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arXiv:0812.1201 · Physical Review Letters

Evolution of the Dynamical Pairing across the Phase Diagram of a Strongly Correlated High-Temperature Superconductor

Marcello Civelli

Published Sep 24, 2009• 33 citations
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Abstract

We study the dynamics of the Cooper pairing across the T = 0 phase diagram of the two-dimensional Hubbard model, relevant for high-temperature superconductors, using a cluster extension of dynamical mean-field theory. We find that the superconducting pairing function evolves from an unconventional form in the overdoped region into a more conventional boson-mediated retarded form in the underdoped region of the phase diagram. The boson, however, promotes the rise of a pseudogap in the electron density of states rather than a superconducting gap as in the standard theory of superconductivity. We discuss our results in terms of Mott-related phenomena, and we show that they can be observed in tunneling experiments.

DOI
10.1103/physrevlett.103.136402

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•Aug 17, 2016•22 citations
We study the dynamics of the Cooper pairing across the T = 0 phase diagram of the two-dimensional Hubbard model, relevant for high-temperature superconductors, using a cluster extension of dynamical mean-field theory. We find that the superconducting pairing function evolves from an unconventional form in the overdoped region into a more conventional boson-mediated retarded form in the underdoped region of the phase diagram. The boson, however, promotes the rise of a pseudogap in the electron density of states rather than a superconducting gap as in the standard theory of superconductivity. We discuss our results in terms of Mott-related phenomena, and we show that they can be observed in tunneling experiments.
Abstract We investigate the interplay between the pseudogap state and d-wave superconductivity in the two-dimensional doped Hubbard model by employing an eight-site cluster dynamical mean-field theory method. By tuning electron hopping parameters, the strong-coupling pseudogap in the two-dimensional Hubbard model can be either enhanced or suppressed in the doped Mott insulator regime. We find that in underdoped cases, the closing of pseudogap leads to a significant enhancement of superconductivity, indicating competition between the two in the underdoped regime. In contrast, at large dopings, suppressing the pseudogap is accompanied by a concurrent decrease in the superconducting transition temperature T c, which can be attributed to a reduction in antiferromagnetic correlations behind both the pseudogap and superconductivity. We elucidate this evolving relationship between pseudogap and superconductivity across different doping regimes.
We solve by dynamical mean field theory a toy model that has a phase diagram strikingly similar to that of high-Tc{T}_{c}Tc​ superconductors: a bell-shaped superconducting region adjacent to the Mott insulator and a normal phase that evolves from a conventional Fermi liquid to a pseudogapped semimetal as the Mott transition is approached. Guided by the physics of the impurity model that is self-consistently solved within dynamical mean field theory, we introduce an analytical ansatz to model the dynamical behavior across the various phases which fits the numerical data very accurately. The ansatz is based on the assumption that the wave-function renormalization, which is very severe, especially in the pseudogap phase close to the Mott transition, is perfectly canceled by the vertex corrections in the Cooper pairing channel. A remarkable outcome is that a superconducting state can develop even from a pseudogapped normal state in which there are no low-energy quasiparticles. The overall physical scenario that emerges, although unraveled in a specific model and in an infinite-coordination Bethe lattice, can be interpreted in terms of arguments general enough to suggest that it can be realized in other correlated systems.
The pseudogap state of cuprate high-temperature superconductors has been often viewed as either a yet unknown competing order or a precursor state to superconductivity. While awaiting the resolution of the pseudogap problem in cuprates, we demonstrate that local pairing fluctuations, vortex liquid dynamics, and other precursor phenomena can emerge quite generally whenever fermionic excitations remain gapped across the superconducting transition, regardless of the gap origin. Our choice of a tractable model is a lattice band insulator with short-range attractive interactions between fermions in the sss-wave channel. An effective crossover between Bardeen-Cooper-Schrieffer (BCS) and Bose-Einstein condensate (BEC) regimes can be identified in any band insulator above two dimensions, while in two dimensions