of the bandwidth $W\ensuremath{\lesssim}U$ (UUU---value of the local Coulomb interaction) are considered. The densities of states, the spectral functions, and the angle resolved photoemission spectra calculated within the $\mathrm{DMFT}+{\ensuremath{\Sigma}}_{\mathbf{k}}$ show a pseudogap formation near the Fermi level of the quasiparticle band.
An intricate interplay between superconductivity, pseudogap, and Mott transition, either bandwidth driven or doping driven, occurs in materials. Layered organic conductors and cuprates offer two prime examples. We provide a unified perspective of this interplay in the two-dimensional Hubbard model within cellular dynamical mean-field theory on a 2×2 plaquette and using the continuous-time quantum Monte Carlo method as impurity solver. Both at half filling and at finite doping, the metallic normal state close to the Mott insulator is unstable to d-wave superconductivity. Superconductivity can destroy the first-order transition that separates the pseudogap phase from the overdoped metal, yet that normal state transition leaves its marks on the dynamic properties of the superconducting phase. For example, as a function of doping one finds a rapid change in the particle-hole asymmetry of the superconducting density of states. In the doped Mott insulator, the dynamical mean-field superconducting transition temperature T(c)(d) does not scale with the order parameter when there is a normal-state pseudogap. T(c)(d) corresponds to the local pair formation temperature observed in tunneling experiments and is distinct from the pseudogap temperature.
High-temperature superconductivity emerges upon doping a state of matter that is insulating because of interactions. A widely studied model considers one orbital per CuO2{\mathrm{CuO}}_{2}CuO2​ unit cell on a square lattice with a strong intraorbital repulsion that leads to a so-called Mott-Hubbard insulator. Here we solve a model that takes into account, within each unit cell, two oxygen orbitals where there is no electron-electron repulsion and a copper orbital with strong electron-electron repulsion. The insulating phase is a so-called charge-transfer insulator, not a Mott-Hubbard insulator. Using cluster dynamical mean-field theory with continuous-time quantum Monte Carlo as an impurity solver and 12 atoms per cluster, we report the normal and superconducting phase diagram of this model as a function of doping, interaction strength, and temperature. As expected, the three-orbital model is consistent with the experimental observation that doped holes are located predominantly on oxygens, a result that goes beyond the one-orbital model. Nevertheless, the phase boundary between pseudogap and correlated metal, the Widom line, and the origin of the pairing energy (kinetic vs potential) are similar to the one-orbital model, demonstrating that these are emergent phenomena characteristic of doped Mott insulators, independently of many microscopic details. Broader implications are discussed.
The pseudogap state of cuprate high-temperature superconductors has been often viewed as either a yet unknown competing order or a precursor state to superconductivity. While awaiting the resolution of the pseudogap problem in cuprates, we demonstrate that local pairing fluctuations, vortex liquid dynamics, and other precursor phenomena can emerge quite generally whenever fermionic excitations remain gapped across the superconducting transition, regardless of the gap origin. Our choice of a tractable model is a lattice band insulator with short-range attractive interactions between fermions in the sss-wave channel. An effective crossover between Bardeen-Cooper-Schrieffer (BCS) and Bose-Einstein condensate (BEC) regimes can be identified in any band insulator above two dimensions, while in two dimensions only the BEC regime exists. The superconducting transition is ``unconventional'' (non-pair-breaking) in the BEC regime, identified by either the bosonic mean field or XY\mathit{XY}XY universality class. The insulator adjacent to the superconductor in the BEC regime is a bosonic Mott insulator of Cooper pairs, which may be susceptible to charge density wave ordering. We construct a function of the many-body excitation spectrum whose nonanalytic changes define a sharp distinction between band and Mott insulators. The corresponding ``second-order transition'' can be observed out of equilibrium by driving a Cooper pair laser in the Mott insulator. We explicitly show that the gap for charged bosonic excitations lies below the threshold for Cooper pair breakup in any BEC regime, despite quantum fluctuations. Our discussion ends with a view of possible consequences for cuprates, where antinodal pair dynamics has certain features in common with our simple sss-wave picture.