only the BEC regime exists. The superconducting transition is ``unconventional'' (non-pair-breaking) in the BEC regime, identified by either the bosonic mean field or XY\mathit{XY}XY universality class. The insulator adjacent to the superconductor in the BEC regime is a bosonic Mott insulator of Cooper pairs, which may be susceptible to charge density wave ordering. We construct a function of the many-body excitation spectrum whose nonanalytic changes define a sharp distinction between band and Mott insulators. The corresponding ``second-order transition'' can be observed out of equilibrium by driving a Cooper pair laser in the Mott insulator. We explicitly show that the gap for charged bosonic excitations lies below the threshold for Cooper pair breakup in any BEC regime, despite quantum fluctuations. Our discussion ends with a view of possible consequences for cuprates, where antinodal pair dynamics has certain features in common with our simple sss-wave picture.
The dynamics of a microscopic cuprate model, namely, the two-dimensional Hubbard model, is studied with a cluster extension of the dynamical mean-field theory. We find a nontrivial structure of the frequency-dependent self-energies, which describes an unprecedented interplay between the pseudogap and superconductivity. We show that these properties are well described by quasiparticles hybridizing with (hidden) fermionic excitations, emergent from the strong electronic correlations. The hidden fermion enhances superconductivity via a mechanism distinct from a conventional boson-mediated pairing, and originates the normal-state pseudogap. Though the hidden fermion is elusive in experiments, it can solve many experimental puzzles.
In this paper we investigate the zero-temperature doping-driven evolution of a superconductor toward the Mott insulator in a two-dimensional electron model, relevant for high-temperature superconductivity. To this purpose we use a cluster extension of dynamical mean-field theory. Our results show that a standard ddd-wave superconductor, realized at high doping, is driven into the Mott insulator via an intermediate superconducting state displaying unconventional physical properties. By restoring the translational invariance of the lattice, we give an interpretation of these findings in momentum space. In particular, we show that at a finite doping a strong momentum-space differentiation takes place: non-Fermi liquid and insulatinglike (pseudogap) characters rise in some regions (antinodes), while Fermi liquid quasiparticles survive in other regions (nodes) of momentum space. We describe the consequence of these happenings on the spectral properties, stressing in particular the behavior of the superconducting gap, which reveals two distinct nodal and antinodal energy scales as a function of doping, detected in photoemission and Raman spectroscopy experiments. We study and compare with experimental results the doping-dependent behavior of other physical quantities, such as for instance, the nodal quasiparticle velocity (extracted in angle-resolved photoemission) and the low-energy slopes of the local density of states and of the Raman scattering response. We then propose a description of the evolution of the electronic structure while approaching the Mott transition. We show that, within our formalism, a strong asymmetry naturally arises in the local density of states, measured in scanning tunneling spectroscopy. We investigate in detail the doping evolution of the electronic bands, focusing on the kinklike quasiparticle dispersion observed with angle-resolved photoemission in specific cuts of the momentum-energy space. We finally show the consequences of the properties presented above in the doping dependence of the Hall resistivity, measured in magnetotransport experiments.
Underdoped Mott insulators provide us with a challenge of many-body physics. Recent renewed understanding is discussed in terms of the evolution of pole and zero structure of the single-particle Green's function. Pseudogap as well as Fermi arc/pocket structure in the underdoped cuprates is well reproduced from the recent cluster extension of the dynamical mean-field theory. Emergent coexisting zeros and poles set the underdoped Mott insulator apart from the Fermi liquid, separated by topological transitions. Cofermion proposed as a generalization of exciton in the slave-boson framework accounts for the origin of the zero surface formation. The cofermion-quasiparticle hybridization gap offers a natural understanding of the pseudogap and various unusual Mottness. Furthermore the cofermion offers a novel pairing mechanism, where the cofermion has two roles: It reinforces the Cooper pair as a pair partner of the quasiparticle and acts as a glue as well. It provides a strong insight for solving the puzzle found in the dichotomy of the gap structure.